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All‐in‐One Structured Lithium‐Metal Battery

3D batteries possess apparent advantage in electrochemical ion‐transport kinetics than the conventional‐structured batteries. However, due to the special electrode configuration and fabrication complexity, 3D battery design has inherent issue of mechanical stability and only succeeds in microsystems...

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Detalles Bibliográficos
Autores principales: Dong, Lei, Zhang, Chang, Liu, Wei
Formato: Online Artículo Texto
Lenguaje:English
Publicado: John Wiley and Sons Inc. 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9189645/
https://www.ncbi.nlm.nih.gov/pubmed/35416408
http://dx.doi.org/10.1002/advs.202200547
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author Dong, Lei
Zhang, Chang
Liu, Wei
author_facet Dong, Lei
Zhang, Chang
Liu, Wei
author_sort Dong, Lei
collection PubMed
description 3D batteries possess apparent advantage in electrochemical ion‐transport kinetics than the conventional‐structured batteries. However, due to the special electrode configuration and fabrication complexity, 3D battery design has inherent issue of mechanical stability and only succeeds in microsystems, far from ideal. Herein, a high‐stable, all‐in‐one structured 3D lithium‐metal battery is designed which consists of paralleled microcell arrays. Fast ion‐transport kinetics in full cell level can not only address the key issue of lithium dendrites in anode but also improve electrochemical performance of cathode. As a result, the resultant lithium metal anode acquires long‐term stability of 1000‐cycle life at a high current density of 10 mA cm(−2). Also the all‐in‐one structured lithium metal battery has general applicability for various cathodic materials and delivers significantly improved rate and cycling performance, as well as high areal capacity up to 10.4 mAh cm(−2).
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spelling pubmed-91896452022-06-16 All‐in‐One Structured Lithium‐Metal Battery Dong, Lei Zhang, Chang Liu, Wei Adv Sci (Weinh) Research Articles 3D batteries possess apparent advantage in electrochemical ion‐transport kinetics than the conventional‐structured batteries. However, due to the special electrode configuration and fabrication complexity, 3D battery design has inherent issue of mechanical stability and only succeeds in microsystems, far from ideal. Herein, a high‐stable, all‐in‐one structured 3D lithium‐metal battery is designed which consists of paralleled microcell arrays. Fast ion‐transport kinetics in full cell level can not only address the key issue of lithium dendrites in anode but also improve electrochemical performance of cathode. As a result, the resultant lithium metal anode acquires long‐term stability of 1000‐cycle life at a high current density of 10 mA cm(−2). Also the all‐in‐one structured lithium metal battery has general applicability for various cathodic materials and delivers significantly improved rate and cycling performance, as well as high areal capacity up to 10.4 mAh cm(−2). John Wiley and Sons Inc. 2022-04-13 /pmc/articles/PMC9189645/ /pubmed/35416408 http://dx.doi.org/10.1002/advs.202200547 Text en © 2022 The Authors. Advanced Science published by Wiley‐VCH GmbH https://creativecommons.org/licenses/by/4.0/This is an open access article under the terms of the http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) License, which permits use, distribution and reproduction in any medium, provided the original work is properly cited.
spellingShingle Research Articles
Dong, Lei
Zhang, Chang
Liu, Wei
All‐in‐One Structured Lithium‐Metal Battery
title All‐in‐One Structured Lithium‐Metal Battery
title_full All‐in‐One Structured Lithium‐Metal Battery
title_fullStr All‐in‐One Structured Lithium‐Metal Battery
title_full_unstemmed All‐in‐One Structured Lithium‐Metal Battery
title_short All‐in‐One Structured Lithium‐Metal Battery
title_sort all‐in‐one structured lithium‐metal battery
topic Research Articles
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9189645/
https://www.ncbi.nlm.nih.gov/pubmed/35416408
http://dx.doi.org/10.1002/advs.202200547
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