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Ytterbium-Doped Cesium Lead Chloride Perovskite as an X-ray Scintillator with High Light Yield

[Image: see text] Ytterbium-doped cesium lead halides are quantum cutting materials with exceptionally high photoluminescence quantum yields, making them promising materials as scintillators. In this work, we report ytterbium-doped cesium lead chloride (Yb(3+):CsPbCl(3)) with an X-ray scintillation...

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Detalles Bibliográficos
Autores principales: Dagnall, Katelyn A., Conley, Ashley M., Yoon, Lucy U., Rajeev, Haritha S., Lee, Seung-Hun, Choi, Joshua J.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2022
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9219522/
https://www.ncbi.nlm.nih.gov/pubmed/35755380
http://dx.doi.org/10.1021/acsomega.2c01712
Descripción
Sumario:[Image: see text] Ytterbium-doped cesium lead halides are quantum cutting materials with exceptionally high photoluminescence quantum yields, making them promising materials as scintillators. In this work, we report ytterbium-doped cesium lead chloride (Yb(3+):CsPbCl(3)) with an X-ray scintillation light yield of 102,000 photons/MeV at room temperature, which is brighter than the current state-of-the-art commercial scintillators. The high light yield was achieved based on a novel method of synthesizing Yb(3+):CsPbCl(3) powders using water and low-temperature processing. The combination of high light yield and the simple and inexpensive manufacturing method reported in this work demonstrates the great potential of Yb(3+):CsPbCl(3) for scintillation applications.