Concerted Electron-Nuclear Motion in Proton-Coupled Electron Transfer-Driven Grotthuss-Type Proton Translocation

[Image: see text] Photoinduced proton-coupled electron transfer and long-range two-proton transport via a Grotthuss-type mechanism are investigated in a biomimetic construct. The ultrafast, nonequilibrium dynamics are assessed via two-dimensional electronic vibrational spectroscopy, in concert with...

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Detalles Bibliográficos
Autores principales: Arsenault, Eric A., Guerra, Walter D., Shee, James, Reyes Cruz, Edgar A., Yoneda, Yusuke, Wadsworth, Brian L., Odella, Emmanuel, Urrutia, Maria N., Kodis, Gerdenis, Moore, Gary F., Head-Gordon, Martin, Moore, Ana L., Moore, Thomas A., Fleming, Graham R.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2022
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9150097/
https://www.ncbi.nlm.nih.gov/pubmed/35575065
http://dx.doi.org/10.1021/acs.jpclett.2c00585

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