Aerosol Jet Printing of Hybrid Ti(3)C(2)T( x )/C Nanospheres for Planar Micro-supercapacitors

When utilized in energy devices, the restacking tendency of MXene Ti(3)C(2)T( x ) inhibits its electrochemical performance. Using aerosol jet printing (AJP) technology, hybrid Ti(3)C(2)T( x )/C nanospheres are synthesized with C nanoparticle-bonded MXene nanosheets, and the restacking of MXene nanos...

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Autores principales: Wu, Yu, Lin, Aiping, Zhang, Jidi, Zhao, Danjiao, Fan, Lanlan, Lu, Cheng, Wang, Shufen, Cao, Lei, Gu, Feng
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Frontiers Media S.A. 2022
Materias:
Chemistry
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9304703/
https://www.ncbi.nlm.nih.gov/pubmed/35873057
http://dx.doi.org/10.3389/fchem.2022.933319
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author Wu, Yu
Lin, Aiping
Zhang, Jidi
Zhao, Danjiao
Fan, Lanlan
Lu, Cheng
Wang, Shufen
Cao, Lei
Gu, Feng
author_facet Wu, Yu
Lin, Aiping
Zhang, Jidi
Zhao, Danjiao
Fan, Lanlan
Lu, Cheng
Wang, Shufen
Cao, Lei
Gu, Feng
author_sort Wu, Yu
collection PubMed
description When utilized in energy devices, the restacking tendency of MXene Ti(3)C(2)T( x ) inhibits its electrochemical performance. Using aerosol jet printing (AJP) technology, hybrid Ti(3)C(2)T( x )/C nanospheres are synthesized with C nanoparticle-bonded MXene nanosheets, and the restacking of MXene nanosheets is blocked efficiently. The formation mechanism for hybrid Ti(3)C(2)T( x )/C nanospheres has been hypothesized, and the Ti(3)C(2)T( x )/C is anticipated to assemble and shape along the droplet surface in tandem with the Marangoni flow within the droplet. The planar microsupercapacitor devices generated from these hybrid spherical nanostructures with increased interlayer spacing exhibit exceptional areal capacitance performance. This concept offers a straightforward and effective method for constructing 3D-structured MXene with suppressed self-stacking for diverse high-performance micro energy storage devices.
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spelling pubmed-93047032022-07-23 Aerosol Jet Printing of Hybrid Ti(3)C(2)T( x )/C Nanospheres for Planar Micro-supercapacitors Wu, Yu Lin, Aiping Zhang, Jidi Zhao, Danjiao Fan, Lanlan Lu, Cheng Wang, Shufen Cao, Lei Gu, Feng Front Chem Chemistry When utilized in energy devices, the restacking tendency of MXene Ti(3)C(2)T( x ) inhibits its electrochemical performance. Using aerosol jet printing (AJP) technology, hybrid Ti(3)C(2)T( x )/C nanospheres are synthesized with C nanoparticle-bonded MXene nanosheets, and the restacking of MXene nanosheets is blocked efficiently. The formation mechanism for hybrid Ti(3)C(2)T( x )/C nanospheres has been hypothesized, and the Ti(3)C(2)T( x )/C is anticipated to assemble and shape along the droplet surface in tandem with the Marangoni flow within the droplet. The planar microsupercapacitor devices generated from these hybrid spherical nanostructures with increased interlayer spacing exhibit exceptional areal capacitance performance. This concept offers a straightforward and effective method for constructing 3D-structured MXene with suppressed self-stacking for diverse high-performance micro energy storage devices. Frontiers Media S.A. 2022-07-08 /pmc/articles/PMC9304703/ /pubmed/35873057 http://dx.doi.org/10.3389/fchem.2022.933319 Text en Copyright © 2022 Wu, Lin, Zhang, Zhao, Fan, Lu, Wang, Cao and Gu. https://creativecommons.org/licenses/by/4.0/This is an open-access article distributed under the terms of the Creative Commons Attribution License (CC BY). The use, distribution or reproduction in other forums is permitted, provided the original author(s) and the copyright owner(s) are credited and that the original publication in this journal is cited, in accordance with accepted academic practice. No use, distribution or reproduction is permitted which does not comply with these terms.
spellingShingle Chemistry
Wu, Yu
Lin, Aiping
Zhang, Jidi
Zhao, Danjiao
Fan, Lanlan
Lu, Cheng
Wang, Shufen
Cao, Lei
Gu, Feng
Aerosol Jet Printing of Hybrid Ti(3)C(2)T( x )/C Nanospheres for Planar Micro-supercapacitors
title Aerosol Jet Printing of Hybrid Ti(3)C(2)T( x )/C Nanospheres for Planar Micro-supercapacitors
title_full Aerosol Jet Printing of Hybrid Ti(3)C(2)T( x )/C Nanospheres for Planar Micro-supercapacitors
title_fullStr Aerosol Jet Printing of Hybrid Ti(3)C(2)T( x )/C Nanospheres for Planar Micro-supercapacitors
title_full_unstemmed Aerosol Jet Printing of Hybrid Ti(3)C(2)T( x )/C Nanospheres for Planar Micro-supercapacitors
title_short Aerosol Jet Printing of Hybrid Ti(3)C(2)T( x )/C Nanospheres for Planar Micro-supercapacitors
title_sort aerosol jet printing of hybrid ti(3)c(2)t( x )/c nanospheres for planar micro-supercapacitors
topic Chemistry
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9304703/
https://www.ncbi.nlm.nih.gov/pubmed/35873057
http://dx.doi.org/10.3389/fchem.2022.933319
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