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Carbon electrode engineering for high efficiency all-inorganic perovskite solar cells

Carbon-based inorganic perovskite solar cells (PSCs) have demonstrated an excellent performance in the field of photovoltaics owing to their simple fabrication techniques, low-cost and superior stability. Despite the lower efficiency of devices with a carbon electrode compared with the conventional...

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Detalles Bibliográficos
Autores principales: Mi, Longfei, Zhang, Yan, Chen, Taotao, Xu, Enze, Jiang, Yang
Formato: Online Artículo Texto
Lenguaje:English
Publicado: The Royal Society of Chemistry 2020
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9051046/
https://www.ncbi.nlm.nih.gov/pubmed/35497632
http://dx.doi.org/10.1039/d0ra00288g
Descripción
Sumario:Carbon-based inorganic perovskite solar cells (PSCs) have demonstrated an excellent performance in the field of photovoltaics owing to their simple fabrication techniques, low-cost and superior stability. Despite the lower efficiency of devices with a carbon electrode compared with the conventional structure, the potential applications in large scale have attracted increasing attention. Herein, we employ a mixed carbon electrode inorganic PSC by incorporating one-dimensional structure carbon nanotubes (CNTs) and two-dimensional Ti(3)C(2)-MXene nanosheets into a commercial carbon paste. This mixed carbon electrode, which is different from the pure carbon electrode in showing a point-to-point contact, provides a network structure and multi-dimensional charge transfer path, which effectively increases the conductivity of the carbon electrode and carriers transport. A respectable power conversion efficiency of 7.09% is obtained through carbon/CNT/MXene mixed electrode in CsPbBr(3)-based solar cells.