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Anisotropy-driven quantum criticality in an intermediate valence system

Intermetallic compounds containing f-electron elements have been prototypical materials for investigating strong electron correlations and quantum criticality (QC). Their heavy fermion ground state evoked by the magnetic f-electrons is susceptible to the onset of quantum phases, such as magnetism or...

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Detalles Bibliográficos
Autores principales: Grbić, Mihael S., O’Farrell, Eoin C. T., Matsumoto, Yosuke, Kuga, Kentaro, Brando, Manuel, Küchler, Robert, Nevidomskyy, Andriy H., Yoshida, Makoto, Sakakibara, Toshiro, Kono, Yohei, Shimura, Yasuyuki, Sutherland, Michael L., Takigawa, Masashi, Nakatsuji, Satoru
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9019086/
https://www.ncbi.nlm.nih.gov/pubmed/35440657
http://dx.doi.org/10.1038/s41467-022-29757-9
Descripción
Sumario:Intermetallic compounds containing f-electron elements have been prototypical materials for investigating strong electron correlations and quantum criticality (QC). Their heavy fermion ground state evoked by the magnetic f-electrons is susceptible to the onset of quantum phases, such as magnetism or superconductivity, due to the enhanced effective mass (m(*)) and a corresponding decrease of the Fermi temperature. However, the presence of f-electron valence fluctuations to a non-magnetic state is regarded an anathema to QC, as it usually generates a paramagnetic Fermi-liquid state with quasiparticles of moderate m(*). Such systems are typically isotropic, with a characteristic energy scale T(0) of the order of hundreds of kelvins that require large magnetic fields or pressures to promote a valence or magnetic instability. Here we show the discovery of a quantum critical behaviour and a Lifshitz transition under low magnetic field in an intermediate valence compound α-YbAlB(4). The QC origin is attributed to the anisotropic hybridization between the conduction and localized f-electrons. These findings suggest a new route to bypass the large valence energy scale in developing the QC.