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Impact of interannual and multidecadal trends on methane-climate feedbacks and sensitivity

We estimate the causal contributions of spatiotemporal changes in temperature (T) and precipitation (Pr) to changes in Earth’s atmospheric methane concentration (C(CH4)) and its isotope ratio δ(13)CH(4) over the last four decades. We identify oscillations between positive and negative feedbacks, sho...

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Autores principales: Cheng, Chin-Hsien, Redfern, Simon A. T.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9226131/
https://www.ncbi.nlm.nih.gov/pubmed/35739128
http://dx.doi.org/10.1038/s41467-022-31345-w
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author Cheng, Chin-Hsien
Redfern, Simon A. T.
author_facet Cheng, Chin-Hsien
Redfern, Simon A. T.
author_sort Cheng, Chin-Hsien
collection PubMed
description We estimate the causal contributions of spatiotemporal changes in temperature (T) and precipitation (Pr) to changes in Earth’s atmospheric methane concentration (C(CH4)) and its isotope ratio δ(13)CH(4) over the last four decades. We identify oscillations between positive and negative feedbacks, showing that both contribute to increasing C(CH4). Interannually, increased emissions via positive feedbacks (e.g. wetland emissions and wildfires) with higher land surface air temperature (LSAT) are often followed by increasing C(CH4) due to weakened methane sink via atmospheric (•)OH, via negative feedbacks with lowered sea surface temperatures (SST), especially in the tropics. Over decadal time scales, we find alternating rate-limiting factors for methane oxidation: when C(CH4) is limiting, positive methane-climate feedback via direct oceanic emissions dominates; when (•)OH is limiting, negative feedback is favoured. Incorporating the interannually increasing C(CH4) via negative feedbacks gives historical methane-climate feedback sensitivity ≈ 0.08 W m(−2) °C(−1), much higher than the IPCC AR6 estimate.
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spelling pubmed-92261312022-06-25 Impact of interannual and multidecadal trends on methane-climate feedbacks and sensitivity Cheng, Chin-Hsien Redfern, Simon A. T. Nat Commun Article We estimate the causal contributions of spatiotemporal changes in temperature (T) and precipitation (Pr) to changes in Earth’s atmospheric methane concentration (C(CH4)) and its isotope ratio δ(13)CH(4) over the last four decades. We identify oscillations between positive and negative feedbacks, showing that both contribute to increasing C(CH4). Interannually, increased emissions via positive feedbacks (e.g. wetland emissions and wildfires) with higher land surface air temperature (LSAT) are often followed by increasing C(CH4) due to weakened methane sink via atmospheric (•)OH, via negative feedbacks with lowered sea surface temperatures (SST), especially in the tropics. Over decadal time scales, we find alternating rate-limiting factors for methane oxidation: when C(CH4) is limiting, positive methane-climate feedback via direct oceanic emissions dominates; when (•)OH is limiting, negative feedback is favoured. Incorporating the interannually increasing C(CH4) via negative feedbacks gives historical methane-climate feedback sensitivity ≈ 0.08 W m(−2) °C(−1), much higher than the IPCC AR6 estimate. Nature Publishing Group UK 2022-06-23 /pmc/articles/PMC9226131/ /pubmed/35739128 http://dx.doi.org/10.1038/s41467-022-31345-w Text en © The Author(s) 2022 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Cheng, Chin-Hsien
Redfern, Simon A. T.
Impact of interannual and multidecadal trends on methane-climate feedbacks and sensitivity
title Impact of interannual and multidecadal trends on methane-climate feedbacks and sensitivity
title_full Impact of interannual and multidecadal trends on methane-climate feedbacks and sensitivity
title_fullStr Impact of interannual and multidecadal trends on methane-climate feedbacks and sensitivity
title_full_unstemmed Impact of interannual and multidecadal trends on methane-climate feedbacks and sensitivity
title_short Impact of interannual and multidecadal trends on methane-climate feedbacks and sensitivity
title_sort impact of interannual and multidecadal trends on methane-climate feedbacks and sensitivity
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9226131/
https://www.ncbi.nlm.nih.gov/pubmed/35739128
http://dx.doi.org/10.1038/s41467-022-31345-w
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