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Photoemission of Plasmonic Gold Nanostars in Laser-Controlled Electron Current Devices for Technical and Biomedical Applications

The main goal of this work was to modify the previously developed blade-type planar structure using plasmonic gold nanostars in order to stimulate photofield emission and provide efficient laser control of the electron current. Localization and enhancement of the field at the tips of gold nanostars...

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Autores principales: Yakunin, Alexander N., Avetisyan, Yury A., Akchurin, Garif G., Zarkov, Sergey V., Aban’shin, Nikolay P., Khanadeev, Vitaly A., Tuchin, Valery V.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9185440/
https://www.ncbi.nlm.nih.gov/pubmed/35684746
http://dx.doi.org/10.3390/s22114127
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author Yakunin, Alexander N.
Avetisyan, Yury A.
Akchurin, Garif G.
Zarkov, Sergey V.
Aban’shin, Nikolay P.
Khanadeev, Vitaly A.
Tuchin, Valery V.
author_facet Yakunin, Alexander N.
Avetisyan, Yury A.
Akchurin, Garif G.
Zarkov, Sergey V.
Aban’shin, Nikolay P.
Khanadeev, Vitaly A.
Tuchin, Valery V.
author_sort Yakunin, Alexander N.
collection PubMed
description The main goal of this work was to modify the previously developed blade-type planar structure using plasmonic gold nanostars in order to stimulate photofield emission and provide efficient laser control of the electron current. Localization and enhancement of the field at the tips of gold nanostars provided a significant increase in the tunneling electron current in the experimental sample (both electrical field and photofield emission). Irradiation at a wavelength in the vicinity of the plasmon resonance (red laser) provided a gain in the photoresponse value of up to 5 times compared to irradiation far from the resonance (green laser). The prospects for transition to regimes of structure irradiation by femtosecond laser pulses at the wavelength of surface plasmon resonance, which lead to an increase in the local optical field, are discussed. The kinetics of the energy density of photoinduced hot and thermalized electrons is estimated. The proposed laser-controlled matrix current source is promising for use in X-ray computed tomography systems.
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spelling pubmed-91854402022-06-11 Photoemission of Plasmonic Gold Nanostars in Laser-Controlled Electron Current Devices for Technical and Biomedical Applications Yakunin, Alexander N. Avetisyan, Yury A. Akchurin, Garif G. Zarkov, Sergey V. Aban’shin, Nikolay P. Khanadeev, Vitaly A. Tuchin, Valery V. Sensors (Basel) Article The main goal of this work was to modify the previously developed blade-type planar structure using plasmonic gold nanostars in order to stimulate photofield emission and provide efficient laser control of the electron current. Localization and enhancement of the field at the tips of gold nanostars provided a significant increase in the tunneling electron current in the experimental sample (both electrical field and photofield emission). Irradiation at a wavelength in the vicinity of the plasmon resonance (red laser) provided a gain in the photoresponse value of up to 5 times compared to irradiation far from the resonance (green laser). The prospects for transition to regimes of structure irradiation by femtosecond laser pulses at the wavelength of surface plasmon resonance, which lead to an increase in the local optical field, are discussed. The kinetics of the energy density of photoinduced hot and thermalized electrons is estimated. The proposed laser-controlled matrix current source is promising for use in X-ray computed tomography systems. MDPI 2022-05-29 /pmc/articles/PMC9185440/ /pubmed/35684746 http://dx.doi.org/10.3390/s22114127 Text en © 2022 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Yakunin, Alexander N.
Avetisyan, Yury A.
Akchurin, Garif G.
Zarkov, Sergey V.
Aban’shin, Nikolay P.
Khanadeev, Vitaly A.
Tuchin, Valery V.
Photoemission of Plasmonic Gold Nanostars in Laser-Controlled Electron Current Devices for Technical and Biomedical Applications
title Photoemission of Plasmonic Gold Nanostars in Laser-Controlled Electron Current Devices for Technical and Biomedical Applications
title_full Photoemission of Plasmonic Gold Nanostars in Laser-Controlled Electron Current Devices for Technical and Biomedical Applications
title_fullStr Photoemission of Plasmonic Gold Nanostars in Laser-Controlled Electron Current Devices for Technical and Biomedical Applications
title_full_unstemmed Photoemission of Plasmonic Gold Nanostars in Laser-Controlled Electron Current Devices for Technical and Biomedical Applications
title_short Photoemission of Plasmonic Gold Nanostars in Laser-Controlled Electron Current Devices for Technical and Biomedical Applications
title_sort photoemission of plasmonic gold nanostars in laser-controlled electron current devices for technical and biomedical applications
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9185440/
https://www.ncbi.nlm.nih.gov/pubmed/35684746
http://dx.doi.org/10.3390/s22114127
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