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Minute-Scale Synthesis of Nano Silicalite-1 Zeolites
Synthesis of zeolites in more efficient and greener methods is of great significance in both industrial and academic fields. However, the relative long time for zeolite crystallization and much consumption of water solvent make the target challengeable. Herein, a route for ultrafast synthesis of nan...
Autores principales: | , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Frontiers Media S.A.
2022
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9024212/ https://www.ncbi.nlm.nih.gov/pubmed/35464233 http://dx.doi.org/10.3389/fchem.2022.860795 |
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author | Zhang, Changsheng Chu, Shaoqi Jiang, Jie Zhao, Jinchong Wen, Song Sun, Bing Xu, Wei |
author_facet | Zhang, Changsheng Chu, Shaoqi Jiang, Jie Zhao, Jinchong Wen, Song Sun, Bing Xu, Wei |
author_sort | Zhang, Changsheng |
collection | PubMed |
description | Synthesis of zeolites in more efficient and greener methods is of great significance in both industrial and academic fields. However, the relative long time for zeolite crystallization and much consumption of water solvent make the target challengeable. Herein, a route for ultrafast synthesis of nano Silicalite-1 zeolites in 10 min with much less water consumption has been developed. Comprehensive characterizations, i.e., X-ray powder diffraction, N(2) sorption, scanning electron microscope, and NMR, confirm the high quality of such obtained Silicalite-1 zeolites. In the catalytic deoxygenation of O(2)-containing ethylene (mixture of O(2) and ethylene), these reported Silicalite-1 zeolite samples show the comparable performance with the conventional Silicalite-1 zeolites synthesized under hydrothermal conditions. This research therefore provides a new trial toward the ultrafast synthesis of zeolite materials in an environment-friendly route. |
format | Online Article Text |
id | pubmed-9024212 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2022 |
publisher | Frontiers Media S.A. |
record_format | MEDLINE/PubMed |
spelling | pubmed-90242122022-04-23 Minute-Scale Synthesis of Nano Silicalite-1 Zeolites Zhang, Changsheng Chu, Shaoqi Jiang, Jie Zhao, Jinchong Wen, Song Sun, Bing Xu, Wei Front Chem Chemistry Synthesis of zeolites in more efficient and greener methods is of great significance in both industrial and academic fields. However, the relative long time for zeolite crystallization and much consumption of water solvent make the target challengeable. Herein, a route for ultrafast synthesis of nano Silicalite-1 zeolites in 10 min with much less water consumption has been developed. Comprehensive characterizations, i.e., X-ray powder diffraction, N(2) sorption, scanning electron microscope, and NMR, confirm the high quality of such obtained Silicalite-1 zeolites. In the catalytic deoxygenation of O(2)-containing ethylene (mixture of O(2) and ethylene), these reported Silicalite-1 zeolite samples show the comparable performance with the conventional Silicalite-1 zeolites synthesized under hydrothermal conditions. This research therefore provides a new trial toward the ultrafast synthesis of zeolite materials in an environment-friendly route. Frontiers Media S.A. 2022-04-08 /pmc/articles/PMC9024212/ /pubmed/35464233 http://dx.doi.org/10.3389/fchem.2022.860795 Text en Copyright © 2022 Zhang, Chu, Jiang, Zhao, Wen, Sun and Xu. https://creativecommons.org/licenses/by/4.0/This is an open-access article distributed under the terms of the Creative Commons Attribution License (CC BY). The use, distribution or reproduction in other forums is permitted, provided the original author(s) and the copyright owner(s) are credited and that the original publication in this journal is cited, in accordance with accepted academic practice. No use, distribution or reproduction is permitted which does not comply with these terms. |
spellingShingle | Chemistry Zhang, Changsheng Chu, Shaoqi Jiang, Jie Zhao, Jinchong Wen, Song Sun, Bing Xu, Wei Minute-Scale Synthesis of Nano Silicalite-1 Zeolites |
title | Minute-Scale Synthesis of Nano Silicalite-1 Zeolites |
title_full | Minute-Scale Synthesis of Nano Silicalite-1 Zeolites |
title_fullStr | Minute-Scale Synthesis of Nano Silicalite-1 Zeolites |
title_full_unstemmed | Minute-Scale Synthesis of Nano Silicalite-1 Zeolites |
title_short | Minute-Scale Synthesis of Nano Silicalite-1 Zeolites |
title_sort | minute-scale synthesis of nano silicalite-1 zeolites |
topic | Chemistry |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9024212/ https://www.ncbi.nlm.nih.gov/pubmed/35464233 http://dx.doi.org/10.3389/fchem.2022.860795 |
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