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Selective Control of Eu(3+) Radiative Emission by Hyperbolic Metamaterials

In recent years the quest for novel materials possessing peculiar abilities of manipulating light at the nanoscale has been significantly boosted due to the strict demands of advanced nanophotonics and quantum technologies. In this framework radiative decay engineering of quantum emitters is of para...

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Autores principales: Genchi, Domenico, Kalinic, Boris, Balasa, Ionut Gabriel, Cesca, Tiziana, Mattei, Giovanni
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9322813/
https://www.ncbi.nlm.nih.gov/pubmed/35888390
http://dx.doi.org/10.3390/ma15144923
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author Genchi, Domenico
Kalinic, Boris
Balasa, Ionut Gabriel
Cesca, Tiziana
Mattei, Giovanni
author_facet Genchi, Domenico
Kalinic, Boris
Balasa, Ionut Gabriel
Cesca, Tiziana
Mattei, Giovanni
author_sort Genchi, Domenico
collection PubMed
description In recent years the quest for novel materials possessing peculiar abilities of manipulating light at the nanoscale has been significantly boosted due to the strict demands of advanced nanophotonics and quantum technologies. In this framework radiative decay engineering of quantum emitters is of paramount importance for developing efficient single-photon sources or nanolasers. Hyperbolic metamaterials stand out among the best cutting-edge candidates for photoluminescence control owing to their potentially unlimited photonic density of states and their ability to sustain high-k modes that allow us to strongly enhance the radiative decay rate of quantum light emitters. The aim of the present paper is to show how Au/ [Formula: see text] hyperbolic multilayers can be used to selectively control the photoluminescence of coupled [Formula: see text] emitters. We point out an enhancement of the [Formula: see text] transitions when they are in the hyperbolic regime of the metamaterials and a significant alteration of the ED and MD branching ratios by changing the emitter–metamaterial distance.
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spelling pubmed-93228132022-07-27 Selective Control of Eu(3+) Radiative Emission by Hyperbolic Metamaterials Genchi, Domenico Kalinic, Boris Balasa, Ionut Gabriel Cesca, Tiziana Mattei, Giovanni Materials (Basel) Article In recent years the quest for novel materials possessing peculiar abilities of manipulating light at the nanoscale has been significantly boosted due to the strict demands of advanced nanophotonics and quantum technologies. In this framework radiative decay engineering of quantum emitters is of paramount importance for developing efficient single-photon sources or nanolasers. Hyperbolic metamaterials stand out among the best cutting-edge candidates for photoluminescence control owing to their potentially unlimited photonic density of states and their ability to sustain high-k modes that allow us to strongly enhance the radiative decay rate of quantum light emitters. The aim of the present paper is to show how Au/ [Formula: see text] hyperbolic multilayers can be used to selectively control the photoluminescence of coupled [Formula: see text] emitters. We point out an enhancement of the [Formula: see text] transitions when they are in the hyperbolic regime of the metamaterials and a significant alteration of the ED and MD branching ratios by changing the emitter–metamaterial distance. MDPI 2022-07-15 /pmc/articles/PMC9322813/ /pubmed/35888390 http://dx.doi.org/10.3390/ma15144923 Text en © 2022 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Genchi, Domenico
Kalinic, Boris
Balasa, Ionut Gabriel
Cesca, Tiziana
Mattei, Giovanni
Selective Control of Eu(3+) Radiative Emission by Hyperbolic Metamaterials
title Selective Control of Eu(3+) Radiative Emission by Hyperbolic Metamaterials
title_full Selective Control of Eu(3+) Radiative Emission by Hyperbolic Metamaterials
title_fullStr Selective Control of Eu(3+) Radiative Emission by Hyperbolic Metamaterials
title_full_unstemmed Selective Control of Eu(3+) Radiative Emission by Hyperbolic Metamaterials
title_short Selective Control of Eu(3+) Radiative Emission by Hyperbolic Metamaterials
title_sort selective control of eu(3+) radiative emission by hyperbolic metamaterials
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9322813/
https://www.ncbi.nlm.nih.gov/pubmed/35888390
http://dx.doi.org/10.3390/ma15144923
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