Cargando…
Cadmium sulfide net framework nanoparticles for photo-catalyzed cell redox
A strategy for synthesizing cadmium sulfide net framework (CdS-NF) nanoparticles was developed in a water-based system under mild reaction conditions. The CdS-NFs have not only the excellent photocatalytic properties of CdS, but also the large surface area and diverse porous structures of a metal–or...
Autores principales: | , , , , , , |
---|---|
Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
The Royal Society of Chemistry
2020
|
Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9057183/ https://www.ncbi.nlm.nih.gov/pubmed/35515163 http://dx.doi.org/10.1039/d0ra08235j |
_version_ | 1784697839434072064 |
---|---|
author | Chang, Zhaoyu Zhang, Jian Dong, Wanyuan Meng, Xiangqi Wang, Hualei Wei, Dongzhi Ren, Yuhong |
author_facet | Chang, Zhaoyu Zhang, Jian Dong, Wanyuan Meng, Xiangqi Wang, Hualei Wei, Dongzhi Ren, Yuhong |
author_sort | Chang, Zhaoyu |
collection | PubMed |
description | A strategy for synthesizing cadmium sulfide net framework (CdS-NF) nanoparticles was developed in a water-based system under mild reaction conditions. The CdS-NFs have not only the excellent photocatalytic properties of CdS, but also the large surface area and diverse porous structures of a metal–organic framework. An Escherichia coli–CdS-NF hybrid system was constructed using NADH regeneration to promote the conversion of trimethylpyruvate acid to l-tert-leucine. The E. coli–CdS-NF system showed higher NAD(+) recycling efficiency and substrate conversion rate than CdS QDs under visible light illumination. This work demonstrates a novel method for developing a brilliant coenzyme recycling photocatalyst in bio-redox reactions. |
format | Online Article Text |
id | pubmed-9057183 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2020 |
publisher | The Royal Society of Chemistry |
record_format | MEDLINE/PubMed |
spelling | pubmed-90571832022-05-04 Cadmium sulfide net framework nanoparticles for photo-catalyzed cell redox Chang, Zhaoyu Zhang, Jian Dong, Wanyuan Meng, Xiangqi Wang, Hualei Wei, Dongzhi Ren, Yuhong RSC Adv Chemistry A strategy for synthesizing cadmium sulfide net framework (CdS-NF) nanoparticles was developed in a water-based system under mild reaction conditions. The CdS-NFs have not only the excellent photocatalytic properties of CdS, but also the large surface area and diverse porous structures of a metal–organic framework. An Escherichia coli–CdS-NF hybrid system was constructed using NADH regeneration to promote the conversion of trimethylpyruvate acid to l-tert-leucine. The E. coli–CdS-NF system showed higher NAD(+) recycling efficiency and substrate conversion rate than CdS QDs under visible light illumination. This work demonstrates a novel method for developing a brilliant coenzyme recycling photocatalyst in bio-redox reactions. The Royal Society of Chemistry 2020-10-13 /pmc/articles/PMC9057183/ /pubmed/35515163 http://dx.doi.org/10.1039/d0ra08235j Text en This journal is © The Royal Society of Chemistry https://creativecommons.org/licenses/by-nc/3.0/ |
spellingShingle | Chemistry Chang, Zhaoyu Zhang, Jian Dong, Wanyuan Meng, Xiangqi Wang, Hualei Wei, Dongzhi Ren, Yuhong Cadmium sulfide net framework nanoparticles for photo-catalyzed cell redox |
title | Cadmium sulfide net framework nanoparticles for photo-catalyzed cell redox |
title_full | Cadmium sulfide net framework nanoparticles for photo-catalyzed cell redox |
title_fullStr | Cadmium sulfide net framework nanoparticles for photo-catalyzed cell redox |
title_full_unstemmed | Cadmium sulfide net framework nanoparticles for photo-catalyzed cell redox |
title_short | Cadmium sulfide net framework nanoparticles for photo-catalyzed cell redox |
title_sort | cadmium sulfide net framework nanoparticles for photo-catalyzed cell redox |
topic | Chemistry |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9057183/ https://www.ncbi.nlm.nih.gov/pubmed/35515163 http://dx.doi.org/10.1039/d0ra08235j |
work_keys_str_mv | AT changzhaoyu cadmiumsulfidenetframeworknanoparticlesforphotocatalyzedcellredox AT zhangjian cadmiumsulfidenetframeworknanoparticlesforphotocatalyzedcellredox AT dongwanyuan cadmiumsulfidenetframeworknanoparticlesforphotocatalyzedcellredox AT mengxiangqi cadmiumsulfidenetframeworknanoparticlesforphotocatalyzedcellredox AT wanghualei cadmiumsulfidenetframeworknanoparticlesforphotocatalyzedcellredox AT weidongzhi cadmiumsulfidenetframeworknanoparticlesforphotocatalyzedcellredox AT renyuhong cadmiumsulfidenetframeworknanoparticlesforphotocatalyzedcellredox |