Protein-Based Flexible Conductive Aerogels for Piezoresistive Pressure Sensors

[Image: see text] Gelatin is an excellent gelling agent and is widely employed for hydrogel formation. Because of the poor mechanical properties of gelatin when dry, gelatin-aerogels are comparatively rare. Herein we demonstrate that protein nanofibrils can be employed to improve the mechanical properties of gelatin aerogels, and the materials can moreover be functionalized with a an electrically conductive polyelectrolyte resulting in formation of an elastic electrically conductive aerogel that can be employed as a piezoresistive pressure sensor. The aerogel sensor shows a good linear relationship in a wide pressure range (1.8–300 kPa) with a sensitivity of 1.8 kPa(–1). This work presents a convenient way to produce electrically conductive elastic aerogels from low-cost protein precursors.