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Facile Preparation of Loose P84 Copolyimide/GO Composite Membrane with Excellent Selectivity and Solvent Resistance
In this study, multilayer graphene oxide (GO) was used to prepare the functional layer of polyimide/GO composite membrane with polyimide (P84) used as the supporting layer. Chitosan added in the functional layer was utilized to adjust the selectivity of the composite membrane. The effects of GO and...
Autores principales: | , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
MDPI
2022
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9002502/ https://www.ncbi.nlm.nih.gov/pubmed/35406229 http://dx.doi.org/10.3390/polym14071353 |
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author | Han, Runlin Wu, Kui Xu, Lingfeng |
author_facet | Han, Runlin Wu, Kui Xu, Lingfeng |
author_sort | Han, Runlin |
collection | PubMed |
description | In this study, multilayer graphene oxide (GO) was used to prepare the functional layer of polyimide/GO composite membrane with polyimide (P84) used as the supporting layer. Chitosan added in the functional layer was utilized to adjust the selectivity of the composite membrane. The effects of GO and chitosan contents on membrane morphology and separation performance were investigated in detail. The composite membrane showed high rejection to Congo red and Methyl orange with high flux but low rejection to Na(2)SO(4) and MgCl(2) at 0.2 MPa and ambient temperature. The membrane exhibited excellent solvent resistance in N,N-dimethylacetamide (DMAc) after being crosslinked with 0.5 wt.% triethylene tetramine. The result means that a highly selective and solvent-resistant P84/GO composite membrane was prepared with the facile filtration preparation method. |
format | Online Article Text |
id | pubmed-9002502 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2022 |
publisher | MDPI |
record_format | MEDLINE/PubMed |
spelling | pubmed-90025022022-04-13 Facile Preparation of Loose P84 Copolyimide/GO Composite Membrane with Excellent Selectivity and Solvent Resistance Han, Runlin Wu, Kui Xu, Lingfeng Polymers (Basel) Communication In this study, multilayer graphene oxide (GO) was used to prepare the functional layer of polyimide/GO composite membrane with polyimide (P84) used as the supporting layer. Chitosan added in the functional layer was utilized to adjust the selectivity of the composite membrane. The effects of GO and chitosan contents on membrane morphology and separation performance were investigated in detail. The composite membrane showed high rejection to Congo red and Methyl orange with high flux but low rejection to Na(2)SO(4) and MgCl(2) at 0.2 MPa and ambient temperature. The membrane exhibited excellent solvent resistance in N,N-dimethylacetamide (DMAc) after being crosslinked with 0.5 wt.% triethylene tetramine. The result means that a highly selective and solvent-resistant P84/GO composite membrane was prepared with the facile filtration preparation method. MDPI 2022-03-27 /pmc/articles/PMC9002502/ /pubmed/35406229 http://dx.doi.org/10.3390/polym14071353 Text en © 2022 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/). |
spellingShingle | Communication Han, Runlin Wu, Kui Xu, Lingfeng Facile Preparation of Loose P84 Copolyimide/GO Composite Membrane with Excellent Selectivity and Solvent Resistance |
title | Facile Preparation of Loose P84 Copolyimide/GO Composite Membrane with Excellent Selectivity and Solvent Resistance |
title_full | Facile Preparation of Loose P84 Copolyimide/GO Composite Membrane with Excellent Selectivity and Solvent Resistance |
title_fullStr | Facile Preparation of Loose P84 Copolyimide/GO Composite Membrane with Excellent Selectivity and Solvent Resistance |
title_full_unstemmed | Facile Preparation of Loose P84 Copolyimide/GO Composite Membrane with Excellent Selectivity and Solvent Resistance |
title_short | Facile Preparation of Loose P84 Copolyimide/GO Composite Membrane with Excellent Selectivity and Solvent Resistance |
title_sort | facile preparation of loose p84 copolyimide/go composite membrane with excellent selectivity and solvent resistance |
topic | Communication |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9002502/ https://www.ncbi.nlm.nih.gov/pubmed/35406229 http://dx.doi.org/10.3390/polym14071353 |
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