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Evidence for isotropic s-wave superconductivity in high-entropy alloys

High-entropy alloys (HEA) form through the random arrangement of five or more chemical elements on a crystalline lattice. Despite the significant amount of resulting compositional disorder, a subset of HEAs enters a superconducting state below critical temperatures, [Formula: see text] K. The superc...

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Autores principales: Leung, Casey K. W., Zhang, Xiaofu, von Rohr, Fabian, Lortz, Rolf, Jäck, Berthold
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9329343/
https://www.ncbi.nlm.nih.gov/pubmed/35896621
http://dx.doi.org/10.1038/s41598-022-16355-4
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author Leung, Casey K. W.
Zhang, Xiaofu
von Rohr, Fabian
Lortz, Rolf
Jäck, Berthold
author_facet Leung, Casey K. W.
Zhang, Xiaofu
von Rohr, Fabian
Lortz, Rolf
Jäck, Berthold
author_sort Leung, Casey K. W.
collection PubMed
description High-entropy alloys (HEA) form through the random arrangement of five or more chemical elements on a crystalline lattice. Despite the significant amount of resulting compositional disorder, a subset of HEAs enters a superconducting state below critical temperatures, [Formula: see text] K. The superconducting properties of the known HEAs seem to suffice a Bardeen–Cooper–Schrieffer (BCS) description, but little is known about their superconducting order parameter and the microscopic role of disorder. We report on magnetic susceptibility measurements on films of the superconducting HEA (TaNb)[Formula: see text] (ZrHfTi)[Formula: see text] for characterizing the lower and upper critical fields [Formula: see text] and [Formula: see text] , respectively as a function of temperature T. Our resulting analysis of the Ginzburg–Landau coherence length and penetration depth demonstrates that HEAs of this type are single-band isotropic s-wave superconductors in the dirty limit. Despite a significant difference in the elemental composition between the [Formula: see text] and [Formula: see text] films, we find that the observed [Formula: see text] variations cannot be explained by disorder effects.
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spelling pubmed-93293432022-07-29 Evidence for isotropic s-wave superconductivity in high-entropy alloys Leung, Casey K. W. Zhang, Xiaofu von Rohr, Fabian Lortz, Rolf Jäck, Berthold Sci Rep Article High-entropy alloys (HEA) form through the random arrangement of five or more chemical elements on a crystalline lattice. Despite the significant amount of resulting compositional disorder, a subset of HEAs enters a superconducting state below critical temperatures, [Formula: see text] K. The superconducting properties of the known HEAs seem to suffice a Bardeen–Cooper–Schrieffer (BCS) description, but little is known about their superconducting order parameter and the microscopic role of disorder. We report on magnetic susceptibility measurements on films of the superconducting HEA (TaNb)[Formula: see text] (ZrHfTi)[Formula: see text] for characterizing the lower and upper critical fields [Formula: see text] and [Formula: see text] , respectively as a function of temperature T. Our resulting analysis of the Ginzburg–Landau coherence length and penetration depth demonstrates that HEAs of this type are single-band isotropic s-wave superconductors in the dirty limit. Despite a significant difference in the elemental composition between the [Formula: see text] and [Formula: see text] films, we find that the observed [Formula: see text] variations cannot be explained by disorder effects. Nature Publishing Group UK 2022-07-27 /pmc/articles/PMC9329343/ /pubmed/35896621 http://dx.doi.org/10.1038/s41598-022-16355-4 Text en © The Author(s) 2022 https://creativecommons.org/licenses/by/4.0/Open AccessThis article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Leung, Casey K. W.
Zhang, Xiaofu
von Rohr, Fabian
Lortz, Rolf
Jäck, Berthold
Evidence for isotropic s-wave superconductivity in high-entropy alloys
title Evidence for isotropic s-wave superconductivity in high-entropy alloys
title_full Evidence for isotropic s-wave superconductivity in high-entropy alloys
title_fullStr Evidence for isotropic s-wave superconductivity in high-entropy alloys
title_full_unstemmed Evidence for isotropic s-wave superconductivity in high-entropy alloys
title_short Evidence for isotropic s-wave superconductivity in high-entropy alloys
title_sort evidence for isotropic s-wave superconductivity in high-entropy alloys
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9329343/
https://www.ncbi.nlm.nih.gov/pubmed/35896621
http://dx.doi.org/10.1038/s41598-022-16355-4
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