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Far-Field and Non-Intrusive Optical Mapping of Nanoscale Structures

Far-field high-density optics storage and readout involve the interaction of a sub-100 nm beam profile laser to store and retrieve data with nanostructure media. Hence, understanding the light–matter interaction responding in the far-field in such a small scale is essential for effective optical inf...

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Detalles Bibliográficos
Autores principales: Guan, Guorong, Zhang, Aiqin, Xie, Xiangsheng, Meng, Yan, Zhang, Weihua, Zhou, Jianying, Liang, Haowen
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9268055/
https://www.ncbi.nlm.nih.gov/pubmed/35808109
http://dx.doi.org/10.3390/nano12132274
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author Guan, Guorong
Zhang, Aiqin
Xie, Xiangsheng
Meng, Yan
Zhang, Weihua
Zhou, Jianying
Liang, Haowen
author_facet Guan, Guorong
Zhang, Aiqin
Xie, Xiangsheng
Meng, Yan
Zhang, Weihua
Zhou, Jianying
Liang, Haowen
author_sort Guan, Guorong
collection PubMed
description Far-field high-density optics storage and readout involve the interaction of a sub-100 nm beam profile laser to store and retrieve data with nanostructure media. Hence, understanding the light–matter interaction responding in the far-field in such a small scale is essential for effective optical information processing. We present a theoretical analysis and an experimental study for far-field and non-intrusive optical mapping of nanostructures. By a comprehensive analytical derivation for interaction between the modulated light and the target in a confocal laser scanning microscopy (CLSM) configuration, it is found that the CLSM probes the local density of states (LDOSs) in the far field rather than the sample geometric morphology. With a radially polarized (RP) light for illumination, the far-field mapping of LDOS at the optical resolution down to 74 nm is obtained. In addition, it is experimentally verified that the target morphology is mapped only when the far-field mapping of LDOS coincides with the geometric morphology, while light may be blocked from entering the nanostructures medium with weak or missing LDOS, hence invalidating high-density optical information storage and retrieval. In this scenario, nanosphere gaps as small as 33 nm are clearly observed. We further discuss the characterization for far-field and non-intrusive interaction with nanostructures of different geometric morphology and compare them with those obtainable with the projection of near-field LDOS and scanning electronic microscopic results.
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spelling pubmed-92680552022-07-09 Far-Field and Non-Intrusive Optical Mapping of Nanoscale Structures Guan, Guorong Zhang, Aiqin Xie, Xiangsheng Meng, Yan Zhang, Weihua Zhou, Jianying Liang, Haowen Nanomaterials (Basel) Article Far-field high-density optics storage and readout involve the interaction of a sub-100 nm beam profile laser to store and retrieve data with nanostructure media. Hence, understanding the light–matter interaction responding in the far-field in such a small scale is essential for effective optical information processing. We present a theoretical analysis and an experimental study for far-field and non-intrusive optical mapping of nanostructures. By a comprehensive analytical derivation for interaction between the modulated light and the target in a confocal laser scanning microscopy (CLSM) configuration, it is found that the CLSM probes the local density of states (LDOSs) in the far field rather than the sample geometric morphology. With a radially polarized (RP) light for illumination, the far-field mapping of LDOS at the optical resolution down to 74 nm is obtained. In addition, it is experimentally verified that the target morphology is mapped only when the far-field mapping of LDOS coincides with the geometric morphology, while light may be blocked from entering the nanostructures medium with weak or missing LDOS, hence invalidating high-density optical information storage and retrieval. In this scenario, nanosphere gaps as small as 33 nm are clearly observed. We further discuss the characterization for far-field and non-intrusive interaction with nanostructures of different geometric morphology and compare them with those obtainable with the projection of near-field LDOS and scanning electronic microscopic results. MDPI 2022-07-01 /pmc/articles/PMC9268055/ /pubmed/35808109 http://dx.doi.org/10.3390/nano12132274 Text en © 2022 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Guan, Guorong
Zhang, Aiqin
Xie, Xiangsheng
Meng, Yan
Zhang, Weihua
Zhou, Jianying
Liang, Haowen
Far-Field and Non-Intrusive Optical Mapping of Nanoscale Structures
title Far-Field and Non-Intrusive Optical Mapping of Nanoscale Structures
title_full Far-Field and Non-Intrusive Optical Mapping of Nanoscale Structures
title_fullStr Far-Field and Non-Intrusive Optical Mapping of Nanoscale Structures
title_full_unstemmed Far-Field and Non-Intrusive Optical Mapping of Nanoscale Structures
title_short Far-Field and Non-Intrusive Optical Mapping of Nanoscale Structures
title_sort far-field and non-intrusive optical mapping of nanoscale structures
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9268055/
https://www.ncbi.nlm.nih.gov/pubmed/35808109
http://dx.doi.org/10.3390/nano12132274
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