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Narrow and Stable Single Photon Emission from Dibenzoterrylene in para‐Terphenyl Nanocrystals
Single organic molecules are promising photon sources for quantum technologies. In this work we show photon emission from dibenzoterrylene, a widely used organic emitter, in a new host matrix, para‐terphenyl. We present a reprecipitation growth method that produces para‐terphenyl nanocrystals which...
Autores principales: | , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
John Wiley and Sons Inc.
2022
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9302619/ https://www.ncbi.nlm.nih.gov/pubmed/34905640 http://dx.doi.org/10.1002/cphc.202100809 |
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author | Schofield, Ross C. Burdekin, Paul Fasoulakis, Anastasios Devanz, Louise Bogusz, Dominika P. Hoggarth, Rowan A. Major, Kyle D. Clark, Alex S. |
author_facet | Schofield, Ross C. Burdekin, Paul Fasoulakis, Anastasios Devanz, Louise Bogusz, Dominika P. Hoggarth, Rowan A. Major, Kyle D. Clark, Alex S. |
author_sort | Schofield, Ross C. |
collection | PubMed |
description | Single organic molecules are promising photon sources for quantum technologies. In this work we show photon emission from dibenzoterrylene, a widely used organic emitter, in a new host matrix, para‐terphenyl. We present a reprecipitation growth method that produces para‐terphenyl nanocrystals which are ideal for integration into nanophotonic devices due to their small size. We characterise the optical properties of dibenzoterrylene in nanocrystals at room and cryogenic temperatures, showing bright, narrow emission from a single molecule. Spectral data on the vibrational energies is presented and a further 25 additional molecules are characterised. This emitter‐host combination has potential for quantum technology purposes with wavelengths suitable for interfacing with quantum memories. |
format | Online Article Text |
id | pubmed-9302619 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2022 |
publisher | John Wiley and Sons Inc. |
record_format | MEDLINE/PubMed |
spelling | pubmed-93026192022-07-22 Narrow and Stable Single Photon Emission from Dibenzoterrylene in para‐Terphenyl Nanocrystals Schofield, Ross C. Burdekin, Paul Fasoulakis, Anastasios Devanz, Louise Bogusz, Dominika P. Hoggarth, Rowan A. Major, Kyle D. Clark, Alex S. Chemphyschem Research Articles Single organic molecules are promising photon sources for quantum technologies. In this work we show photon emission from dibenzoterrylene, a widely used organic emitter, in a new host matrix, para‐terphenyl. We present a reprecipitation growth method that produces para‐terphenyl nanocrystals which are ideal for integration into nanophotonic devices due to their small size. We characterise the optical properties of dibenzoterrylene in nanocrystals at room and cryogenic temperatures, showing bright, narrow emission from a single molecule. Spectral data on the vibrational energies is presented and a further 25 additional molecules are characterised. This emitter‐host combination has potential for quantum technology purposes with wavelengths suitable for interfacing with quantum memories. John Wiley and Sons Inc. 2022-01-12 2022-02-16 /pmc/articles/PMC9302619/ /pubmed/34905640 http://dx.doi.org/10.1002/cphc.202100809 Text en © 2021 The Authors. ChemPhysChem published by Wiley-VCH GmbH https://creativecommons.org/licenses/by/4.0/This is an open access article under the terms of the http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) License, which permits use, distribution and reproduction in any medium, provided the original work is properly cited. |
spellingShingle | Research Articles Schofield, Ross C. Burdekin, Paul Fasoulakis, Anastasios Devanz, Louise Bogusz, Dominika P. Hoggarth, Rowan A. Major, Kyle D. Clark, Alex S. Narrow and Stable Single Photon Emission from Dibenzoterrylene in para‐Terphenyl Nanocrystals |
title | Narrow and Stable Single Photon Emission from Dibenzoterrylene in para‐Terphenyl Nanocrystals |
title_full | Narrow and Stable Single Photon Emission from Dibenzoterrylene in para‐Terphenyl Nanocrystals |
title_fullStr | Narrow and Stable Single Photon Emission from Dibenzoterrylene in para‐Terphenyl Nanocrystals |
title_full_unstemmed | Narrow and Stable Single Photon Emission from Dibenzoterrylene in para‐Terphenyl Nanocrystals |
title_short | Narrow and Stable Single Photon Emission from Dibenzoterrylene in para‐Terphenyl Nanocrystals |
title_sort | narrow and stable single photon emission from dibenzoterrylene in para‐terphenyl nanocrystals |
topic | Research Articles |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9302619/ https://www.ncbi.nlm.nih.gov/pubmed/34905640 http://dx.doi.org/10.1002/cphc.202100809 |
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