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Novel organic–inorganic hybrid powder SrGa(12)O(19):Mn(2+)–ethyl cellulose for efficient latent fingerprint recognition via time-gated fluorescence

Latent fingerprints (LFPs) are important evidence in crime scenes and forensic investigations, but they are invisible to the naked eye. In this work, a novel fluorescent probe was developed by integrating a narrow-band-emitting green afterglow phosphor, SrGa(12)O(19):Mn(2+) (SGO:Mn), and ethyl cellu...

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Autores principales: Lai, Jun'an, Long, Zhangwen, Qiu, Jianbei, Zhou, Dacheng, Wang, Qi, Yang, Yong, Hu, Songhan, Wang, Zhe, Zhang, Ke
Formato: Online Artículo Texto
Lenguaje:English
Publicado: The Royal Society of Chemistry 2020
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9049934/
https://www.ncbi.nlm.nih.gov/pubmed/35497857
http://dx.doi.org/10.1039/d0ra00138d
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author Lai, Jun'an
Long, Zhangwen
Qiu, Jianbei
Zhou, Dacheng
Wang, Qi
Yang, Yong
Hu, Songhan
Wang, Zhe
Zhang, Ke
author_facet Lai, Jun'an
Long, Zhangwen
Qiu, Jianbei
Zhou, Dacheng
Wang, Qi
Yang, Yong
Hu, Songhan
Wang, Zhe
Zhang, Ke
author_sort Lai, Jun'an
collection PubMed
description Latent fingerprints (LFPs) are important evidence in crime scenes and forensic investigations, but they are invisible to the naked eye. In this work, a novel fluorescent probe was developed by integrating a narrow-band-emitting green afterglow phosphor, SrGa(12)O(19):Mn(2+) (SGO:Mn), and ethyl cellulose (EC) for the efficient visualization of LFPs. The hydrophobic interactions between the powder and lipid-rich LFPs made the ridge structures more defined and easily identifiable. The background fluorescence of the substrates was completely avoided because of the time-gated fluorescence of the afterglow phosphor. All the three levels of LFP degrees were clearly imaged due to the high sensitivity. Moreover, the SGO:Mn–EC powder was highly stable in neutral, acidic, and alkaline environments. In addition, 60 day-aged LFPs were successfully visualized by the powder. All performances showed that this strategy for LFP recognition has merits such as low cost, non-destructive nature, reliability, superior universality, and legible details. Together, these results show the great application prospects of this powder in forensic identification and criminal investigation.
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spelling pubmed-90499342022-04-29 Novel organic–inorganic hybrid powder SrGa(12)O(19):Mn(2+)–ethyl cellulose for efficient latent fingerprint recognition via time-gated fluorescence Lai, Jun'an Long, Zhangwen Qiu, Jianbei Zhou, Dacheng Wang, Qi Yang, Yong Hu, Songhan Wang, Zhe Zhang, Ke RSC Adv Chemistry Latent fingerprints (LFPs) are important evidence in crime scenes and forensic investigations, but they are invisible to the naked eye. In this work, a novel fluorescent probe was developed by integrating a narrow-band-emitting green afterglow phosphor, SrGa(12)O(19):Mn(2+) (SGO:Mn), and ethyl cellulose (EC) for the efficient visualization of LFPs. The hydrophobic interactions between the powder and lipid-rich LFPs made the ridge structures more defined and easily identifiable. The background fluorescence of the substrates was completely avoided because of the time-gated fluorescence of the afterglow phosphor. All the three levels of LFP degrees were clearly imaged due to the high sensitivity. Moreover, the SGO:Mn–EC powder was highly stable in neutral, acidic, and alkaline environments. In addition, 60 day-aged LFPs were successfully visualized by the powder. All performances showed that this strategy for LFP recognition has merits such as low cost, non-destructive nature, reliability, superior universality, and legible details. Together, these results show the great application prospects of this powder in forensic identification and criminal investigation. The Royal Society of Chemistry 2020-02-26 /pmc/articles/PMC9049934/ /pubmed/35497857 http://dx.doi.org/10.1039/d0ra00138d Text en This journal is © The Royal Society of Chemistry https://creativecommons.org/licenses/by/3.0/
spellingShingle Chemistry
Lai, Jun'an
Long, Zhangwen
Qiu, Jianbei
Zhou, Dacheng
Wang, Qi
Yang, Yong
Hu, Songhan
Wang, Zhe
Zhang, Ke
Novel organic–inorganic hybrid powder SrGa(12)O(19):Mn(2+)–ethyl cellulose for efficient latent fingerprint recognition via time-gated fluorescence
title Novel organic–inorganic hybrid powder SrGa(12)O(19):Mn(2+)–ethyl cellulose for efficient latent fingerprint recognition via time-gated fluorescence
title_full Novel organic–inorganic hybrid powder SrGa(12)O(19):Mn(2+)–ethyl cellulose for efficient latent fingerprint recognition via time-gated fluorescence
title_fullStr Novel organic–inorganic hybrid powder SrGa(12)O(19):Mn(2+)–ethyl cellulose for efficient latent fingerprint recognition via time-gated fluorescence
title_full_unstemmed Novel organic–inorganic hybrid powder SrGa(12)O(19):Mn(2+)–ethyl cellulose for efficient latent fingerprint recognition via time-gated fluorescence
title_short Novel organic–inorganic hybrid powder SrGa(12)O(19):Mn(2+)–ethyl cellulose for efficient latent fingerprint recognition via time-gated fluorescence
title_sort novel organic–inorganic hybrid powder srga(12)o(19):mn(2+)–ethyl cellulose for efficient latent fingerprint recognition via time-gated fluorescence
topic Chemistry
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9049934/
https://www.ncbi.nlm.nih.gov/pubmed/35497857
http://dx.doi.org/10.1039/d0ra00138d
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