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Energy-efficient pathway for selectively exciting solute molecules to high vibrational states via solvent vibration-polariton pumping

Selectively exciting target molecules to high vibrational states is inefficient in the liquid phase, which restricts the use of IR pumping to catalyze ground-state chemical reactions. Here, we demonstrate that this inefficiency can sometimes be solved by confining the liquid to an optical cavity und...

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Detalles Bibliográficos
Autores principales: Li, Tao E., Nitzan, Abraham, Subotnik, Joseph E.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9300737/
https://www.ncbi.nlm.nih.gov/pubmed/35858927
http://dx.doi.org/10.1038/s41467-022-31703-8

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