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Towards kilohertz synchrotron coherent diffractive imaging
X-ray coherent diffractive imaging (CDI) techniques have been applied with widespread impact to study nanoscale material properties. New fast framing detectors may reveal dynamics that occur at millisecond timescales. This work demonstrates by simulation that kilohertz synchrotron CDI is possible, b...
Autores principales: | , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
International Union of Crystallography
2022
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9172028/ https://www.ncbi.nlm.nih.gov/pubmed/35719300 http://dx.doi.org/10.1107/S1600576722003466 |
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author | Hinsley, Gerard N. Kewish, Cameron M. van Riessen, Grant A. |
author_facet | Hinsley, Gerard N. Kewish, Cameron M. van Riessen, Grant A. |
author_sort | Hinsley, Gerard N. |
collection | PubMed |
description | X-ray coherent diffractive imaging (CDI) techniques have been applied with widespread impact to study nanoscale material properties. New fast framing detectors may reveal dynamics that occur at millisecond timescales. This work demonstrates by simulation that kilohertz synchrotron CDI is possible, by making use of redundant information from static parts of the image field. Reconstruction ambiguities are strongly suppressed by applying a spatiotemporal constraint, obviating the need for slower methods of introducing diversity such as ptychography. The relationship between image fidelity and time resolution is investigated and shows that dynamics an order of magnitude faster can be reconstructed, compared with conventional CDI. |
format | Online Article Text |
id | pubmed-9172028 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2022 |
publisher | International Union of Crystallography |
record_format | MEDLINE/PubMed |
spelling | pubmed-91720282022-06-17 Towards kilohertz synchrotron coherent diffractive imaging Hinsley, Gerard N. Kewish, Cameron M. van Riessen, Grant A. J Appl Crystallogr Research Papers X-ray coherent diffractive imaging (CDI) techniques have been applied with widespread impact to study nanoscale material properties. New fast framing detectors may reveal dynamics that occur at millisecond timescales. This work demonstrates by simulation that kilohertz synchrotron CDI is possible, by making use of redundant information from static parts of the image field. Reconstruction ambiguities are strongly suppressed by applying a spatiotemporal constraint, obviating the need for slower methods of introducing diversity such as ptychography. The relationship between image fidelity and time resolution is investigated and shows that dynamics an order of magnitude faster can be reconstructed, compared with conventional CDI. International Union of Crystallography 2022-05-08 /pmc/articles/PMC9172028/ /pubmed/35719300 http://dx.doi.org/10.1107/S1600576722003466 Text en © Gerard N. Hinsley et al. 2022 https://creativecommons.org/licenses/by/4.0/This is an open-access article distributed under the terms of the Creative Commons Attribution (CC-BY) Licence, which permits unrestricted use, distribution, and reproduction in any medium, provided the original authors and source are cited. |
spellingShingle | Research Papers Hinsley, Gerard N. Kewish, Cameron M. van Riessen, Grant A. Towards kilohertz synchrotron coherent diffractive imaging |
title | Towards kilohertz synchrotron coherent diffractive imaging |
title_full | Towards kilohertz synchrotron coherent diffractive imaging |
title_fullStr | Towards kilohertz synchrotron coherent diffractive imaging |
title_full_unstemmed | Towards kilohertz synchrotron coherent diffractive imaging |
title_short | Towards kilohertz synchrotron coherent diffractive imaging |
title_sort | towards kilohertz synchrotron coherent diffractive imaging |
topic | Research Papers |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9172028/ https://www.ncbi.nlm.nih.gov/pubmed/35719300 http://dx.doi.org/10.1107/S1600576722003466 |
work_keys_str_mv | AT hinsleygerardn towardskilohertzsynchrotroncoherentdiffractiveimaging AT kewishcameronm towardskilohertzsynchrotroncoherentdiffractiveimaging AT vanriessengranta towardskilohertzsynchrotroncoherentdiffractiveimaging |