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Boosting charge separation and nitrogen vacancies in graphitic carbon nitride by implanted strontium vanadate for highly efficient photocatalytic reduction of hexavalent chromium
Strontium vanadate nanoparticles embedded graphitic carbon nitride (g-C(3)N(4)/Sr(2)V(2)O(7)) was facilely prepared in situ via a hydrothermal method. It was shown that the Sr(2)V(2)O(7) nanoparticles implanted into g-carbon nitride had a small size and high distribution. Importantly, compared with...
Autores principales: | , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
The Royal Society of Chemistry
2021
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9030169/ https://www.ncbi.nlm.nih.gov/pubmed/35481208 http://dx.doi.org/10.1039/d1ra01489g |
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author | Zhou, Yuzhi Kang, Shi-Zhao Qin, Lixia Li, Xiangqing |
author_facet | Zhou, Yuzhi Kang, Shi-Zhao Qin, Lixia Li, Xiangqing |
author_sort | Zhou, Yuzhi |
collection | PubMed |
description | Strontium vanadate nanoparticles embedded graphitic carbon nitride (g-C(3)N(4)/Sr(2)V(2)O(7)) was facilely prepared in situ via a hydrothermal method. It was shown that the Sr(2)V(2)O(7) nanoparticles implanted into g-carbon nitride had a small size and high distribution. Importantly, compared with some other photocatalysts, the as-prepared g-C(3)N(4)/Sr(2)V(2)O(7) nanohybrid showed excellent photocatalytic activity for reduction of Cr(vi), and as high as 99% efficiency for Cr(vi) reduction (100 mg L(−1)) was reached within 8 min. Moreover, its activity was hardly changed after five cycles, demonstrating that the developed g-C(3)N(4)/Sr(2)V(2)O(7) nanohybrid was highly stable and promising an efficacious disposal of Cr(vi) in water. It was confirmed that the improved charge separation owing to more nitrogen vacancies in the hybrid was the main reason for the improved performance of the g-C(3)N(4)-Sr(2)V(2)O(7) nanohybrid. |
format | Online Article Text |
id | pubmed-9030169 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2021 |
publisher | The Royal Society of Chemistry |
record_format | MEDLINE/PubMed |
spelling | pubmed-90301692022-04-26 Boosting charge separation and nitrogen vacancies in graphitic carbon nitride by implanted strontium vanadate for highly efficient photocatalytic reduction of hexavalent chromium Zhou, Yuzhi Kang, Shi-Zhao Qin, Lixia Li, Xiangqing RSC Adv Chemistry Strontium vanadate nanoparticles embedded graphitic carbon nitride (g-C(3)N(4)/Sr(2)V(2)O(7)) was facilely prepared in situ via a hydrothermal method. It was shown that the Sr(2)V(2)O(7) nanoparticles implanted into g-carbon nitride had a small size and high distribution. Importantly, compared with some other photocatalysts, the as-prepared g-C(3)N(4)/Sr(2)V(2)O(7) nanohybrid showed excellent photocatalytic activity for reduction of Cr(vi), and as high as 99% efficiency for Cr(vi) reduction (100 mg L(−1)) was reached within 8 min. Moreover, its activity was hardly changed after five cycles, demonstrating that the developed g-C(3)N(4)/Sr(2)V(2)O(7) nanohybrid was highly stable and promising an efficacious disposal of Cr(vi) in water. It was confirmed that the improved charge separation owing to more nitrogen vacancies in the hybrid was the main reason for the improved performance of the g-C(3)N(4)-Sr(2)V(2)O(7) nanohybrid. The Royal Society of Chemistry 2021-04-29 /pmc/articles/PMC9030169/ /pubmed/35481208 http://dx.doi.org/10.1039/d1ra01489g Text en This journal is © The Royal Society of Chemistry https://creativecommons.org/licenses/by-nc/3.0/ |
spellingShingle | Chemistry Zhou, Yuzhi Kang, Shi-Zhao Qin, Lixia Li, Xiangqing Boosting charge separation and nitrogen vacancies in graphitic carbon nitride by implanted strontium vanadate for highly efficient photocatalytic reduction of hexavalent chromium |
title | Boosting charge separation and nitrogen vacancies in graphitic carbon nitride by implanted strontium vanadate for highly efficient photocatalytic reduction of hexavalent chromium |
title_full | Boosting charge separation and nitrogen vacancies in graphitic carbon nitride by implanted strontium vanadate for highly efficient photocatalytic reduction of hexavalent chromium |
title_fullStr | Boosting charge separation and nitrogen vacancies in graphitic carbon nitride by implanted strontium vanadate for highly efficient photocatalytic reduction of hexavalent chromium |
title_full_unstemmed | Boosting charge separation and nitrogen vacancies in graphitic carbon nitride by implanted strontium vanadate for highly efficient photocatalytic reduction of hexavalent chromium |
title_short | Boosting charge separation and nitrogen vacancies in graphitic carbon nitride by implanted strontium vanadate for highly efficient photocatalytic reduction of hexavalent chromium |
title_sort | boosting charge separation and nitrogen vacancies in graphitic carbon nitride by implanted strontium vanadate for highly efficient photocatalytic reduction of hexavalent chromium |
topic | Chemistry |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9030169/ https://www.ncbi.nlm.nih.gov/pubmed/35481208 http://dx.doi.org/10.1039/d1ra01489g |
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