Cargando…
High Quality TaS(2) Nanosheet SPR Biosensors Improved Sensitivity and the Experimental Demonstration for the Detection of Hg(2+)
TaS(2) as transition metal dichalcogenide (TMD) two-dimensional (2D) material has sufficient unstructured bonds and large inter-layer spacing, which highly supports transporting and absorbing mercury ions. The structural characterizations and simulation data show that an SPR sensor with high sensiti...
Autores principales: | , , |
---|---|
Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
MDPI
2022
|
Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9228406/ https://www.ncbi.nlm.nih.gov/pubmed/35745416 http://dx.doi.org/10.3390/nano12122075 |
_version_ | 1784734460747448320 |
---|---|
author | Jia, Yue Liao, Yunlong Cai, Houzhi |
author_facet | Jia, Yue Liao, Yunlong Cai, Houzhi |
author_sort | Jia, Yue |
collection | PubMed |
description | TaS(2) as transition metal dichalcogenide (TMD) two-dimensional (2D) material has sufficient unstructured bonds and large inter-layer spacing, which highly supports transporting and absorbing mercury ions. The structural characterizations and simulation data show that an SPR sensor with high sensitivity can be obtained with a TaS(2) material-modified sensitive layer. In this paper, the role of TaS(2) nanoparticles in an SPR sensor was explored by simulation and experiment, and the TaS(2) layer in an SPR sensor was characterized by SEM, elemental mapping, XPS, and other methods. The application range of structured TaS(2) nanoparticles is explored, these TaS(2) based sensors were applied to detect Hg(2+) ions at a detection limit approaching 1 pM, and an innovative idea for designing highly sensitive detection techniques is provided. |
format | Online Article Text |
id | pubmed-9228406 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2022 |
publisher | MDPI |
record_format | MEDLINE/PubMed |
spelling | pubmed-92284062022-06-25 High Quality TaS(2) Nanosheet SPR Biosensors Improved Sensitivity and the Experimental Demonstration for the Detection of Hg(2+) Jia, Yue Liao, Yunlong Cai, Houzhi Nanomaterials (Basel) Article TaS(2) as transition metal dichalcogenide (TMD) two-dimensional (2D) material has sufficient unstructured bonds and large inter-layer spacing, which highly supports transporting and absorbing mercury ions. The structural characterizations and simulation data show that an SPR sensor with high sensitivity can be obtained with a TaS(2) material-modified sensitive layer. In this paper, the role of TaS(2) nanoparticles in an SPR sensor was explored by simulation and experiment, and the TaS(2) layer in an SPR sensor was characterized by SEM, elemental mapping, XPS, and other methods. The application range of structured TaS(2) nanoparticles is explored, these TaS(2) based sensors were applied to detect Hg(2+) ions at a detection limit approaching 1 pM, and an innovative idea for designing highly sensitive detection techniques is provided. MDPI 2022-06-16 /pmc/articles/PMC9228406/ /pubmed/35745416 http://dx.doi.org/10.3390/nano12122075 Text en © 2022 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/). |
spellingShingle | Article Jia, Yue Liao, Yunlong Cai, Houzhi High Quality TaS(2) Nanosheet SPR Biosensors Improved Sensitivity and the Experimental Demonstration for the Detection of Hg(2+) |
title | High Quality TaS(2) Nanosheet SPR Biosensors Improved Sensitivity and the Experimental Demonstration for the Detection of Hg(2+) |
title_full | High Quality TaS(2) Nanosheet SPR Biosensors Improved Sensitivity and the Experimental Demonstration for the Detection of Hg(2+) |
title_fullStr | High Quality TaS(2) Nanosheet SPR Biosensors Improved Sensitivity and the Experimental Demonstration for the Detection of Hg(2+) |
title_full_unstemmed | High Quality TaS(2) Nanosheet SPR Biosensors Improved Sensitivity and the Experimental Demonstration for the Detection of Hg(2+) |
title_short | High Quality TaS(2) Nanosheet SPR Biosensors Improved Sensitivity and the Experimental Demonstration for the Detection of Hg(2+) |
title_sort | high quality tas(2) nanosheet spr biosensors improved sensitivity and the experimental demonstration for the detection of hg(2+) |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9228406/ https://www.ncbi.nlm.nih.gov/pubmed/35745416 http://dx.doi.org/10.3390/nano12122075 |
work_keys_str_mv | AT jiayue highqualitytas2nanosheetsprbiosensorsimprovedsensitivityandtheexperimentaldemonstrationforthedetectionofhg2 AT liaoyunlong highqualitytas2nanosheetsprbiosensorsimprovedsensitivityandtheexperimentaldemonstrationforthedetectionofhg2 AT caihouzhi highqualitytas2nanosheetsprbiosensorsimprovedsensitivityandtheexperimentaldemonstrationforthedetectionofhg2 |