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Impact of interannual and multidecadal trends on methane-climate feedbacks and sensitivity
We estimate the causal contributions of spatiotemporal changes in temperature (T) and precipitation (Pr) to changes in Earth’s atmospheric methane concentration (C(CH4)) and its isotope ratio δ(13)CH(4) over the last four decades. We identify oscillations between positive and negative feedbacks, sho...
Autores principales: | , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2022
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9226131/ https://www.ncbi.nlm.nih.gov/pubmed/35739128 http://dx.doi.org/10.1038/s41467-022-31345-w |
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author | Cheng, Chin-Hsien Redfern, Simon A. T. |
author_facet | Cheng, Chin-Hsien Redfern, Simon A. T. |
author_sort | Cheng, Chin-Hsien |
collection | PubMed |
description | We estimate the causal contributions of spatiotemporal changes in temperature (T) and precipitation (Pr) to changes in Earth’s atmospheric methane concentration (C(CH4)) and its isotope ratio δ(13)CH(4) over the last four decades. We identify oscillations between positive and negative feedbacks, showing that both contribute to increasing C(CH4). Interannually, increased emissions via positive feedbacks (e.g. wetland emissions and wildfires) with higher land surface air temperature (LSAT) are often followed by increasing C(CH4) due to weakened methane sink via atmospheric (•)OH, via negative feedbacks with lowered sea surface temperatures (SST), especially in the tropics. Over decadal time scales, we find alternating rate-limiting factors for methane oxidation: when C(CH4) is limiting, positive methane-climate feedback via direct oceanic emissions dominates; when (•)OH is limiting, negative feedback is favoured. Incorporating the interannually increasing C(CH4) via negative feedbacks gives historical methane-climate feedback sensitivity ≈ 0.08 W m(−2) °C(−1), much higher than the IPCC AR6 estimate. |
format | Online Article Text |
id | pubmed-9226131 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2022 |
publisher | Nature Publishing Group UK |
record_format | MEDLINE/PubMed |
spelling | pubmed-92261312022-06-25 Impact of interannual and multidecadal trends on methane-climate feedbacks and sensitivity Cheng, Chin-Hsien Redfern, Simon A. T. Nat Commun Article We estimate the causal contributions of spatiotemporal changes in temperature (T) and precipitation (Pr) to changes in Earth’s atmospheric methane concentration (C(CH4)) and its isotope ratio δ(13)CH(4) over the last four decades. We identify oscillations between positive and negative feedbacks, showing that both contribute to increasing C(CH4). Interannually, increased emissions via positive feedbacks (e.g. wetland emissions and wildfires) with higher land surface air temperature (LSAT) are often followed by increasing C(CH4) due to weakened methane sink via atmospheric (•)OH, via negative feedbacks with lowered sea surface temperatures (SST), especially in the tropics. Over decadal time scales, we find alternating rate-limiting factors for methane oxidation: when C(CH4) is limiting, positive methane-climate feedback via direct oceanic emissions dominates; when (•)OH is limiting, negative feedback is favoured. Incorporating the interannually increasing C(CH4) via negative feedbacks gives historical methane-climate feedback sensitivity ≈ 0.08 W m(−2) °C(−1), much higher than the IPCC AR6 estimate. Nature Publishing Group UK 2022-06-23 /pmc/articles/PMC9226131/ /pubmed/35739128 http://dx.doi.org/10.1038/s41467-022-31345-w Text en © The Author(s) 2022 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) . |
spellingShingle | Article Cheng, Chin-Hsien Redfern, Simon A. T. Impact of interannual and multidecadal trends on methane-climate feedbacks and sensitivity |
title | Impact of interannual and multidecadal trends on methane-climate feedbacks and sensitivity |
title_full | Impact of interannual and multidecadal trends on methane-climate feedbacks and sensitivity |
title_fullStr | Impact of interannual and multidecadal trends on methane-climate feedbacks and sensitivity |
title_full_unstemmed | Impact of interannual and multidecadal trends on methane-climate feedbacks and sensitivity |
title_short | Impact of interannual and multidecadal trends on methane-climate feedbacks and sensitivity |
title_sort | impact of interannual and multidecadal trends on methane-climate feedbacks and sensitivity |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9226131/ https://www.ncbi.nlm.nih.gov/pubmed/35739128 http://dx.doi.org/10.1038/s41467-022-31345-w |
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