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Using magneto-electroluminescence as a fingerprint to identify the spin polarization and spin–orbit coupling of magnetic nanoparticle doped polymer light emitting diodes
The spin polarization and spin–orbit coupling (SOC) in polymer light emitting diodes (PLEDs) with the active layer doped with Fe(3)O(4) nanoparticles (NPs) were identified through magneto-electroluminescence (MEL). By comparing the MEL characteristics such as linewidth and magnitude between PLEDs wi...
Autores principales: | , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
The Royal Society of Chemistry
2019
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9064273/ https://www.ncbi.nlm.nih.gov/pubmed/35521377 http://dx.doi.org/10.1039/c9ra01501a |
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author | Jia, Weiyao Ikoma, Tadaaki Chen, Lixiang Zhu, Hongqiang Tang, Xiantong Qu, Fenlan Xiong, Zuhong |
author_facet | Jia, Weiyao Ikoma, Tadaaki Chen, Lixiang Zhu, Hongqiang Tang, Xiantong Qu, Fenlan Xiong, Zuhong |
author_sort | Jia, Weiyao |
collection | PubMed |
description | The spin polarization and spin–orbit coupling (SOC) in polymer light emitting diodes (PLEDs) with the active layer doped with Fe(3)O(4) nanoparticles (NPs) were identified through magneto-electroluminescence (MEL). By comparing the MEL characteristics such as linewidth and magnitude between PLEDs with and without Fe(3)O(4) dopant, we confirmed the existence of spin polarization, but ruled out the existence of SOC. Although the spin polarization is positive to electroluminescence, the brightness–current characteristics suggested that the current efficiency of the doped PLED does not improve. We attributed it to the current leakage caused by the Fe(3)O(4) NPs in the active layer. This work is beneficial for us to further understand the effect of magnetic nanoparticle doping on the dynamic behavior of excitons and polaron pairs in organic semiconductor devices. |
format | Online Article Text |
id | pubmed-9064273 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2019 |
publisher | The Royal Society of Chemistry |
record_format | MEDLINE/PubMed |
spelling | pubmed-90642732022-05-04 Using magneto-electroluminescence as a fingerprint to identify the spin polarization and spin–orbit coupling of magnetic nanoparticle doped polymer light emitting diodes Jia, Weiyao Ikoma, Tadaaki Chen, Lixiang Zhu, Hongqiang Tang, Xiantong Qu, Fenlan Xiong, Zuhong RSC Adv Chemistry The spin polarization and spin–orbit coupling (SOC) in polymer light emitting diodes (PLEDs) with the active layer doped with Fe(3)O(4) nanoparticles (NPs) were identified through magneto-electroluminescence (MEL). By comparing the MEL characteristics such as linewidth and magnitude between PLEDs with and without Fe(3)O(4) dopant, we confirmed the existence of spin polarization, but ruled out the existence of SOC. Although the spin polarization is positive to electroluminescence, the brightness–current characteristics suggested that the current efficiency of the doped PLED does not improve. We attributed it to the current leakage caused by the Fe(3)O(4) NPs in the active layer. This work is beneficial for us to further understand the effect of magnetic nanoparticle doping on the dynamic behavior of excitons and polaron pairs in organic semiconductor devices. The Royal Society of Chemistry 2019-05-21 /pmc/articles/PMC9064273/ /pubmed/35521377 http://dx.doi.org/10.1039/c9ra01501a Text en This journal is © The Royal Society of Chemistry https://creativecommons.org/licenses/by/3.0/ |
spellingShingle | Chemistry Jia, Weiyao Ikoma, Tadaaki Chen, Lixiang Zhu, Hongqiang Tang, Xiantong Qu, Fenlan Xiong, Zuhong Using magneto-electroluminescence as a fingerprint to identify the spin polarization and spin–orbit coupling of magnetic nanoparticle doped polymer light emitting diodes |
title | Using magneto-electroluminescence as a fingerprint to identify the spin polarization and spin–orbit coupling of magnetic nanoparticle doped polymer light emitting diodes |
title_full | Using magneto-electroluminescence as a fingerprint to identify the spin polarization and spin–orbit coupling of magnetic nanoparticle doped polymer light emitting diodes |
title_fullStr | Using magneto-electroluminescence as a fingerprint to identify the spin polarization and spin–orbit coupling of magnetic nanoparticle doped polymer light emitting diodes |
title_full_unstemmed | Using magneto-electroluminescence as a fingerprint to identify the spin polarization and spin–orbit coupling of magnetic nanoparticle doped polymer light emitting diodes |
title_short | Using magneto-electroluminescence as a fingerprint to identify the spin polarization and spin–orbit coupling of magnetic nanoparticle doped polymer light emitting diodes |
title_sort | using magneto-electroluminescence as a fingerprint to identify the spin polarization and spin–orbit coupling of magnetic nanoparticle doped polymer light emitting diodes |
topic | Chemistry |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9064273/ https://www.ncbi.nlm.nih.gov/pubmed/35521377 http://dx.doi.org/10.1039/c9ra01501a |
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