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Ytterbium-Doped Cesium Lead Chloride Perovskite as an X-ray Scintillator with High Light Yield

[Image: see text] Ytterbium-doped cesium lead halides are quantum cutting materials with exceptionally high photoluminescence quantum yields, making them promising materials as scintillators. In this work, we report ytterbium-doped cesium lead chloride (Yb(3+):CsPbCl(3)) with an X-ray scintillation...

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Autores principales: Dagnall, Katelyn A., Conley, Ashley M., Yoon, Lucy U., Rajeev, Haritha S., Lee, Seung-Hun, Choi, Joshua J.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2022
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9219522/
https://www.ncbi.nlm.nih.gov/pubmed/35755380
http://dx.doi.org/10.1021/acsomega.2c01712
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author Dagnall, Katelyn A.
Conley, Ashley M.
Yoon, Lucy U.
Rajeev, Haritha S.
Lee, Seung-Hun
Choi, Joshua J.
author_facet Dagnall, Katelyn A.
Conley, Ashley M.
Yoon, Lucy U.
Rajeev, Haritha S.
Lee, Seung-Hun
Choi, Joshua J.
author_sort Dagnall, Katelyn A.
collection PubMed
description [Image: see text] Ytterbium-doped cesium lead halides are quantum cutting materials with exceptionally high photoluminescence quantum yields, making them promising materials as scintillators. In this work, we report ytterbium-doped cesium lead chloride (Yb(3+):CsPbCl(3)) with an X-ray scintillation light yield of 102,000 photons/MeV at room temperature, which is brighter than the current state-of-the-art commercial scintillators. The high light yield was achieved based on a novel method of synthesizing Yb(3+):CsPbCl(3) powders using water and low-temperature processing. The combination of high light yield and the simple and inexpensive manufacturing method reported in this work demonstrates the great potential of Yb(3+):CsPbCl(3) for scintillation applications.
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spelling pubmed-92195222022-06-24 Ytterbium-Doped Cesium Lead Chloride Perovskite as an X-ray Scintillator with High Light Yield Dagnall, Katelyn A. Conley, Ashley M. Yoon, Lucy U. Rajeev, Haritha S. Lee, Seung-Hun Choi, Joshua J. ACS Omega [Image: see text] Ytterbium-doped cesium lead halides are quantum cutting materials with exceptionally high photoluminescence quantum yields, making them promising materials as scintillators. In this work, we report ytterbium-doped cesium lead chloride (Yb(3+):CsPbCl(3)) with an X-ray scintillation light yield of 102,000 photons/MeV at room temperature, which is brighter than the current state-of-the-art commercial scintillators. The high light yield was achieved based on a novel method of synthesizing Yb(3+):CsPbCl(3) powders using water and low-temperature processing. The combination of high light yield and the simple and inexpensive manufacturing method reported in this work demonstrates the great potential of Yb(3+):CsPbCl(3) for scintillation applications. American Chemical Society 2022-06-06 /pmc/articles/PMC9219522/ /pubmed/35755380 http://dx.doi.org/10.1021/acsomega.2c01712 Text en © 2022 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by-nc-nd/4.0/Permits non-commercial access and re-use, provided that author attribution and integrity are maintained; but does not permit creation of adaptations or other derivative works (https://creativecommons.org/licenses/by-nc-nd/4.0/).
spellingShingle Dagnall, Katelyn A.
Conley, Ashley M.
Yoon, Lucy U.
Rajeev, Haritha S.
Lee, Seung-Hun
Choi, Joshua J.
Ytterbium-Doped Cesium Lead Chloride Perovskite as an X-ray Scintillator with High Light Yield
title Ytterbium-Doped Cesium Lead Chloride Perovskite as an X-ray Scintillator with High Light Yield
title_full Ytterbium-Doped Cesium Lead Chloride Perovskite as an X-ray Scintillator with High Light Yield
title_fullStr Ytterbium-Doped Cesium Lead Chloride Perovskite as an X-ray Scintillator with High Light Yield
title_full_unstemmed Ytterbium-Doped Cesium Lead Chloride Perovskite as an X-ray Scintillator with High Light Yield
title_short Ytterbium-Doped Cesium Lead Chloride Perovskite as an X-ray Scintillator with High Light Yield
title_sort ytterbium-doped cesium lead chloride perovskite as an x-ray scintillator with high light yield
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9219522/
https://www.ncbi.nlm.nih.gov/pubmed/35755380
http://dx.doi.org/10.1021/acsomega.2c01712
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