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Over 65% Sunlight Absorption in a 1 μm Si Slab with Hyperuniform Texture

[Image: see text] Thin, flexible, and invisible solar cells will be a ubiquitous technology in the near future. Ultrathin crystalline silicon (c-Si) cells capitalize on the success of bulk silicon cells while being lightweight and mechanically flexible, but suffer from poor absorption and efficiency...

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Autores principales: Tavakoli, Nasim, Spalding, Richard, Lambertz, Alexander, Koppejan, Pepijn, Gkantzounis, Georgios, Wan, Chenglong, Röhrich, Ruslan, Kontoleta, Evgenia, Koenderink, A. Femius, Sapienza, Riccardo, Florescu, Marian, Alarcon-Llado, Esther
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2022
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9026274/
https://www.ncbi.nlm.nih.gov/pubmed/35480493
http://dx.doi.org/10.1021/acsphotonics.1c01668
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author Tavakoli, Nasim
Spalding, Richard
Lambertz, Alexander
Koppejan, Pepijn
Gkantzounis, Georgios
Wan, Chenglong
Röhrich, Ruslan
Kontoleta, Evgenia
Koenderink, A. Femius
Sapienza, Riccardo
Florescu, Marian
Alarcon-Llado, Esther
author_facet Tavakoli, Nasim
Spalding, Richard
Lambertz, Alexander
Koppejan, Pepijn
Gkantzounis, Georgios
Wan, Chenglong
Röhrich, Ruslan
Kontoleta, Evgenia
Koenderink, A. Femius
Sapienza, Riccardo
Florescu, Marian
Alarcon-Llado, Esther
author_sort Tavakoli, Nasim
collection PubMed
description [Image: see text] Thin, flexible, and invisible solar cells will be a ubiquitous technology in the near future. Ultrathin crystalline silicon (c-Si) cells capitalize on the success of bulk silicon cells while being lightweight and mechanically flexible, but suffer from poor absorption and efficiency. Here we present a new family of surface texturing, based on correlated disordered hyperuniform patterns, capable of efficiently coupling the incident spectrum into the silicon slab optical modes. We experimentally demonstrate 66.5% solar light absorption in free-standing 1 μm c-Si layers by hyperuniform nanostructuring for the spectral range of 400 to 1050 nm. The absorption equivalent photocurrent derived from our measurements is 26.3 mA/cm(2), which is far above the highest found in literature for Si of similar thickness. Considering state-of-the-art Si PV technologies, we estimate that the enhanced light trapping can result in a cell efficiency above 15%. The light absorption can potentially be increased up to 33.8 mA/cm(2) by incorporating a back-reflector and improved antireflection, for which we estimate a photovoltaic efficiency above 21% for 1 μm thick Si cells.
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spelling pubmed-90262742022-04-25 Over 65% Sunlight Absorption in a 1 μm Si Slab with Hyperuniform Texture Tavakoli, Nasim Spalding, Richard Lambertz, Alexander Koppejan, Pepijn Gkantzounis, Georgios Wan, Chenglong Röhrich, Ruslan Kontoleta, Evgenia Koenderink, A. Femius Sapienza, Riccardo Florescu, Marian Alarcon-Llado, Esther ACS Photonics [Image: see text] Thin, flexible, and invisible solar cells will be a ubiquitous technology in the near future. Ultrathin crystalline silicon (c-Si) cells capitalize on the success of bulk silicon cells while being lightweight and mechanically flexible, but suffer from poor absorption and efficiency. Here we present a new family of surface texturing, based on correlated disordered hyperuniform patterns, capable of efficiently coupling the incident spectrum into the silicon slab optical modes. We experimentally demonstrate 66.5% solar light absorption in free-standing 1 μm c-Si layers by hyperuniform nanostructuring for the spectral range of 400 to 1050 nm. The absorption equivalent photocurrent derived from our measurements is 26.3 mA/cm(2), which is far above the highest found in literature for Si of similar thickness. Considering state-of-the-art Si PV technologies, we estimate that the enhanced light trapping can result in a cell efficiency above 15%. The light absorption can potentially be increased up to 33.8 mA/cm(2) by incorporating a back-reflector and improved antireflection, for which we estimate a photovoltaic efficiency above 21% for 1 μm thick Si cells. American Chemical Society 2022-03-22 2022-04-20 /pmc/articles/PMC9026274/ /pubmed/35480493 http://dx.doi.org/10.1021/acsphotonics.1c01668 Text en © 2022 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by/4.0/Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Tavakoli, Nasim
Spalding, Richard
Lambertz, Alexander
Koppejan, Pepijn
Gkantzounis, Georgios
Wan, Chenglong
Röhrich, Ruslan
Kontoleta, Evgenia
Koenderink, A. Femius
Sapienza, Riccardo
Florescu, Marian
Alarcon-Llado, Esther
Over 65% Sunlight Absorption in a 1 μm Si Slab with Hyperuniform Texture
title Over 65% Sunlight Absorption in a 1 μm Si Slab with Hyperuniform Texture
title_full Over 65% Sunlight Absorption in a 1 μm Si Slab with Hyperuniform Texture
title_fullStr Over 65% Sunlight Absorption in a 1 μm Si Slab with Hyperuniform Texture
title_full_unstemmed Over 65% Sunlight Absorption in a 1 μm Si Slab with Hyperuniform Texture
title_short Over 65% Sunlight Absorption in a 1 μm Si Slab with Hyperuniform Texture
title_sort over 65% sunlight absorption in a 1 μm si slab with hyperuniform texture
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9026274/
https://www.ncbi.nlm.nih.gov/pubmed/35480493
http://dx.doi.org/10.1021/acsphotonics.1c01668
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