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Ultrahigh transverse thermoelectric power factor in flexible Weyl semimetal WTe(2)

Topological semimetals are well known for their interesting physical properties, while their mechanical properties have rarely received attention. With the increasing demand for flexible electronics, we explore the great potential of the van der Waals bonded Weyl semimetal WTe(2) for flexible thermo...

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Detalles Bibliográficos
Autores principales: Pan, Yu, He, Bin, Helm, Toni, Chen, Dong, Schnelle, Walter, Felser, Claudia
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9262886/
https://www.ncbi.nlm.nih.gov/pubmed/35798731
http://dx.doi.org/10.1038/s41467-022-31372-7
Descripción
Sumario:Topological semimetals are well known for their interesting physical properties, while their mechanical properties have rarely received attention. With the increasing demand for flexible electronics, we explore the great potential of the van der Waals bonded Weyl semimetal WTe(2) for flexible thermoelectric applications. We find that WTe(2) single crystals have an ultrahigh Nernst power factor of ~3 Wm(−1)K(−2), which outperforms the conventional Seebeck power factors of the state-of-the-art thermoelectric semiconductors by 2–3 orders of magnitude. A unique band structure that hosts compensated electrons and holes with extremely high mobilities is the primary mechanism for this huge Nernst power factor. Moreover, a large Ettingshausen signal of ~5 × 10(−5) KA(−1)m is observed at 23.1 K and 9 T. In this work, the combination of the exceptional Nernst–Ettingshausen performance and excellent mechanical transformative ability of WTe(2) would be instructive for flexible micro-/nano-thermoelectric devices.