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Efficient electrocatalyst of α-Fe(2)O(3) nanorings for oxygen evolution reaction in acidic conditions
Large-scale application of sustainable energy devices urgently requires cost-effective electrocatalysts to overcome the sluggish kinetics related to the oxygen evolution reaction (OER) under acidic conditions. Here, we first report the highly efficient electrocatalytic characteristics of α-Fe(2)O(3)...
Autores principales: | , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
The Royal Society of Chemistry
2020
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9055951/ https://www.ncbi.nlm.nih.gov/pubmed/35521123 http://dx.doi.org/10.1039/d0ra04262e |
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author | Liang, Xiaolei Qian, Jinmei Liu, Yonggang Zhang, Zhengmei Gao, Daqiang |
author_facet | Liang, Xiaolei Qian, Jinmei Liu, Yonggang Zhang, Zhengmei Gao, Daqiang |
author_sort | Liang, Xiaolei |
collection | PubMed |
description | Large-scale application of sustainable energy devices urgently requires cost-effective electrocatalysts to overcome the sluggish kinetics related to the oxygen evolution reaction (OER) under acidic conditions. Here, we first report the highly efficient electrocatalytic characteristics of α-Fe(2)O(3) nanorings (NRs), which exhibits prominent OER electrocatalytic activity with lower overpotential of 1.43 V at 10 mA cm(−2) and great stability in 1 M HCl, surpassing the start-of-the art Ir/C electrocatalyst. The significantly optimized OER activity of the α-Fe(2)O(3) NRs mainly attributes to the synergistic effect of the excellent electrical conductivity and a large effective active surface because of their unique nanoring structure, disordered surface, and the dynamic stability of α-Fe(2)O(3) NRs in acidic conditions. |
format | Online Article Text |
id | pubmed-9055951 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2020 |
publisher | The Royal Society of Chemistry |
record_format | MEDLINE/PubMed |
spelling | pubmed-90559512022-05-04 Efficient electrocatalyst of α-Fe(2)O(3) nanorings for oxygen evolution reaction in acidic conditions Liang, Xiaolei Qian, Jinmei Liu, Yonggang Zhang, Zhengmei Gao, Daqiang RSC Adv Chemistry Large-scale application of sustainable energy devices urgently requires cost-effective electrocatalysts to overcome the sluggish kinetics related to the oxygen evolution reaction (OER) under acidic conditions. Here, we first report the highly efficient electrocatalytic characteristics of α-Fe(2)O(3) nanorings (NRs), which exhibits prominent OER electrocatalytic activity with lower overpotential of 1.43 V at 10 mA cm(−2) and great stability in 1 M HCl, surpassing the start-of-the art Ir/C electrocatalyst. The significantly optimized OER activity of the α-Fe(2)O(3) NRs mainly attributes to the synergistic effect of the excellent electrical conductivity and a large effective active surface because of their unique nanoring structure, disordered surface, and the dynamic stability of α-Fe(2)O(3) NRs in acidic conditions. The Royal Society of Chemistry 2020-08-06 /pmc/articles/PMC9055951/ /pubmed/35521123 http://dx.doi.org/10.1039/d0ra04262e Text en This journal is © The Royal Society of Chemistry https://creativecommons.org/licenses/by-nc/3.0/ |
spellingShingle | Chemistry Liang, Xiaolei Qian, Jinmei Liu, Yonggang Zhang, Zhengmei Gao, Daqiang Efficient electrocatalyst of α-Fe(2)O(3) nanorings for oxygen evolution reaction in acidic conditions |
title | Efficient electrocatalyst of α-Fe(2)O(3) nanorings for oxygen evolution reaction in acidic conditions |
title_full | Efficient electrocatalyst of α-Fe(2)O(3) nanorings for oxygen evolution reaction in acidic conditions |
title_fullStr | Efficient electrocatalyst of α-Fe(2)O(3) nanorings for oxygen evolution reaction in acidic conditions |
title_full_unstemmed | Efficient electrocatalyst of α-Fe(2)O(3) nanorings for oxygen evolution reaction in acidic conditions |
title_short | Efficient electrocatalyst of α-Fe(2)O(3) nanorings for oxygen evolution reaction in acidic conditions |
title_sort | efficient electrocatalyst of α-fe(2)o(3) nanorings for oxygen evolution reaction in acidic conditions |
topic | Chemistry |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9055951/ https://www.ncbi.nlm.nih.gov/pubmed/35521123 http://dx.doi.org/10.1039/d0ra04262e |
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