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Full experimental determination of tunneling time with attosecond-scale streaking method

Tunneling is one of the most fundamental and ubiquitous processes in the quantum world. The question of how long a particle takes to tunnel through a potential barrier has sparked a long-standing debate since the early days of quantum mechanics. Here, we propose and demonstrate a novel scheme to acc...

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Autores principales: Yu, Miao, Liu, Kun, Li, Min, Yan, Jiaqing, Cao, Chuanpeng, Tan, Jia, Liang, Jintai, Guo, Keyu, Cao, Wei, Lan, Pengfei, Zhang, Qingbin, Zhou, Yueming, Lu, Peixiang
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9262890/
https://www.ncbi.nlm.nih.gov/pubmed/35798716
http://dx.doi.org/10.1038/s41377-022-00911-8
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author Yu, Miao
Liu, Kun
Li, Min
Yan, Jiaqing
Cao, Chuanpeng
Tan, Jia
Liang, Jintai
Guo, Keyu
Cao, Wei
Lan, Pengfei
Zhang, Qingbin
Zhou, Yueming
Lu, Peixiang
author_facet Yu, Miao
Liu, Kun
Li, Min
Yan, Jiaqing
Cao, Chuanpeng
Tan, Jia
Liang, Jintai
Guo, Keyu
Cao, Wei
Lan, Pengfei
Zhang, Qingbin
Zhou, Yueming
Lu, Peixiang
author_sort Yu, Miao
collection PubMed
description Tunneling is one of the most fundamental and ubiquitous processes in the quantum world. The question of how long a particle takes to tunnel through a potential barrier has sparked a long-standing debate since the early days of quantum mechanics. Here, we propose and demonstrate a novel scheme to accurately determine the tunneling time of an electron. In this scheme, a weak laser field is used to streak the tunneling current produced by a strong elliptically polarized laser field in an attoclock configuration, allowing us to retrieve the tunneling ionization time relative to the field maximum with a precision of a few attoseconds. This overcomes the difficulties in previous attoclock measurements wherein the Coulomb effect on the photoelectron momentum distribution has to be removed with theoretical models and it requires accurate information of the driving laser fields. We demonstrate that the tunneling time of an electron from an atom is close to zero within our experimental accuracy. Our study represents a straightforward approach toward attosecond time-resolved imaging of electron motion in atoms and molecules.
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spelling pubmed-92628902022-07-09 Full experimental determination of tunneling time with attosecond-scale streaking method Yu, Miao Liu, Kun Li, Min Yan, Jiaqing Cao, Chuanpeng Tan, Jia Liang, Jintai Guo, Keyu Cao, Wei Lan, Pengfei Zhang, Qingbin Zhou, Yueming Lu, Peixiang Light Sci Appl Article Tunneling is one of the most fundamental and ubiquitous processes in the quantum world. The question of how long a particle takes to tunnel through a potential barrier has sparked a long-standing debate since the early days of quantum mechanics. Here, we propose and demonstrate a novel scheme to accurately determine the tunneling time of an electron. In this scheme, a weak laser field is used to streak the tunneling current produced by a strong elliptically polarized laser field in an attoclock configuration, allowing us to retrieve the tunneling ionization time relative to the field maximum with a precision of a few attoseconds. This overcomes the difficulties in previous attoclock measurements wherein the Coulomb effect on the photoelectron momentum distribution has to be removed with theoretical models and it requires accurate information of the driving laser fields. We demonstrate that the tunneling time of an electron from an atom is close to zero within our experimental accuracy. Our study represents a straightforward approach toward attosecond time-resolved imaging of electron motion in atoms and molecules. Nature Publishing Group UK 2022-07-07 /pmc/articles/PMC9262890/ /pubmed/35798716 http://dx.doi.org/10.1038/s41377-022-00911-8 Text en © The Author(s) 2022 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Yu, Miao
Liu, Kun
Li, Min
Yan, Jiaqing
Cao, Chuanpeng
Tan, Jia
Liang, Jintai
Guo, Keyu
Cao, Wei
Lan, Pengfei
Zhang, Qingbin
Zhou, Yueming
Lu, Peixiang
Full experimental determination of tunneling time with attosecond-scale streaking method
title Full experimental determination of tunneling time with attosecond-scale streaking method
title_full Full experimental determination of tunneling time with attosecond-scale streaking method
title_fullStr Full experimental determination of tunneling time with attosecond-scale streaking method
title_full_unstemmed Full experimental determination of tunneling time with attosecond-scale streaking method
title_short Full experimental determination of tunneling time with attosecond-scale streaking method
title_sort full experimental determination of tunneling time with attosecond-scale streaking method
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9262890/
https://www.ncbi.nlm.nih.gov/pubmed/35798716
http://dx.doi.org/10.1038/s41377-022-00911-8
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