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Efficient removal of sulfamerazine (SMR) by ozonation in acetic acid solution after enrichment SMR from water using granular activated carbon

Sulfamerazine (SMR) as a persistent organic pollutant in waste streams is of growing environmental concern. This study explores the extraction SMR from water into an acetic acid (AA) solution using granular activated carbon (GAC), and removal of SMR by ozonation in AA solution. Systematic experiment...

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Detalles Bibliográficos
Autores principales: Yao, Youru, Mi, Na, Zhu, Yongqing, Yin, Li, Zhang, Yong, Li, Shiyin
Formato: Online Artículo Texto
Lenguaje:English
Publicado: The Royal Society of Chemistry 2019
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9062022/
https://www.ncbi.nlm.nih.gov/pubmed/35517672
http://dx.doi.org/10.1039/c8ra10429h
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author Yao, Youru
Mi, Na
Zhu, Yongqing
Yin, Li
Zhang, Yong
Li, Shiyin
author_facet Yao, Youru
Mi, Na
Zhu, Yongqing
Yin, Li
Zhang, Yong
Li, Shiyin
author_sort Yao, Youru
collection PubMed
description Sulfamerazine (SMR) as a persistent organic pollutant in waste streams is of growing environmental concern. This study explores the extraction SMR from water into an acetic acid (AA) solution using granular activated carbon (GAC), and removal of SMR by ozonation in AA solution. Systematic experiments have shown that GAC can be used as an adsorbent to transfer sulfamerazine from water to AA solution. SMR removal efficiency is 99.5% in 10% AA aqueous solution, which is better than in water. The removal rate of SMR in the AA solution decreased as the initial molar ratio of SMR and O(3) increased. The removal rate of SMR decreased with Fe(3+) present in the reactive system. The removal of SMR is dominated by indirect ozonation in water, while the SMR removal is an effect of both direct and indirect ozonation in AA solution. It is a very efficient process for the degradation of SMR in micro polluted water when using combined GAC adsorption–desorption in AA solution and ozonation of the resulting solution.
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spelling pubmed-90620222022-05-04 Efficient removal of sulfamerazine (SMR) by ozonation in acetic acid solution after enrichment SMR from water using granular activated carbon Yao, Youru Mi, Na Zhu, Yongqing Yin, Li Zhang, Yong Li, Shiyin RSC Adv Chemistry Sulfamerazine (SMR) as a persistent organic pollutant in waste streams is of growing environmental concern. This study explores the extraction SMR from water into an acetic acid (AA) solution using granular activated carbon (GAC), and removal of SMR by ozonation in AA solution. Systematic experiments have shown that GAC can be used as an adsorbent to transfer sulfamerazine from water to AA solution. SMR removal efficiency is 99.5% in 10% AA aqueous solution, which is better than in water. The removal rate of SMR in the AA solution decreased as the initial molar ratio of SMR and O(3) increased. The removal rate of SMR decreased with Fe(3+) present in the reactive system. The removal of SMR is dominated by indirect ozonation in water, while the SMR removal is an effect of both direct and indirect ozonation in AA solution. It is a very efficient process for the degradation of SMR in micro polluted water when using combined GAC adsorption–desorption in AA solution and ozonation of the resulting solution. The Royal Society of Chemistry 2019-03-19 /pmc/articles/PMC9062022/ /pubmed/35517672 http://dx.doi.org/10.1039/c8ra10429h Text en This journal is © The Royal Society of Chemistry https://creativecommons.org/licenses/by-nc/3.0/
spellingShingle Chemistry
Yao, Youru
Mi, Na
Zhu, Yongqing
Yin, Li
Zhang, Yong
Li, Shiyin
Efficient removal of sulfamerazine (SMR) by ozonation in acetic acid solution after enrichment SMR from water using granular activated carbon
title Efficient removal of sulfamerazine (SMR) by ozonation in acetic acid solution after enrichment SMR from water using granular activated carbon
title_full Efficient removal of sulfamerazine (SMR) by ozonation in acetic acid solution after enrichment SMR from water using granular activated carbon
title_fullStr Efficient removal of sulfamerazine (SMR) by ozonation in acetic acid solution after enrichment SMR from water using granular activated carbon
title_full_unstemmed Efficient removal of sulfamerazine (SMR) by ozonation in acetic acid solution after enrichment SMR from water using granular activated carbon
title_short Efficient removal of sulfamerazine (SMR) by ozonation in acetic acid solution after enrichment SMR from water using granular activated carbon
title_sort efficient removal of sulfamerazine (smr) by ozonation in acetic acid solution after enrichment smr from water using granular activated carbon
topic Chemistry
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9062022/
https://www.ncbi.nlm.nih.gov/pubmed/35517672
http://dx.doi.org/10.1039/c8ra10429h
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