Cargando…

A study on the high efficiency reduction of p-nitrophenol (4-NP) by a Fe(OH)(3)/Fe(2)O(3)@Au composite catalyst

Precious metal nanometric catalysts are widely used in the removal of harmful substances. In the process of synthesis and catalytic reaction, it is particularly important to study green and simple synthesis methods and high catalytic efficiency. In this paper, a green one-step method was used to syn...

Descripción completa

Detalles Bibliográficos
Autores principales: Fu, Meirong, Li, Mingqiang, Zhao, Yingying, Bai, Yunxiang, Fang, Xingzhong, Kang, Xiaolong, Yang, Min, Wei, Yanping, Xu, Xia
Formato: Online Artículo Texto
Lenguaje:English
Publicado: The Royal Society of Chemistry 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9037387/
https://www.ncbi.nlm.nih.gov/pubmed/35479987
http://dx.doi.org/10.1039/d1ra04073a
_version_ 1784693726321311744
author Fu, Meirong
Li, Mingqiang
Zhao, Yingying
Bai, Yunxiang
Fang, Xingzhong
Kang, Xiaolong
Yang, Min
Wei, Yanping
Xu, Xia
author_facet Fu, Meirong
Li, Mingqiang
Zhao, Yingying
Bai, Yunxiang
Fang, Xingzhong
Kang, Xiaolong
Yang, Min
Wei, Yanping
Xu, Xia
author_sort Fu, Meirong
collection PubMed
description Precious metal nanometric catalysts are widely used in the removal of harmful substances. In the process of synthesis and catalytic reaction, it is particularly important to study green and simple synthesis methods and high catalytic efficiency. In this paper, a green one-step method was used to synthesize the Fe(OH)(3)/Fe(2)O(3)@Au composite catalyst, in which Au was single atom-dispersed. The removal of 4-nitrophenol (4-NP), a typical dangerous chemical widely existing in factory waste gas, waste water and automobile exhaust gas, was catalysed by Fe(OH)(3)/Fe(2)O(3)@Au. The catalytic performance of Fe(OH)(3)/Fe(2)O(3)@Au with different synthesis conditions (different amounts of MES, NaBH(4), FeSO(4), Au and Pt) on the 4-NP reduction reaction were systematically studied. Finally, the stability and recyclability of Fe(OH)(3)/Fe(2)O(3)@Au composite nanocatalyst were investigated thoroughly.
format Online
Article
Text
id pubmed-9037387
institution National Center for Biotechnology Information
language English
publishDate 2021
publisher The Royal Society of Chemistry
record_format MEDLINE/PubMed
spelling pubmed-90373872022-04-26 A study on the high efficiency reduction of p-nitrophenol (4-NP) by a Fe(OH)(3)/Fe(2)O(3)@Au composite catalyst Fu, Meirong Li, Mingqiang Zhao, Yingying Bai, Yunxiang Fang, Xingzhong Kang, Xiaolong Yang, Min Wei, Yanping Xu, Xia RSC Adv Chemistry Precious metal nanometric catalysts are widely used in the removal of harmful substances. In the process of synthesis and catalytic reaction, it is particularly important to study green and simple synthesis methods and high catalytic efficiency. In this paper, a green one-step method was used to synthesize the Fe(OH)(3)/Fe(2)O(3)@Au composite catalyst, in which Au was single atom-dispersed. The removal of 4-nitrophenol (4-NP), a typical dangerous chemical widely existing in factory waste gas, waste water and automobile exhaust gas, was catalysed by Fe(OH)(3)/Fe(2)O(3)@Au. The catalytic performance of Fe(OH)(3)/Fe(2)O(3)@Au with different synthesis conditions (different amounts of MES, NaBH(4), FeSO(4), Au and Pt) on the 4-NP reduction reaction were systematically studied. Finally, the stability and recyclability of Fe(OH)(3)/Fe(2)O(3)@Au composite nanocatalyst were investigated thoroughly. The Royal Society of Chemistry 2021-08-03 /pmc/articles/PMC9037387/ /pubmed/35479987 http://dx.doi.org/10.1039/d1ra04073a Text en This journal is © The Royal Society of Chemistry https://creativecommons.org/licenses/by-nc/3.0/
