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Scaling of a catalytic cracking fluidized bed downer reactor based on computational fluid dynamics simulations

Circulating fluidized bed downer reactors (downer reactors) exhibit good heat and mass transfer, and the flow behavior approaches the ideal plug flow. This reactor is superior for catalytic cracking reactions in which the intermediate is the desired product. However, the hydrodynamic behavior and re...

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Autores principales: Khongprom, Parinya, Ratchasombat, Supawadee, Wanchan, Waritnan, Bumphenkiattikul, Panut, Limtrakul, Sunun
Formato: Online Artículo Texto
Lenguaje:English
Publicado: The Royal Society of Chemistry 2020
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9048978/
https://www.ncbi.nlm.nih.gov/pubmed/35496099
http://dx.doi.org/10.1039/c9ra10080f
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author Khongprom, Parinya
Ratchasombat, Supawadee
Wanchan, Waritnan
Bumphenkiattikul, Panut
Limtrakul, Sunun
author_facet Khongprom, Parinya
Ratchasombat, Supawadee
Wanchan, Waritnan
Bumphenkiattikul, Panut
Limtrakul, Sunun
author_sort Khongprom, Parinya
collection PubMed
description Circulating fluidized bed downer reactors (downer reactors) exhibit good heat and mass transfer, and the flow behavior approaches the ideal plug flow. This reactor is superior for catalytic cracking reactions in which the intermediate is the desired product. However, the hydrodynamic behavior and reactor performance have mostly been investigated in small-scale or laboratory-scale reactors. The objective of this study was to investigate the up-scaling of the catalytic cracking of heavy oil in three downer reactors with heights of 5, 15, and 30 m, using computational fluid dynamics simulations. A two-fluid model with the kinetic theory of granular flow was used to predict the hydrodynamics and performance of the chemical reactions. The kinetics of catalytic cracking of heavy oil were described by a 4-lump kinetic model. The chemical performance similarity was identified by using radial and axial distributions of heavy oil conversion, gasoline mass fraction, and gasoline selectivity. The chemical performance similarity cannot be achieved by using the hydrodynamic similarity parameter [Image: see text]. A modified up-scaling parameter was proposed, [Image: see text]. The chemical performance similarity of identical catalytic cracking downer reactors can be achieved with deviation in the range of ±10% and mean relative absolute error of less than 5%.
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spelling pubmed-90489782022-04-28 Scaling of a catalytic cracking fluidized bed downer reactor based on computational fluid dynamics simulations Khongprom, Parinya Ratchasombat, Supawadee Wanchan, Waritnan Bumphenkiattikul, Panut Limtrakul, Sunun RSC Adv Chemistry Circulating fluidized bed downer reactors (downer reactors) exhibit good heat and mass transfer, and the flow behavior approaches the ideal plug flow. This reactor is superior for catalytic cracking reactions in which the intermediate is the desired product. However, the hydrodynamic behavior and reactor performance have mostly been investigated in small-scale or laboratory-scale reactors. The objective of this study was to investigate the up-scaling of the catalytic cracking of heavy oil in three downer reactors with heights of 5, 15, and 30 m, using computational fluid dynamics simulations. A two-fluid model with the kinetic theory of granular flow was used to predict the hydrodynamics and performance of the chemical reactions. The kinetics of catalytic cracking of heavy oil were described by a 4-lump kinetic model. The chemical performance similarity was identified by using radial and axial distributions of heavy oil conversion, gasoline mass fraction, and gasoline selectivity. The chemical performance similarity cannot be achieved by using the hydrodynamic similarity parameter [Image: see text]. A modified up-scaling parameter was proposed, [Image: see text]. The chemical performance similarity of identical catalytic cracking downer reactors can be achieved with deviation in the range of ±10% and mean relative absolute error of less than 5%. The Royal Society of Chemistry 2020-01-16 /pmc/articles/PMC9048978/ /pubmed/35496099 http://dx.doi.org/10.1039/c9ra10080f Text en This journal is © The Royal Society of Chemistry https://creativecommons.org/licenses/by-nc/3.0/
spellingShingle Chemistry
Khongprom, Parinya
Ratchasombat, Supawadee
Wanchan, Waritnan
Bumphenkiattikul, Panut
Limtrakul, Sunun
Scaling of a catalytic cracking fluidized bed downer reactor based on computational fluid dynamics simulations
title Scaling of a catalytic cracking fluidized bed downer reactor based on computational fluid dynamics simulations
title_full Scaling of a catalytic cracking fluidized bed downer reactor based on computational fluid dynamics simulations
title_fullStr Scaling of a catalytic cracking fluidized bed downer reactor based on computational fluid dynamics simulations
title_full_unstemmed Scaling of a catalytic cracking fluidized bed downer reactor based on computational fluid dynamics simulations
title_short Scaling of a catalytic cracking fluidized bed downer reactor based on computational fluid dynamics simulations
title_sort scaling of a catalytic cracking fluidized bed downer reactor based on computational fluid dynamics simulations
topic Chemistry
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9048978/
https://www.ncbi.nlm.nih.gov/pubmed/35496099
http://dx.doi.org/10.1039/c9ra10080f
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