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A solar tower fuel plant for the thermochemical production of kerosene from H(2)O and CO(2)

Developing solar technologies for producing carbon-neutral aviation fuels has become a global energy challenge, but their readiness level has largely been limited to laboratory-scale studies. Here, we report on the experimental demonstration of a fully integrated thermochemical production chain from...

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Autores principales: Zoller, Stefan, Koepf, Erik, Nizamian, Dustin, Stephan, Marco, Patané, Adriano, Haueter, Philipp, Romero, Manuel, González-Aguilar, José, Lieftink, Dick, de Wit, Ellart, Brendelberger, Stefan, Sizmann, Andreas, Steinfeld, Aldo
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Cell Press 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9332358/
https://www.ncbi.nlm.nih.gov/pubmed/35915707
http://dx.doi.org/10.1016/j.joule.2022.06.012
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author Zoller, Stefan
Koepf, Erik
Nizamian, Dustin
Stephan, Marco
Patané, Adriano
Haueter, Philipp
Romero, Manuel
González-Aguilar, José
Lieftink, Dick
de Wit, Ellart
Brendelberger, Stefan
Sizmann, Andreas
Steinfeld, Aldo
author_facet Zoller, Stefan
Koepf, Erik
Nizamian, Dustin
Stephan, Marco
Patané, Adriano
Haueter, Philipp
Romero, Manuel
González-Aguilar, José
Lieftink, Dick
de Wit, Ellart
Brendelberger, Stefan
Sizmann, Andreas
Steinfeld, Aldo
author_sort Zoller, Stefan
collection PubMed
description Developing solar technologies for producing carbon-neutral aviation fuels has become a global energy challenge, but their readiness level has largely been limited to laboratory-scale studies. Here, we report on the experimental demonstration of a fully integrated thermochemical production chain from H(2)O and CO(2) to kerosene using concentrated solar energy in a solar tower configuration. The co-splitting of H(2)O and CO(2) was performed via a ceria-based thermochemical redox cycle to produce a tailored mixture of H(2) and CO (syngas) with full selectivity, which was further processed to kerosene. The 50-kW solar reactor consisted of a cavity-receiver containing a reticulated porous structure directly exposed to a mean solar flux concentration of 2,500 suns. A solar-to-syngas energy conversion efficiency of 4.1% was achieved without applying heat recovery. This solar tower fuel plant was operated with a setup relevant to industrial implementation, setting a technological milestone toward the production of sustainable aviation fuels.
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spelling pubmed-93323582022-07-30 A solar tower fuel plant for the thermochemical production of kerosene from H(2)O and CO(2) Zoller, Stefan Koepf, Erik Nizamian, Dustin Stephan, Marco Patané, Adriano Haueter, Philipp Romero, Manuel González-Aguilar, José Lieftink, Dick de Wit, Ellart Brendelberger, Stefan Sizmann, Andreas Steinfeld, Aldo Joule Article Developing solar technologies for producing carbon-neutral aviation fuels has become a global energy challenge, but their readiness level has largely been limited to laboratory-scale studies. Here, we report on the experimental demonstration of a fully integrated thermochemical production chain from H(2)O and CO(2) to kerosene using concentrated solar energy in a solar tower configuration. The co-splitting of H(2)O and CO(2) was performed via a ceria-based thermochemical redox cycle to produce a tailored mixture of H(2) and CO (syngas) with full selectivity, which was further processed to kerosene. The 50-kW solar reactor consisted of a cavity-receiver containing a reticulated porous structure directly exposed to a mean solar flux concentration of 2,500 suns. A solar-to-syngas energy conversion efficiency of 4.1% was achieved without applying heat recovery. This solar tower fuel plant was operated with a setup relevant to industrial implementation, setting a technological milestone toward the production of sustainable aviation fuels. Cell Press 2022-07-20 /pmc/articles/PMC9332358/ /pubmed/35915707 http://dx.doi.org/10.1016/j.joule.2022.06.012 Text en © 2022 The Author(s) https://creativecommons.org/licenses/by/4.0/This is an open access article under the CC BY license (http://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Zoller, Stefan
Koepf, Erik
Nizamian, Dustin
Stephan, Marco
Patané, Adriano
Haueter, Philipp
Romero, Manuel
González-Aguilar, José
Lieftink, Dick
de Wit, Ellart
Brendelberger, Stefan
Sizmann, Andreas
Steinfeld, Aldo
A solar tower fuel plant for the thermochemical production of kerosene from H(2)O and CO(2)
title A solar tower fuel plant for the thermochemical production of kerosene from H(2)O and CO(2)
title_full A solar tower fuel plant for the thermochemical production of kerosene from H(2)O and CO(2)
title_fullStr A solar tower fuel plant for the thermochemical production of kerosene from H(2)O and CO(2)
title_full_unstemmed A solar tower fuel plant for the thermochemical production of kerosene from H(2)O and CO(2)
title_short A solar tower fuel plant for the thermochemical production of kerosene from H(2)O and CO(2)
title_sort solar tower fuel plant for the thermochemical production of kerosene from h(2)o and co(2)
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9332358/
https://www.ncbi.nlm.nih.gov/pubmed/35915707
http://dx.doi.org/10.1016/j.joule.2022.06.012
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