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A study on the high efficiency reduction of p-nitrophenol (4-NP) by a Fe(OH)(3)/Fe(2)O(3)@Au composite catalyst
Precious metal nanometric catalysts are widely used in the removal of harmful substances. In the process of synthesis and catalytic reaction, it is particularly important to study green and simple synthesis methods and high catalytic efficiency. In this paper, a green one-step method was used to syn...
Autores principales: | , , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
The Royal Society of Chemistry
2021
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9037387/ https://www.ncbi.nlm.nih.gov/pubmed/35479987 http://dx.doi.org/10.1039/d1ra04073a |
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author | Fu, Meirong Li, Mingqiang Zhao, Yingying Bai, Yunxiang Fang, Xingzhong Kang, Xiaolong Yang, Min Wei, Yanping Xu, Xia |
author_facet | Fu, Meirong Li, Mingqiang Zhao, Yingying Bai, Yunxiang Fang, Xingzhong Kang, Xiaolong Yang, Min Wei, Yanping Xu, Xia |
author_sort | Fu, Meirong |
collection | PubMed |
description | Precious metal nanometric catalysts are widely used in the removal of harmful substances. In the process of synthesis and catalytic reaction, it is particularly important to study green and simple synthesis methods and high catalytic efficiency. In this paper, a green one-step method was used to synthesize the Fe(OH)(3)/Fe(2)O(3)@Au composite catalyst, in which Au was single atom-dispersed. The removal of 4-nitrophenol (4-NP), a typical dangerous chemical widely existing in factory waste gas, waste water and automobile exhaust gas, was catalysed by Fe(OH)(3)/Fe(2)O(3)@Au. The catalytic performance of Fe(OH)(3)/Fe(2)O(3)@Au with different synthesis conditions (different amounts of MES, NaBH(4), FeSO(4), Au and Pt) on the 4-NP reduction reaction were systematically studied. Finally, the stability and recyclability of Fe(OH)(3)/Fe(2)O(3)@Au composite nanocatalyst were investigated thoroughly. |
format | Online Article Text |
id | pubmed-9037387 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2021 |
publisher | The Royal Society of Chemistry |
record_format | MEDLINE/PubMed |
spelling | pubmed-90373872022-04-26 A study on the high efficiency reduction of p-nitrophenol (4-NP) by a Fe(OH)(3)/Fe(2)O(3)@Au composite catalyst Fu, Meirong Li, Mingqiang Zhao, Yingying Bai, Yunxiang Fang, Xingzhong Kang, Xiaolong Yang, Min Wei, Yanping Xu, Xia RSC Adv Chemistry Precious metal nanometric catalysts are widely used in the removal of harmful substances. In the process of synthesis and catalytic reaction, it is particularly important to study green and simple synthesis methods and high catalytic efficiency. In this paper, a green one-step method was used to synthesize the Fe(OH)(3)/Fe(2)O(3)@Au composite catalyst, in which Au was single atom-dispersed. The removal of 4-nitrophenol (4-NP), a typical dangerous chemical widely existing in factory waste gas, waste water and automobile exhaust gas, was catalysed by Fe(OH)(3)/Fe(2)O(3)@Au. The catalytic performance of Fe(OH)(3)/Fe(2)O(3)@Au with different synthesis conditions (different amounts of MES, NaBH(4), FeSO(4), Au and Pt) on the 4-NP reduction reaction were systematically studied. Finally, the stability and recyclability of Fe(OH)(3)/Fe(2)O(3)@Au composite nanocatalyst were investigated thoroughly. The Royal Society of Chemistry 2021-08-03 /pmc/articles/PMC9037387/ /pubmed/35479987 http://dx.doi.org/10.1039/d1ra04073a Text en This journal is © The Royal Society of Chemistry https://creativecommons.org/licenses/by-nc/3.0/ |
spellingShingle | Chemistry Fu, Meirong Li, Mingqiang Zhao, Yingying Bai, Yunxiang Fang, Xingzhong Kang, Xiaolong Yang, Min Wei, Yanping Xu, Xia A study on the high efficiency reduction of p-nitrophenol (4-NP) by a Fe(OH)(3)/Fe(2)O(3)@Au composite catalyst |
title | A study on the high efficiency reduction of p-nitrophenol (4-NP) by a Fe(OH)(3)/Fe(2)O(3)@Au composite catalyst |
title_full | A study on the high efficiency reduction of p-nitrophenol (4-NP) by a Fe(OH)(3)/Fe(2)O(3)@Au composite catalyst |
title_fullStr | A study on the high efficiency reduction of p-nitrophenol (4-NP) by a Fe(OH)(3)/Fe(2)O(3)@Au composite catalyst |
title_full_unstemmed | A study on the high efficiency reduction of p-nitrophenol (4-NP) by a Fe(OH)(3)/Fe(2)O(3)@Au composite catalyst |
title_short | A study on the high efficiency reduction of p-nitrophenol (4-NP) by a Fe(OH)(3)/Fe(2)O(3)@Au composite catalyst |
title_sort | study on the high efficiency reduction of p-nitrophenol (4-np) by a fe(oh)(3)/fe(2)o(3)@au composite catalyst |
topic | Chemistry |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9037387/ https://www.ncbi.nlm.nih.gov/pubmed/35479987 http://dx.doi.org/10.1039/d1ra04073a |
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