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Ionic Liquid@Metal-Organic Framework as a Solid Electrolyte in a Lithium-Ion Battery: Current Performance and Perspective at Molecular Level

Searching for a suitable electrolyte in a lithium-ion battery is a challenging task. The electrolyte must not only be chemically and mechanically stable, but also be able to transport lithium ions efficiently. Ionic liquid incorporated into a metal–organic framework (IL@MOF) has currently emerged as...

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Autores principales: Majid, Mohd Faridzuan, Mohd Zaid, Hayyiratul Fatimah, Kait, Chong Fai, Ahmad, Azizan, Jumbri, Khairulazhar
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9000457/
https://www.ncbi.nlm.nih.gov/pubmed/35407194
http://dx.doi.org/10.3390/nano12071076
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author Majid, Mohd Faridzuan
Mohd Zaid, Hayyiratul Fatimah
Kait, Chong Fai
Ahmad, Azizan
Jumbri, Khairulazhar
author_facet Majid, Mohd Faridzuan
Mohd Zaid, Hayyiratul Fatimah
Kait, Chong Fai
Ahmad, Azizan
Jumbri, Khairulazhar
author_sort Majid, Mohd Faridzuan
collection PubMed
description Searching for a suitable electrolyte in a lithium-ion battery is a challenging task. The electrolyte must not only be chemically and mechanically stable, but also be able to transport lithium ions efficiently. Ionic liquid incorporated into a metal–organic framework (IL@MOF) has currently emerged as an interesting class of hybrid material that could offer excellent electrochemical properties. However, the understanding of the mechanism and factors that govern its fast ionic conduction is crucial as well. In this review, the characteristics and potential use of IL@MOF as an electrolyte in a lithium-ion battery are highlighted. The importance of computational methods is emphasized as a comprehensive tool to investigate the atomistic behavior of IL@MOF and its interaction in electrochemical environments.
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spelling pubmed-90004572022-04-12 Ionic Liquid@Metal-Organic Framework as a Solid Electrolyte in a Lithium-Ion Battery: Current Performance and Perspective at Molecular Level Majid, Mohd Faridzuan Mohd Zaid, Hayyiratul Fatimah Kait, Chong Fai Ahmad, Azizan Jumbri, Khairulazhar Nanomaterials (Basel) Review Searching for a suitable electrolyte in a lithium-ion battery is a challenging task. The electrolyte must not only be chemically and mechanically stable, but also be able to transport lithium ions efficiently. Ionic liquid incorporated into a metal–organic framework (IL@MOF) has currently emerged as an interesting class of hybrid material that could offer excellent electrochemical properties. However, the understanding of the mechanism and factors that govern its fast ionic conduction is crucial as well. In this review, the characteristics and potential use of IL@MOF as an electrolyte in a lithium-ion battery are highlighted. The importance of computational methods is emphasized as a comprehensive tool to investigate the atomistic behavior of IL@MOF and its interaction in electrochemical environments. MDPI 2022-03-25 /pmc/articles/PMC9000457/ /pubmed/35407194 http://dx.doi.org/10.3390/nano12071076 Text en © 2022 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Review
Majid, Mohd Faridzuan
Mohd Zaid, Hayyiratul Fatimah
Kait, Chong Fai
Ahmad, Azizan
Jumbri, Khairulazhar
Ionic Liquid@Metal-Organic Framework as a Solid Electrolyte in a Lithium-Ion Battery: Current Performance and Perspective at Molecular Level
title Ionic Liquid@Metal-Organic Framework as a Solid Electrolyte in a Lithium-Ion Battery: Current Performance and Perspective at Molecular Level
title_full Ionic Liquid@Metal-Organic Framework as a Solid Electrolyte in a Lithium-Ion Battery: Current Performance and Perspective at Molecular Level
title_fullStr Ionic Liquid@Metal-Organic Framework as a Solid Electrolyte in a Lithium-Ion Battery: Current Performance and Perspective at Molecular Level
title_full_unstemmed Ionic Liquid@Metal-Organic Framework as a Solid Electrolyte in a Lithium-Ion Battery: Current Performance and Perspective at Molecular Level
title_short Ionic Liquid@Metal-Organic Framework as a Solid Electrolyte in a Lithium-Ion Battery: Current Performance and Perspective at Molecular Level
title_sort ionic liquid@metal-organic framework as a solid electrolyte in a lithium-ion battery: current performance and perspective at molecular level
topic Review
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9000457/
https://www.ncbi.nlm.nih.gov/pubmed/35407194
http://dx.doi.org/10.3390/nano12071076
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