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Scanning near-field optical spectroscopy and carrier transport based analysis in mesoscopic regions for two-dimensional semiconductors

The measurements of photoexcited transport in mesoscopic regimes reveal the states and properties of mesoscopic systems. In this study, we focused on direct measurements of electromagnetic energy transports in the mesoscopic regions and constructed a scanning tunnelling microscope-assisted multi-pro...

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Autores principales: Sakurai, Anri, Iwamoto, Kohei, Miwa, Yoshihiko, Hori, Hirokazu, Ishikawa, Akira, Uchiyama, Kazuharu, Kobayashi, Kiyoshi, Kishino, Katsumi, Sakai, Masaru
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9209510/
https://www.ncbi.nlm.nih.gov/pubmed/35725743
http://dx.doi.org/10.1038/s41598-022-13492-8
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author Sakurai, Anri
Iwamoto, Kohei
Miwa, Yoshihiko
Hori, Hirokazu
Ishikawa, Akira
Uchiyama, Kazuharu
Kobayashi, Kiyoshi
Kishino, Katsumi
Sakai, Masaru
author_facet Sakurai, Anri
Iwamoto, Kohei
Miwa, Yoshihiko
Hori, Hirokazu
Ishikawa, Akira
Uchiyama, Kazuharu
Kobayashi, Kiyoshi
Kishino, Katsumi
Sakai, Masaru
author_sort Sakurai, Anri
collection PubMed
description The measurements of photoexcited transport in mesoscopic regimes reveal the states and properties of mesoscopic systems. In this study, we focused on direct measurements of electromagnetic energy transports in the mesoscopic regions and constructed a scanning tunnelling microscope-assisted multi-probe scanning near-field optical microscope spectroscopy system. After producing an emission energy map through a single-probe measurement, two-probe measurement enables us to observe and analyse carrier transport characteristics. It suggests that exciton generation and transport in the mesoscopic region of semiconductors with quantum structure changes, such as the bias of dopant, affect the excited carrier emission recombination process. The measured probability density of the carrier transported with quantum effects can be used for applications in natural intelligence research by combining it with the analysis using tournament structures. Our developed measurement and analysis methods are expected to clarify the details of carrier's behaviour in the mesoscopic region in various materials and lead to applications for novel optoelectronic devices.
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spelling pubmed-92095102022-06-22 Scanning near-field optical spectroscopy and carrier transport based analysis in mesoscopic regions for two-dimensional semiconductors Sakurai, Anri Iwamoto, Kohei Miwa, Yoshihiko Hori, Hirokazu Ishikawa, Akira Uchiyama, Kazuharu Kobayashi, Kiyoshi Kishino, Katsumi Sakai, Masaru Sci Rep Article The measurements of photoexcited transport in mesoscopic regimes reveal the states and properties of mesoscopic systems. In this study, we focused on direct measurements of electromagnetic energy transports in the mesoscopic regions and constructed a scanning tunnelling microscope-assisted multi-probe scanning near-field optical microscope spectroscopy system. After producing an emission energy map through a single-probe measurement, two-probe measurement enables us to observe and analyse carrier transport characteristics. It suggests that exciton generation and transport in the mesoscopic region of semiconductors with quantum structure changes, such as the bias of dopant, affect the excited carrier emission recombination process. The measured probability density of the carrier transported with quantum effects can be used for applications in natural intelligence research by combining it with the analysis using tournament structures. Our developed measurement and analysis methods are expected to clarify the details of carrier's behaviour in the mesoscopic region in various materials and lead to applications for novel optoelectronic devices. Nature Publishing Group UK 2022-06-20 /pmc/articles/PMC9209510/ /pubmed/35725743 http://dx.doi.org/10.1038/s41598-022-13492-8 Text en © The Author(s) 2022 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Sakurai, Anri
Iwamoto, Kohei
Miwa, Yoshihiko
Hori, Hirokazu
Ishikawa, Akira
Uchiyama, Kazuharu
Kobayashi, Kiyoshi
Kishino, Katsumi
Sakai, Masaru
Scanning near-field optical spectroscopy and carrier transport based analysis in mesoscopic regions for two-dimensional semiconductors
title Scanning near-field optical spectroscopy and carrier transport based analysis in mesoscopic regions for two-dimensional semiconductors
title_full Scanning near-field optical spectroscopy and carrier transport based analysis in mesoscopic regions for two-dimensional semiconductors
title_fullStr Scanning near-field optical spectroscopy and carrier transport based analysis in mesoscopic regions for two-dimensional semiconductors
title_full_unstemmed Scanning near-field optical spectroscopy and carrier transport based analysis in mesoscopic regions for two-dimensional semiconductors
title_short Scanning near-field optical spectroscopy and carrier transport based analysis in mesoscopic regions for two-dimensional semiconductors
title_sort scanning near-field optical spectroscopy and carrier transport based analysis in mesoscopic regions for two-dimensional semiconductors
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9209510/
https://www.ncbi.nlm.nih.gov/pubmed/35725743
http://dx.doi.org/10.1038/s41598-022-13492-8
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