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Two-Dimensional Perovskite (PEA)(2)PbI(4) Two-Color Blue-Green Photodetector

Perovskite materials have been widely used to fabricate solar cells, laser diodes and other photodevices, owing to the advantage of high absorption coefficient, long carrier life and shallow defect energy levels. However, due to easy hydrolysis, it is difficult to fabricate perovskite micro-nano dev...

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Autores principales: Dou, Wei, Yin, Ziwei, Zhang, Yi, Deng, Huiyong, Dai, Ning
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9331230/
https://www.ncbi.nlm.nih.gov/pubmed/35893524
http://dx.doi.org/10.3390/nano12152556
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author Dou, Wei
Yin, Ziwei
Zhang, Yi
Deng, Huiyong
Dai, Ning
author_facet Dou, Wei
Yin, Ziwei
Zhang, Yi
Deng, Huiyong
Dai, Ning
author_sort Dou, Wei
collection PubMed
description Perovskite materials have been widely used to fabricate solar cells, laser diodes and other photodevices, owing to the advantage of high absorption coefficient, long carrier life and shallow defect energy levels. However, due to easy hydrolysis, it is difficult to fabricate perovskite micro-nano devices. Herein, we developed a water-free device fabrication technology and fabricated a two-dimensional (C(6)H(5)C(2)H(4)NH(3))(2)PbI(4) ((PEA)(2)PbI(4)) two-color blue-green light detector, which exhibits high detection performance under the illumination of two-color lasers (λ = 460 nm, 532 nm). Compared with bulk devices, the dark current of the fabricated devices (10(−11) A) was reduced by 2 orders of magnitude. The peak responsivity and detectivity are about 1 A/W and 10(11) Jones, respectively. The photodetection performance of the device is basically the same under the two-color lasers. Our results provide a new process to fabricate perovskite microelectronic devices, and the fabricated photodetector shows great application prospects in underwater detection, owing to the blue-green window existing in water.
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spelling pubmed-93312302022-07-29 Two-Dimensional Perovskite (PEA)(2)PbI(4) Two-Color Blue-Green Photodetector Dou, Wei Yin, Ziwei Zhang, Yi Deng, Huiyong Dai, Ning Nanomaterials (Basel) Article Perovskite materials have been widely used to fabricate solar cells, laser diodes and other photodevices, owing to the advantage of high absorption coefficient, long carrier life and shallow defect energy levels. However, due to easy hydrolysis, it is difficult to fabricate perovskite micro-nano devices. Herein, we developed a water-free device fabrication technology and fabricated a two-dimensional (C(6)H(5)C(2)H(4)NH(3))(2)PbI(4) ((PEA)(2)PbI(4)) two-color blue-green light detector, which exhibits high detection performance under the illumination of two-color lasers (λ = 460 nm, 532 nm). Compared with bulk devices, the dark current of the fabricated devices (10(−11) A) was reduced by 2 orders of magnitude. The peak responsivity and detectivity are about 1 A/W and 10(11) Jones, respectively. The photodetection performance of the device is basically the same under the two-color lasers. Our results provide a new process to fabricate perovskite microelectronic devices, and the fabricated photodetector shows great application prospects in underwater detection, owing to the blue-green window existing in water. MDPI 2022-07-25 /pmc/articles/PMC9331230/ /pubmed/35893524 http://dx.doi.org/10.3390/nano12152556 Text en © 2022 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Dou, Wei
Yin, Ziwei
Zhang, Yi
Deng, Huiyong
Dai, Ning
Two-Dimensional Perovskite (PEA)(2)PbI(4) Two-Color Blue-Green Photodetector
title Two-Dimensional Perovskite (PEA)(2)PbI(4) Two-Color Blue-Green Photodetector
title_full Two-Dimensional Perovskite (PEA)(2)PbI(4) Two-Color Blue-Green Photodetector
title_fullStr Two-Dimensional Perovskite (PEA)(2)PbI(4) Two-Color Blue-Green Photodetector
title_full_unstemmed Two-Dimensional Perovskite (PEA)(2)PbI(4) Two-Color Blue-Green Photodetector
title_short Two-Dimensional Perovskite (PEA)(2)PbI(4) Two-Color Blue-Green Photodetector
title_sort two-dimensional perovskite (pea)(2)pbi(4) two-color blue-green photodetector
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9331230/
https://www.ncbi.nlm.nih.gov/pubmed/35893524
http://dx.doi.org/10.3390/nano12152556
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