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Construction of flower-like MoS(2)/Fe(3)O(4)/rGO composite with enhanced photo-Fenton like catalyst performance

High-performance and recyclable photocatalysts have attracted considerable amounts of attention for use in wastewater treatment. In this paper, a MoS(2)/Fe(3)O(4)/rGO (0.1 wt%) composite was synthesized by an environmentally-friendly and facile strategy, and showed high potential for recyclability....

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Detalles Bibliográficos
Autores principales: Mu, Dongzhao, Chen, Zhe, Shi, Hongfei, Tan, Naidi
Formato: Online Artículo Texto
Lenguaje:English
Publicado: The Royal Society of Chemistry 2018
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9088837/
https://www.ncbi.nlm.nih.gov/pubmed/35558923
http://dx.doi.org/10.1039/c8ra06537c
Descripción
Sumario:High-performance and recyclable photocatalysts have attracted considerable amounts of attention for use in wastewater treatment. In this paper, a MoS(2)/Fe(3)O(4)/rGO (0.1 wt%) composite was synthesized by an environmentally-friendly and facile strategy, and showed high potential for recyclability. The nanocomposite exhibited high photocatalytic activity in the presence of H(2)O(2) and rGO (reduced graphene oxide) under visible-light irradiation. Notably, when 3 mg of MoS(2)/Fe(3)O(4)/rGO (0.1 wt%) was added to rhodamine B (RhB, 30 mg L(−1)) solution, the degradation rate was almost 100% within 40 min at neutral pH under visible-light irradiation. This rate was four times more rapid than that of MoS(2) and double that of MoS(2)/Fe(3)O(4). The results indicate that rGO plays an important role in photocatalysis by suppressing the recombination of photogenerated electron–hole pairs and enhancing the absorption capability of visible-light and organic dyes. Finally, the photocatalytic and stability mechanisms of MoS(2)/Fe(3)O(4)/rGO (0.1 wt%) are proposed. This work further helps our understanding of the photo-Fenton mechanism. Furthermore, the synthesis of this composite has potential for application in energy storage devices.