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Energy-efficient pathway for selectively exciting solute molecules to high vibrational states via solvent vibration-polariton pumping
Selectively exciting target molecules to high vibrational states is inefficient in the liquid phase, which restricts the use of IR pumping to catalyze ground-state chemical reactions. Here, we demonstrate that this inefficiency can sometimes be solved by confining the liquid to an optical cavity und...
Autores principales: | , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2022
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9300737/ https://www.ncbi.nlm.nih.gov/pubmed/35858927 http://dx.doi.org/10.1038/s41467-022-31703-8 |