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Anisotropy-driven quantum criticality in an intermediate valence system

Intermetallic compounds containing f-electron elements have been prototypical materials for investigating strong electron correlations and quantum criticality (QC). Their heavy fermion ground state evoked by the magnetic f-electrons is susceptible to the onset of quantum phases, such as magnetism or...

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Autores principales: Grbić, Mihael S., O’Farrell, Eoin C. T., Matsumoto, Yosuke, Kuga, Kentaro, Brando, Manuel, Küchler, Robert, Nevidomskyy, Andriy H., Yoshida, Makoto, Sakakibara, Toshiro, Kono, Yohei, Shimura, Yasuyuki, Sutherland, Michael L., Takigawa, Masashi, Nakatsuji, Satoru
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9019086/
https://www.ncbi.nlm.nih.gov/pubmed/35440657
http://dx.doi.org/10.1038/s41467-022-29757-9
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author Grbić, Mihael S.
O’Farrell, Eoin C. T.
Matsumoto, Yosuke
Kuga, Kentaro
Brando, Manuel
Küchler, Robert
Nevidomskyy, Andriy H.
Yoshida, Makoto
Sakakibara, Toshiro
Kono, Yohei
Shimura, Yasuyuki
Sutherland, Michael L.
Takigawa, Masashi
Nakatsuji, Satoru
author_facet Grbić, Mihael S.
O’Farrell, Eoin C. T.
Matsumoto, Yosuke
Kuga, Kentaro
Brando, Manuel
Küchler, Robert
Nevidomskyy, Andriy H.
Yoshida, Makoto
Sakakibara, Toshiro
Kono, Yohei
Shimura, Yasuyuki
Sutherland, Michael L.
Takigawa, Masashi
Nakatsuji, Satoru
author_sort Grbić, Mihael S.
collection PubMed
description Intermetallic compounds containing f-electron elements have been prototypical materials for investigating strong electron correlations and quantum criticality (QC). Their heavy fermion ground state evoked by the magnetic f-electrons is susceptible to the onset of quantum phases, such as magnetism or superconductivity, due to the enhanced effective mass (m(*)) and a corresponding decrease of the Fermi temperature. However, the presence of f-electron valence fluctuations to a non-magnetic state is regarded an anathema to QC, as it usually generates a paramagnetic Fermi-liquid state with quasiparticles of moderate m(*). Such systems are typically isotropic, with a characteristic energy scale T(0) of the order of hundreds of kelvins that require large magnetic fields or pressures to promote a valence or magnetic instability. Here we show the discovery of a quantum critical behaviour and a Lifshitz transition under low magnetic field in an intermediate valence compound α-YbAlB(4). The QC origin is attributed to the anisotropic hybridization between the conduction and localized f-electrons. These findings suggest a new route to bypass the large valence energy scale in developing the QC.
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spelling pubmed-90190862022-04-28 Anisotropy-driven quantum criticality in an intermediate valence system Grbić, Mihael S. O’Farrell, Eoin C. T. Matsumoto, Yosuke Kuga, Kentaro Brando, Manuel Küchler, Robert Nevidomskyy, Andriy H. Yoshida, Makoto Sakakibara, Toshiro Kono, Yohei Shimura, Yasuyuki Sutherland, Michael L. Takigawa, Masashi Nakatsuji, Satoru Nat Commun Article Intermetallic compounds containing f-electron elements have been prototypical materials for investigating strong electron correlations and quantum criticality (QC). Their heavy fermion ground state evoked by the magnetic f-electrons is susceptible to the onset of quantum phases, such as magnetism or superconductivity, due to the enhanced effective mass (m(*)) and a corresponding decrease of the Fermi temperature. However, the presence of f-electron valence fluctuations to a non-magnetic state is regarded an anathema to QC, as it usually generates a paramagnetic Fermi-liquid state with quasiparticles of moderate m(*). Such systems are typically isotropic, with a characteristic energy scale T(0) of the order of hundreds of kelvins that require large magnetic fields or pressures to promote a valence or magnetic instability. Here we show the discovery of a quantum critical behaviour and a Lifshitz transition under low magnetic field in an intermediate valence compound α-YbAlB(4). The QC origin is attributed to the anisotropic hybridization between the conduction and localized f-electrons. These findings suggest a new route to bypass the large valence energy scale in developing the QC. Nature Publishing Group UK 2022-04-19 /pmc/articles/PMC9019086/ /pubmed/35440657 http://dx.doi.org/10.1038/s41467-022-29757-9 Text en © The Author(s) 2022 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Grbić, Mihael S.
O’Farrell, Eoin C. T.
Matsumoto, Yosuke
Kuga, Kentaro
Brando, Manuel
Küchler, Robert
Nevidomskyy, Andriy H.
Yoshida, Makoto
Sakakibara, Toshiro
Kono, Yohei
Shimura, Yasuyuki
Sutherland, Michael L.
Takigawa, Masashi
Nakatsuji, Satoru
Anisotropy-driven quantum criticality in an intermediate valence system
title Anisotropy-driven quantum criticality in an intermediate valence system
title_full Anisotropy-driven quantum criticality in an intermediate valence system
title_fullStr Anisotropy-driven quantum criticality in an intermediate valence system
title_full_unstemmed Anisotropy-driven quantum criticality in an intermediate valence system
title_short Anisotropy-driven quantum criticality in an intermediate valence system
title_sort anisotropy-driven quantum criticality in an intermediate valence system
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9019086/
https://www.ncbi.nlm.nih.gov/pubmed/35440657
http://dx.doi.org/10.1038/s41467-022-29757-9
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