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Full experimental determination of tunneling time with attosecond-scale streaking method
Tunneling is one of the most fundamental and ubiquitous processes in the quantum world. The question of how long a particle takes to tunnel through a potential barrier has sparked a long-standing debate since the early days of quantum mechanics. Here, we propose and demonstrate a novel scheme to acc...
Autores principales: | , , , , , , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2022
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9262890/ https://www.ncbi.nlm.nih.gov/pubmed/35798716 http://dx.doi.org/10.1038/s41377-022-00911-8 |
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author | Yu, Miao Liu, Kun Li, Min Yan, Jiaqing Cao, Chuanpeng Tan, Jia Liang, Jintai Guo, Keyu Cao, Wei Lan, Pengfei Zhang, Qingbin Zhou, Yueming Lu, Peixiang |
author_facet | Yu, Miao Liu, Kun Li, Min Yan, Jiaqing Cao, Chuanpeng Tan, Jia Liang, Jintai Guo, Keyu Cao, Wei Lan, Pengfei Zhang, Qingbin Zhou, Yueming Lu, Peixiang |
author_sort | Yu, Miao |
collection | PubMed |
description | Tunneling is one of the most fundamental and ubiquitous processes in the quantum world. The question of how long a particle takes to tunnel through a potential barrier has sparked a long-standing debate since the early days of quantum mechanics. Here, we propose and demonstrate a novel scheme to accurately determine the tunneling time of an electron. In this scheme, a weak laser field is used to streak the tunneling current produced by a strong elliptically polarized laser field in an attoclock configuration, allowing us to retrieve the tunneling ionization time relative to the field maximum with a precision of a few attoseconds. This overcomes the difficulties in previous attoclock measurements wherein the Coulomb effect on the photoelectron momentum distribution has to be removed with theoretical models and it requires accurate information of the driving laser fields. We demonstrate that the tunneling time of an electron from an atom is close to zero within our experimental accuracy. Our study represents a straightforward approach toward attosecond time-resolved imaging of electron motion in atoms and molecules. |
format | Online Article Text |
id | pubmed-9262890 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2022 |
publisher | Nature Publishing Group UK |
record_format | MEDLINE/PubMed |
spelling | pubmed-92628902022-07-09 Full experimental determination of tunneling time with attosecond-scale streaking method Yu, Miao Liu, Kun Li, Min Yan, Jiaqing Cao, Chuanpeng Tan, Jia Liang, Jintai Guo, Keyu Cao, Wei Lan, Pengfei Zhang, Qingbin Zhou, Yueming Lu, Peixiang Light Sci Appl Article Tunneling is one of the most fundamental and ubiquitous processes in the quantum world. The question of how long a particle takes to tunnel through a potential barrier has sparked a long-standing debate since the early days of quantum mechanics. Here, we propose and demonstrate a novel scheme to accurately determine the tunneling time of an electron. In this scheme, a weak laser field is used to streak the tunneling current produced by a strong elliptically polarized laser field in an attoclock configuration, allowing us to retrieve the tunneling ionization time relative to the field maximum with a precision of a few attoseconds. This overcomes the difficulties in previous attoclock measurements wherein the Coulomb effect on the photoelectron momentum distribution has to be removed with theoretical models and it requires accurate information of the driving laser fields. We demonstrate that the tunneling time of an electron from an atom is close to zero within our experimental accuracy. Our study represents a straightforward approach toward attosecond time-resolved imaging of electron motion in atoms and molecules. Nature Publishing Group UK 2022-07-07 /pmc/articles/PMC9262890/ /pubmed/35798716 http://dx.doi.org/10.1038/s41377-022-00911-8 Text en © The Author(s) 2022 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) . |
spellingShingle | Article Yu, Miao Liu, Kun Li, Min Yan, Jiaqing Cao, Chuanpeng Tan, Jia Liang, Jintai Guo, Keyu Cao, Wei Lan, Pengfei Zhang, Qingbin Zhou, Yueming Lu, Peixiang Full experimental determination of tunneling time with attosecond-scale streaking method |
title | Full experimental determination of tunneling time with attosecond-scale streaking method |
title_full | Full experimental determination of tunneling time with attosecond-scale streaking method |
title_fullStr | Full experimental determination of tunneling time with attosecond-scale streaking method |
title_full_unstemmed | Full experimental determination of tunneling time with attosecond-scale streaking method |
title_short | Full experimental determination of tunneling time with attosecond-scale streaking method |
title_sort | full experimental determination of tunneling time with attosecond-scale streaking method |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9262890/ https://www.ncbi.nlm.nih.gov/pubmed/35798716 http://dx.doi.org/10.1038/s41377-022-00911-8 |
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