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Molecular doped, color-tunable, high-mobility, emissive, organic semiconductors for light-emitting transistors
Developing high-mobility emissive organic semiconductors with tunable colors is crucial for organic light-emitting transistors (OLETs), a pivotal component of integrated optoelectronic devices, but remains a great challenge. Here, we demonstrate a series of color-tunable, high-mobility, emissive, or...
Autores principales: | , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Association for the Advancement of Science
2022
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9269892/ https://www.ncbi.nlm.nih.gov/pubmed/35857474 http://dx.doi.org/10.1126/sciadv.abp8775 |
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author | Qin, Zhengsheng Gao, Can Gao, Haikuo Wang, Tianyu Dong, Huanli Hu, Wenping |
author_facet | Qin, Zhengsheng Gao, Can Gao, Haikuo Wang, Tianyu Dong, Huanli Hu, Wenping |
author_sort | Qin, Zhengsheng |
collection | PubMed |
description | Developing high-mobility emissive organic semiconductors with tunable colors is crucial for organic light-emitting transistors (OLETs), a pivotal component of integrated optoelectronic devices, but remains a great challenge. Here, we demonstrate a series of color-tunable, high-mobility, emissive, organic semiconductors via molecular doping with a high-mobility organic semiconductor, 2,6-diphenylanthracene, as the host. The well-matched molecular structures and sizes with efficient energy transfer between the host and guest enable the intrinsically high charge transport with tunable colors. High mobility with the highest value >2 cm(2) V(−1) s(−1) and strong emission with photoluminescence quantum yield >15.8% are obtained for these molecular-doped organic semiconductors. Last, a large color gamut for constructed OLETs is up to 59% National Television System Committee standard, meanwhile with an extremely high current density approaching 326.4 kA cm(−2), showing great potential for full-color smart display, organic electrically pumped lasers and other related logic circuitries. |
format | Online Article Text |
id | pubmed-9269892 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2022 |
publisher | American Association for the Advancement of Science |
record_format | MEDLINE/PubMed |
spelling | pubmed-92698922022-07-20 Molecular doped, color-tunable, high-mobility, emissive, organic semiconductors for light-emitting transistors Qin, Zhengsheng Gao, Can Gao, Haikuo Wang, Tianyu Dong, Huanli Hu, Wenping Sci Adv Physical and Materials Sciences Developing high-mobility emissive organic semiconductors with tunable colors is crucial for organic light-emitting transistors (OLETs), a pivotal component of integrated optoelectronic devices, but remains a great challenge. Here, we demonstrate a series of color-tunable, high-mobility, emissive, organic semiconductors via molecular doping with a high-mobility organic semiconductor, 2,6-diphenylanthracene, as the host. The well-matched molecular structures and sizes with efficient energy transfer between the host and guest enable the intrinsically high charge transport with tunable colors. High mobility with the highest value >2 cm(2) V(−1) s(−1) and strong emission with photoluminescence quantum yield >15.8% are obtained for these molecular-doped organic semiconductors. Last, a large color gamut for constructed OLETs is up to 59% National Television System Committee standard, meanwhile with an extremely high current density approaching 326.4 kA cm(−2), showing great potential for full-color smart display, organic electrically pumped lasers and other related logic circuitries. American Association for the Advancement of Science 2022-07-08 /pmc/articles/PMC9269892/ /pubmed/35857474 http://dx.doi.org/10.1126/sciadv.abp8775 Text en Copyright © 2022 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 (CC BY-NC). https://creativecommons.org/licenses/by-nc/4.0/This is an open-access article distributed under the terms of the Creative Commons Attribution-NonCommercial license (https://creativecommons.org/licenses/by-nc/4.0/) , which permits use, distribution, and reproduction in any medium, so long as the resultant use is not for commercial advantage and provided the original work is properly cited. |
spellingShingle | Physical and Materials Sciences Qin, Zhengsheng Gao, Can Gao, Haikuo Wang, Tianyu Dong, Huanli Hu, Wenping Molecular doped, color-tunable, high-mobility, emissive, organic semiconductors for light-emitting transistors |
title | Molecular doped, color-tunable, high-mobility, emissive, organic semiconductors for light-emitting transistors |
title_full | Molecular doped, color-tunable, high-mobility, emissive, organic semiconductors for light-emitting transistors |
title_fullStr | Molecular doped, color-tunable, high-mobility, emissive, organic semiconductors for light-emitting transistors |
title_full_unstemmed | Molecular doped, color-tunable, high-mobility, emissive, organic semiconductors for light-emitting transistors |
title_short | Molecular doped, color-tunable, high-mobility, emissive, organic semiconductors for light-emitting transistors |
title_sort | molecular doped, color-tunable, high-mobility, emissive, organic semiconductors for light-emitting transistors |
topic | Physical and Materials Sciences |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9269892/ https://www.ncbi.nlm.nih.gov/pubmed/35857474 http://dx.doi.org/10.1126/sciadv.abp8775 |
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