Cargando…
A spin promotion effect in catalytic ammonia synthesis
The need for efficient ammonia synthesis is as urgent as ever. Over the past two decades, many attempts to find new catalysts for ammonia synthesis at mild conditions have been reported and, in particular, many new promoters of the catalytic rate have been introduced beyond the traditional K and Cs...
Autores principales: | , , , , , , , |
---|---|
Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2022
|
Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9061734/ https://www.ncbi.nlm.nih.gov/pubmed/35501341 http://dx.doi.org/10.1038/s41467-022-30034-y |
_version_ | 1784698788287348736 |
---|---|
author | Cao, Ang Bukas, Vanessa J. Shadravan, Vahid Wang, Zhenbin Li, Hao Kibsgaard, Jakob Chorkendorff, Ib Nørskov, Jens K. |
author_facet | Cao, Ang Bukas, Vanessa J. Shadravan, Vahid Wang, Zhenbin Li, Hao Kibsgaard, Jakob Chorkendorff, Ib Nørskov, Jens K. |
author_sort | Cao, Ang |
collection | PubMed |
description | The need for efficient ammonia synthesis is as urgent as ever. Over the past two decades, many attempts to find new catalysts for ammonia synthesis at mild conditions have been reported and, in particular, many new promoters of the catalytic rate have been introduced beyond the traditional K and Cs oxides. Herein, we provide an overview of recent experimental results for non-traditional promoters and develop a comprehensive model to explain how they work. The model has two components. First, we establish what is the most likely structure of the active sites in the presence of the different promoters. We then show that there are two effects dictating the catalytic activity. One is an electrostatic interaction between the adsorbed promoter and the N-N dissociation transition state. In addition, we identify a new promoter effect for magnetic catalysts giving rise to an anomalously large lowering of the activation energy opening the possibility of finding new ammonia synthesis catalysts. |
format | Online Article Text |
id | pubmed-9061734 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2022 |
publisher | Nature Publishing Group UK |
record_format | MEDLINE/PubMed |
spelling | pubmed-90617342022-05-04 A spin promotion effect in catalytic ammonia synthesis Cao, Ang Bukas, Vanessa J. Shadravan, Vahid Wang, Zhenbin Li, Hao Kibsgaard, Jakob Chorkendorff, Ib Nørskov, Jens K. Nat Commun Article The need for efficient ammonia synthesis is as urgent as ever. Over the past two decades, many attempts to find new catalysts for ammonia synthesis at mild conditions have been reported and, in particular, many new promoters of the catalytic rate have been introduced beyond the traditional K and Cs oxides. Herein, we provide an overview of recent experimental results for non-traditional promoters and develop a comprehensive model to explain how they work. The model has two components. First, we establish what is the most likely structure of the active sites in the presence of the different promoters. We then show that there are two effects dictating the catalytic activity. One is an electrostatic interaction between the adsorbed promoter and the N-N dissociation transition state. In addition, we identify a new promoter effect for magnetic catalysts giving rise to an anomalously large lowering of the activation energy opening the possibility of finding new ammonia synthesis catalysts. Nature Publishing Group UK 2022-05-02 /pmc/articles/PMC9061734/ /pubmed/35501341 http://dx.doi.org/10.1038/s41467-022-30034-y Text en © The Author(s) 2022 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) . |
spellingShingle | Article Cao, Ang Bukas, Vanessa J. Shadravan, Vahid Wang, Zhenbin Li, Hao Kibsgaard, Jakob Chorkendorff, Ib Nørskov, Jens K. A spin promotion effect in catalytic ammonia synthesis |
title | A spin promotion effect in catalytic ammonia synthesis |
title_full | A spin promotion effect in catalytic ammonia synthesis |
title_fullStr | A spin promotion effect in catalytic ammonia synthesis |
title_full_unstemmed | A spin promotion effect in catalytic ammonia synthesis |
title_short | A spin promotion effect in catalytic ammonia synthesis |
title_sort | spin promotion effect in catalytic ammonia synthesis |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9061734/ https://www.ncbi.nlm.nih.gov/pubmed/35501341 http://dx.doi.org/10.1038/s41467-022-30034-y |
work_keys_str_mv | AT caoang aspinpromotioneffectincatalyticammoniasynthesis AT bukasvanessaj aspinpromotioneffectincatalyticammoniasynthesis AT shadravanvahid aspinpromotioneffectincatalyticammoniasynthesis AT wangzhenbin aspinpromotioneffectincatalyticammoniasynthesis AT lihao aspinpromotioneffectincatalyticammoniasynthesis AT kibsgaardjakob aspinpromotioneffectincatalyticammoniasynthesis AT chorkendorffib aspinpromotioneffectincatalyticammoniasynthesis AT nørskovjensk aspinpromotioneffectincatalyticammoniasynthesis AT caoang spinpromotioneffectincatalyticammoniasynthesis AT bukasvanessaj spinpromotioneffectincatalyticammoniasynthesis AT shadravanvahid spinpromotioneffectincatalyticammoniasynthesis AT wangzhenbin spinpromotioneffectincatalyticammoniasynthesis AT lihao spinpromotioneffectincatalyticammoniasynthesis AT kibsgaardjakob spinpromotioneffectincatalyticammoniasynthesis AT chorkendorffib spinpromotioneffectincatalyticammoniasynthesis AT nørskovjensk spinpromotioneffectincatalyticammoniasynthesis |