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Molecular Orientation-Induced Second-Harmonic Generation: Deciphering Different Contributions Apart
[Image: see text] We demonstrate and explore an all-optical technique for direct monitoring of the orientation dynamics in gas-phase molecular ensembles. The technique termed “MOISH” utilizes the transiently lifted inversion symmetry of polar gas media and provides a sensitive and spatially localize...
| Autores principales: | , , , |
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| Formato: | Online Artículo Texto |
| Lenguaje: | English |
| Publicado: |
American Chemical Society
2022
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| Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9207934/ https://www.ncbi.nlm.nih.gov/pubmed/35654048 http://dx.doi.org/10.1021/acs.jpca.2c03237 |