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Dealumination of small-pore zeolites through pore-opening migration process with the aid of pore-filler stabilization
Small-pore zeolites are gaining increasing attention owing to their superior catalytic performance. Despite being critical for the catalytic activity and lifetime, postsynthetic tuning of bulk Si/Al ratios of small-pore zeolites has not been achieved with well-preserved crystallinity because of the...
Autores principales: | , , , , , , , , , , , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
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American Association for the Advancement of Science
2022
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9216521/ https://www.ncbi.nlm.nih.gov/pubmed/35731864 http://dx.doi.org/10.1126/sciadv.abo3093 |
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author | Yoshioka, Tatsushi Iyoki, Kenta Hotta, Yuusuke Kamimura, Yoshihiro Yamada, Hiroki Han, Qiao Kato, Takeharu Fisher, Craig A. J. Liu, Zhendong Ohnishi, Ryohji Yanaba, Yutaka Ohara, Koji Sasaki, Yukichi Endo, Akira Takewaki, Takahiko Sano, Tsuneji Okubo, Tatsuya Wakihara, Toru |
author_facet | Yoshioka, Tatsushi Iyoki, Kenta Hotta, Yuusuke Kamimura, Yoshihiro Yamada, Hiroki Han, Qiao Kato, Takeharu Fisher, Craig A. J. Liu, Zhendong Ohnishi, Ryohji Yanaba, Yutaka Ohara, Koji Sasaki, Yukichi Endo, Akira Takewaki, Takahiko Sano, Tsuneji Okubo, Tatsuya Wakihara, Toru |
author_sort | Yoshioka, Tatsushi |
collection | PubMed |
description | Small-pore zeolites are gaining increasing attention owing to their superior catalytic performance. Despite being critical for the catalytic activity and lifetime, postsynthetic tuning of bulk Si/Al ratios of small-pore zeolites has not been achieved with well-preserved crystallinity because of the limited mass transfer of aluminum species through narrow micropores. Here, we demonstrate a postsynthetic approach to tune the composition of small-pore zeolites using a previously unexplored strategy named pore-opening migration process (POMP). Acid treatment assisted by stabilization of the zeolite framework by organic cations in pores is proven to be successful for the removal of Al species from zeolite via POMP. Furthermore, the dealuminated AFX zeolite is treated via defect healing, which yields superior hydrothermal stability against severe steam conditions. Our findings could facilitate industrial applications of small-pore zeolites via aluminum content control and defect healing and could elucidate the structural reconstruction and arrangement processes for inorganic microporous materials. |
format | Online Article Text |
id | pubmed-9216521 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2022 |
publisher | American Association for the Advancement of Science |
record_format | MEDLINE/PubMed |
spelling | pubmed-92165212022-07-07 Dealumination of small-pore zeolites through pore-opening migration process with the aid of pore-filler stabilization Yoshioka, Tatsushi Iyoki, Kenta Hotta, Yuusuke Kamimura, Yoshihiro Yamada, Hiroki Han, Qiao Kato, Takeharu Fisher, Craig A. J. Liu, Zhendong Ohnishi, Ryohji Yanaba, Yutaka Ohara, Koji Sasaki, Yukichi Endo, Akira Takewaki, Takahiko Sano, Tsuneji Okubo, Tatsuya Wakihara, Toru Sci Adv Physical and Materials Sciences Small-pore zeolites are gaining increasing attention owing to their superior catalytic performance. Despite being critical for the catalytic activity and lifetime, postsynthetic tuning of bulk Si/Al ratios of small-pore zeolites has not been achieved with well-preserved crystallinity because of the limited mass transfer of aluminum species through narrow micropores. Here, we demonstrate a postsynthetic approach to tune the composition of small-pore zeolites using a previously unexplored strategy named pore-opening migration process (POMP). Acid treatment assisted by stabilization of the zeolite framework by organic cations in pores is proven to be successful for the removal of Al species from zeolite via POMP. Furthermore, the dealuminated AFX zeolite is treated via defect healing, which yields superior hydrothermal stability against severe steam conditions. Our findings could facilitate industrial applications of small-pore zeolites via aluminum content control and defect healing and could elucidate the structural reconstruction and arrangement processes for inorganic microporous materials. American Association for the Advancement of Science 2022-06-22 /pmc/articles/PMC9216521/ /pubmed/35731864 http://dx.doi.org/10.1126/sciadv.abo3093 Text en Copyright © 2022 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 (CC BY-NC). https://creativecommons.org/licenses/by-nc/4.0/This is an open-access article distributed under the terms of the Creative Commons Attribution-NonCommercial license (https://creativecommons.org/licenses/by-nc/4.0/) , which permits use, distribution, and reproduction in any medium, so long as the resultant use is not for commercial advantage and provided the original work is properly cited. |
spellingShingle | Physical and Materials Sciences Yoshioka, Tatsushi Iyoki, Kenta Hotta, Yuusuke Kamimura, Yoshihiro Yamada, Hiroki Han, Qiao Kato, Takeharu Fisher, Craig A. J. Liu, Zhendong Ohnishi, Ryohji Yanaba, Yutaka Ohara, Koji Sasaki, Yukichi Endo, Akira Takewaki, Takahiko Sano, Tsuneji Okubo, Tatsuya Wakihara, Toru Dealumination of small-pore zeolites through pore-opening migration process with the aid of pore-filler stabilization |
title | Dealumination of small-pore zeolites through pore-opening migration process with the aid of pore-filler stabilization |
title_full | Dealumination of small-pore zeolites through pore-opening migration process with the aid of pore-filler stabilization |
title_fullStr | Dealumination of small-pore zeolites through pore-opening migration process with the aid of pore-filler stabilization |
title_full_unstemmed | Dealumination of small-pore zeolites through pore-opening migration process with the aid of pore-filler stabilization |
title_short | Dealumination of small-pore zeolites through pore-opening migration process with the aid of pore-filler stabilization |
title_sort | dealumination of small-pore zeolites through pore-opening migration process with the aid of pore-filler stabilization |
topic | Physical and Materials Sciences |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9216521/ https://www.ncbi.nlm.nih.gov/pubmed/35731864 http://dx.doi.org/10.1126/sciadv.abo3093 |
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