spellingShingle Chemistry
Fu, Meirong
Li, Mingqiang
Zhao, Yingying
Bai, Yunxiang
Fang, Xingzhong
Kang, Xiaolong
Yang, Min
Wei, Yanping
Xu, Xia
A study on the high efficiency reduction of p-nitrophenol (4-NP) by a Fe(OH)(3)/Fe(2)O(3)@Au composite catalyst
title A study on the high efficiency reduction of p-nitrophenol (4-NP) by a Fe(OH)(3)/Fe(2)O(3)@Au composite catalyst
title_full A study on the high efficiency reduction of p-nitrophenol (4-NP) by a Fe(OH)(3)/Fe(2)O(3)@Au composite catalyst
title_fullStr A study on the high efficiency reduction of p-nitrophenol (4-NP) by a Fe(OH)(3)/Fe(2)O(3)@Au composite catalyst
title_full_unstemmed A study on the high efficiency reduction of p-nitrophenol (4-NP) by a Fe(OH)(3)/Fe(2)O(3)@Au composite catalyst
title_short A study on the high efficiency reduction of p-nitrophenol (4-NP) by a Fe(OH)(3)/Fe(2)O(3)@Au composite catalyst
title_sort study on the high efficiency reduction of p-nitrophenol (4-np) by a fe(oh)(3)/fe(2)o(3)@au composite catalyst
topic Chemistry
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9037387/
https://www.ncbi.nlm.nih.gov/pubmed/35479987
http://dx.doi.org/10.1039/d1ra04073a
work_keys_str_mv AT fumeirong astudyonthehighefficiencyreductionofpnitrophenol4npbyafeoh3fe2o3aucompositecatalyst
AT limingqiang astudyonthehighefficiencyreductionofpnitrophenol4npbyafeoh3fe2o3aucompositecatalyst
AT zhaoyingying astudyonthehighefficiencyreductionofpnitrophenol4npbyafeoh3fe2o3aucompositecatalyst
AT baiyunxiang astudyonthehighefficiencyreductionofpnitrophenol4npbyafeoh3fe2o3aucompositecatalyst
AT fangxingzhong astudyonthehighefficiencyreductionofpnitrophenol4npbyafeoh3fe2o3aucompositecatalyst
AT kangxiaolong astudyonthehighefficiencyreductionofpnitrophenol4npbyafeoh3fe2o3aucompositecatalyst
AT yangmin astudyonthehighefficiencyreductionofpnitrophenol4npbyafeoh3fe2o3aucompositecatalyst
AT weiyanping astudyonthehighefficiencyreductionofpnitrophenol4npbyafeoh3fe2o3aucompositecatalyst
AT xuxia astudyonthehighefficiencyreductionofpnitrophenol4npbyafeoh3fe2o3aucompositecatalyst
AT fumeirong studyonthehighefficiencyreductionofpnitrophenol4npbyafeoh3fe2o3aucompositecatalyst
AT limingqiang studyonthehighefficiencyreductionofpnitrophenol4npbyafeoh3fe2o3aucompositecatalyst
AT zhaoyingying studyonthehighefficiencyreductionofpnitrophenol4npbyafeoh3fe2o3aucompositecatalyst
AT baiyunxiang studyonthehighefficiencyreductionofpnitrophenol4npbyafeoh3fe2o3aucompositecatalyst
AT fangxingzhong studyonthehighefficiencyreductionofpnitrophenol4npbyafeoh3fe2o3aucompositecatalyst
AT kangxiaolong studyonthehighefficiencyreductionofpnitrophenol4npbyafeoh3fe2o3aucompositecatalyst
AT yangmin studyonthehighefficiencyreductionofpnitrophenol4npbyafeoh3fe2o3aucompositecatalyst
AT weiyanping studyonthehighefficiencyreductionofpnitrophenol4npbyafeoh3fe2o3aucompositecatalyst
AT xuxia studyonthehighefficiencyreductionofpnitrophenol4npbyafeoh3fe2o3aucompositecatalyst