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One step synthesis of high-efficiency AgBr–Br–g-C(3)N(4) composite catalysts for photocatalytic H(2)O(2) production via two channel pathway
In this work, a two-component modified AgBr–Br–g-C(3)N(4) composite catalyst with outstanding photocatalytic H(2)O(2) production ability is synthesized. XRD, UV-Vis, N(2) adsorption, TEM, XPS, EPR and PL were used to characterize the obtained catalysts. The as-prepared AgBr–Br–g-C(3)N(4) composite c...
Autores principales: | , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
The Royal Society of Chemistry
2018
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9088936/ https://www.ncbi.nlm.nih.gov/pubmed/35558951 http://dx.doi.org/10.1039/c8ra07749e |
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author | Wang, Yunke Hu, Shaozheng Li, Qiang Gu, Guizhou Zhao, Yanfeng Liang, Hongyu Li, Wei |
author_facet | Wang, Yunke Hu, Shaozheng Li, Qiang Gu, Guizhou Zhao, Yanfeng Liang, Hongyu Li, Wei |
author_sort | Wang, Yunke |
collection | PubMed |
description | In this work, a two-component modified AgBr–Br–g-C(3)N(4) composite catalyst with outstanding photocatalytic H(2)O(2) production ability is synthesized. XRD, UV-Vis, N(2) adsorption, TEM, XPS, EPR and PL were used to characterize the obtained catalysts. The as-prepared AgBr–Br–g-C(3)N(4) composite catalyst shows the highest H(2)O(2) equilibrium concentration of 3.9 mmol L(−1), which is 7.8 and 19.5 times higher than that of GCN and AgBr. A “two channel pathway” is proposed for this reaction system which causes the remarkably promoted H(2)O(2) production ability. In addition, compared with another two-component modified catalyst, Ag–AgBr–g-C(3)N(4), AgBr–Br–g-C(3)N(4) composite catalyst displays the higher photocatalytic H(2)O(2) production ability and stability. |
format | Online Article Text |
id | pubmed-9088936 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2018 |
publisher | The Royal Society of Chemistry |
record_format | MEDLINE/PubMed |
spelling | pubmed-90889362022-05-11 One step synthesis of high-efficiency AgBr–Br–g-C(3)N(4) composite catalysts for photocatalytic H(2)O(2) production via two channel pathway Wang, Yunke Hu, Shaozheng Li, Qiang Gu, Guizhou Zhao, Yanfeng Liang, Hongyu Li, Wei RSC Adv Chemistry In this work, a two-component modified AgBr–Br–g-C(3)N(4) composite catalyst with outstanding photocatalytic H(2)O(2) production ability is synthesized. XRD, UV-Vis, N(2) adsorption, TEM, XPS, EPR and PL were used to characterize the obtained catalysts. The as-prepared AgBr–Br–g-C(3)N(4) composite catalyst shows the highest H(2)O(2) equilibrium concentration of 3.9 mmol L(−1), which is 7.8 and 19.5 times higher than that of GCN and AgBr. A “two channel pathway” is proposed for this reaction system which causes the remarkably promoted H(2)O(2) production ability. In addition, compared with another two-component modified catalyst, Ag–AgBr–g-C(3)N(4), AgBr–Br–g-C(3)N(4) composite catalyst displays the higher photocatalytic H(2)O(2) production ability and stability. The Royal Society of Chemistry 2018-11-01 /pmc/articles/PMC9088936/ /pubmed/35558951 http://dx.doi.org/10.1039/c8ra07749e Text en This journal is © The Royal Society of Chemistry https://creativecommons.org/licenses/by/3.0/ |
spellingShingle | Chemistry Wang, Yunke Hu, Shaozheng Li, Qiang Gu, Guizhou Zhao, Yanfeng Liang, Hongyu Li, Wei One step synthesis of high-efficiency AgBr–Br–g-C(3)N(4) composite catalysts for photocatalytic H(2)O(2) production via two channel pathway |
title | One step synthesis of high-efficiency AgBr–Br–g-C(3)N(4) composite catalysts for photocatalytic H(2)O(2) production via two channel pathway |
title_full | One step synthesis of high-efficiency AgBr–Br–g-C(3)N(4) composite catalysts for photocatalytic H(2)O(2) production via two channel pathway |
title_fullStr | One step synthesis of high-efficiency AgBr–Br–g-C(3)N(4) composite catalysts for photocatalytic H(2)O(2) production via two channel pathway |
title_full_unstemmed | One step synthesis of high-efficiency AgBr–Br–g-C(3)N(4) composite catalysts for photocatalytic H(2)O(2) production via two channel pathway |
title_short | One step synthesis of high-efficiency AgBr–Br–g-C(3)N(4) composite catalysts for photocatalytic H(2)O(2) production via two channel pathway |
title_sort | one step synthesis of high-efficiency agbr–br–g-c(3)n(4) composite catalysts for photocatalytic h(2)o(2) production via two channel pathway |
topic | Chemistry |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9088936/ https://www.ncbi.nlm.nih.gov/pubmed/35558951 http://dx.doi.org/10.1039/c8ra07749e |
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