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Improved Parameterization for the Size Distribution of Emitted Dust Aerosols Reduces Model Underestimation of Super Coarse Dust

Aircraft measurement campaigns have revealed that super coarse dust (diameter >10 μm) surprisingly accounts for approximately a quarter of aerosols by mass in the atmosphere. However, most global aerosol models either underestimate or do not include super coarse dust abundance. To address this pr...

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Autores principales: Meng, Jun, Huang, Yue, Leung, Danny M., Li, Longlei, Adebiyi, Adeyemi A., Ryder, Claire L., Mahowald, Natalie M., Kok, Jasper F.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: John Wiley and Sons Inc. 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9286626/
https://www.ncbi.nlm.nih.gov/pubmed/35866061
http://dx.doi.org/10.1029/2021GL097287
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author Meng, Jun
Huang, Yue
Leung, Danny M.
Li, Longlei
Adebiyi, Adeyemi A.
Ryder, Claire L.
Mahowald, Natalie M.
Kok, Jasper F.
author_facet Meng, Jun
Huang, Yue
Leung, Danny M.
Li, Longlei
Adebiyi, Adeyemi A.
Ryder, Claire L.
Mahowald, Natalie M.
Kok, Jasper F.
author_sort Meng, Jun
collection PubMed
description Aircraft measurement campaigns have revealed that super coarse dust (diameter >10 μm) surprisingly accounts for approximately a quarter of aerosols by mass in the atmosphere. However, most global aerosol models either underestimate or do not include super coarse dust abundance. To address this problem, we use brittle fragmentation theory to develop a parameterization for the emitted dust size distribution that includes emission of super coarse dust. We implement this parameterization in the Community Earth System Model (CESM) and find that it brings the model in good agreement with aircraft measurements of super coarse dust close to dust source regions. However, the CESM still underestimates super coarse dust in dust outflow regions. Thus, we conclude that the model underestimation of super coarse atmospheric dust is in part due to the underestimation of super coarse dust emission and likely in part due to errors in deposition processes.
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spelling pubmed-92866262022-07-19 Improved Parameterization for the Size Distribution of Emitted Dust Aerosols Reduces Model Underestimation of Super Coarse Dust Meng, Jun Huang, Yue Leung, Danny M. Li, Longlei Adebiyi, Adeyemi A. Ryder, Claire L. Mahowald, Natalie M. Kok, Jasper F. Geophys Res Lett Research Letter Aircraft measurement campaigns have revealed that super coarse dust (diameter >10 μm) surprisingly accounts for approximately a quarter of aerosols by mass in the atmosphere. However, most global aerosol models either underestimate or do not include super coarse dust abundance. To address this problem, we use brittle fragmentation theory to develop a parameterization for the emitted dust size distribution that includes emission of super coarse dust. We implement this parameterization in the Community Earth System Model (CESM) and find that it brings the model in good agreement with aircraft measurements of super coarse dust close to dust source regions. However, the CESM still underestimates super coarse dust in dust outflow regions. Thus, we conclude that the model underestimation of super coarse atmospheric dust is in part due to the underestimation of super coarse dust emission and likely in part due to errors in deposition processes. John Wiley and Sons Inc. 2022-04-19 2022-04-28 /pmc/articles/PMC9286626/ /pubmed/35866061 http://dx.doi.org/10.1029/2021GL097287 Text en © 2022. The Authors. https://creativecommons.org/licenses/by/4.0/This is an open access article under the terms of the http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) License, which permits use, distribution and reproduction in any medium, provided the original work is properly cited.
spellingShingle Research Letter
Meng, Jun
Huang, Yue
Leung, Danny M.
Li, Longlei
Adebiyi, Adeyemi A.
Ryder, Claire L.
Mahowald, Natalie M.
Kok, Jasper F.
Improved Parameterization for the Size Distribution of Emitted Dust Aerosols Reduces Model Underestimation of Super Coarse Dust
title Improved Parameterization for the Size Distribution of Emitted Dust Aerosols Reduces Model Underestimation of Super Coarse Dust
title_full Improved Parameterization for the Size Distribution of Emitted Dust Aerosols Reduces Model Underestimation of Super Coarse Dust
title_fullStr Improved Parameterization for the Size Distribution of Emitted Dust Aerosols Reduces Model Underestimation of Super Coarse Dust
title_full_unstemmed Improved Parameterization for the Size Distribution of Emitted Dust Aerosols Reduces Model Underestimation of Super Coarse Dust
title_short Improved Parameterization for the Size Distribution of Emitted Dust Aerosols Reduces Model Underestimation of Super Coarse Dust
title_sort improved parameterization for the size distribution of emitted dust aerosols reduces model underestimation of super coarse dust
topic Research Letter
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9286626/
https://www.ncbi.nlm.nih.gov/pubmed/35866061
http://dx.doi.org/10.1029/2021GL097287
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