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Perovskite‐Gallium Nitride Tandem Light‐Emitting Diodes with Improved Luminance and Color Tunability

Tandem structures with different subpixels are promising for perovskite‐based multicolor electroluminescence (EL) devices in ultra‐high‐resolution full‐color displays; however, realizing excellent luminance‐ and color‐independent tunability considering the low brightness and stability of blue perovs...

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Autores principales: Li, Zong‐Tao, Zhang, Hong‐Wei, Li, Jia‐Sheng, Cao, Kai, Chen, Ziming, Xu, Liang, Ding, Xin‐Rui, Yu, Bin‐Hai, Tang, Yong, Ou, Jian‐Zhen, Kuo, Hao‐Chung, Yip, Hin‐Lap
Formato: Online Artículo Texto
Lenguaje:English
Publicado: John Wiley and Sons Inc. 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9353454/
https://www.ncbi.nlm.nih.gov/pubmed/35596610
http://dx.doi.org/10.1002/advs.202201844
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author Li, Zong‐Tao
Zhang, Hong‐Wei
Li, Jia‐Sheng
Cao, Kai
Chen, Ziming
Xu, Liang
Ding, Xin‐Rui
Yu, Bin‐Hai
Tang, Yong
Ou, Jian‐Zhen
Kuo, Hao‐Chung
Yip, Hin‐Lap
author_facet Li, Zong‐Tao
Zhang, Hong‐Wei
Li, Jia‐Sheng
Cao, Kai
Chen, Ziming
Xu, Liang
Ding, Xin‐Rui
Yu, Bin‐Hai
Tang, Yong
Ou, Jian‐Zhen
Kuo, Hao‐Chung
Yip, Hin‐Lap
author_sort Li, Zong‐Tao
collection PubMed
description Tandem structures with different subpixels are promising for perovskite‐based multicolor electroluminescence (EL) devices in ultra‐high‐resolution full‐color displays; however, realizing excellent luminance‐ and color‐independent tunability considering the low brightness and stability of blue perovskite light‐emitting diodes (PeLEDs) remains a challenge. Herein, a bright and stable blue gallium nitride (GaN) LED is utilized for vertical integration with a green MAPbBr(3) PeLED, successfully achieving a Pe‐GaN tandem LED with independently tunable luminance and color. The electronic and photonic co‐excitation (EPCE) effect is found to suppress the radiative recombination and current injection of PeLEDs, leading to degraded luminance and current efficiency under direct current modulation. Accordingly, the pulse‐width modulation is introduced to the tandem device with a negligible EPCE effect, and the average hybrid current efficiency is significantly improved by 139.5%, finally achieving a record tunable luminance (average tuning range of 16631 cd m(−2) at an arbitrary color from blue to green) for perovskite‐based multi‐color LEDs. The reported excellent independent tunability can be the starting point for perovskite‐based multicolor EL devices, enabling the combination with matured semiconductor technologies to facilitate their commercialization in advanced display applications with ultra‐high resolution.
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spelling pubmed-93534542022-08-09 Perovskite‐Gallium Nitride Tandem Light‐Emitting Diodes with Improved Luminance and Color Tunability Li, Zong‐Tao Zhang, Hong‐Wei Li, Jia‐Sheng Cao, Kai Chen, Ziming Xu, Liang Ding, Xin‐Rui Yu, Bin‐Hai Tang, Yong Ou, Jian‐Zhen Kuo, Hao‐Chung Yip, Hin‐Lap Adv Sci (Weinh) Research Articles Tandem structures with different subpixels are promising for perovskite‐based multicolor electroluminescence (EL) devices in ultra‐high‐resolution full‐color displays; however, realizing excellent luminance‐ and color‐independent tunability considering the low brightness and stability of blue perovskite light‐emitting diodes (PeLEDs) remains a challenge. Herein, a bright and stable blue gallium nitride (GaN) LED is utilized for vertical integration with a green MAPbBr(3) PeLED, successfully achieving a Pe‐GaN tandem LED with independently tunable luminance and color. The electronic and photonic co‐excitation (EPCE) effect is found to suppress the radiative recombination and current injection of PeLEDs, leading to degraded luminance and current efficiency under direct current modulation. Accordingly, the pulse‐width modulation is introduced to the tandem device with a negligible EPCE effect, and the average hybrid current efficiency is significantly improved by 139.5%, finally achieving a record tunable luminance (average tuning range of 16631 cd m(−2) at an arbitrary color from blue to green) for perovskite‐based multi‐color LEDs. The reported excellent independent tunability can be the starting point for perovskite‐based multicolor EL devices, enabling the combination with matured semiconductor technologies to facilitate their commercialization in advanced display applications with ultra‐high resolution. John Wiley and Sons Inc. 2022-05-21 /pmc/articles/PMC9353454/ /pubmed/35596610 http://dx.doi.org/10.1002/advs.202201844 Text en © 2022 The Authors. Advanced Science published by Wiley‐VCH GmbH https://creativecommons.org/licenses/by/4.0/This is an open access article under the terms of the http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) License, which permits use, distribution and reproduction in any medium, provided the original work is properly cited.
spellingShingle Research Articles
Li, Zong‐Tao
Zhang, Hong‐Wei
Li, Jia‐Sheng
Cao, Kai
Chen, Ziming
Xu, Liang
Ding, Xin‐Rui
Yu, Bin‐Hai
Tang, Yong
Ou, Jian‐Zhen
Kuo, Hao‐Chung
Yip, Hin‐Lap
Perovskite‐Gallium Nitride Tandem Light‐Emitting Diodes with Improved Luminance and Color Tunability
title Perovskite‐Gallium Nitride Tandem Light‐Emitting Diodes with Improved Luminance and Color Tunability
title_full Perovskite‐Gallium Nitride Tandem Light‐Emitting Diodes with Improved Luminance and Color Tunability
title_fullStr Perovskite‐Gallium Nitride Tandem Light‐Emitting Diodes with Improved Luminance and Color Tunability
title_full_unstemmed Perovskite‐Gallium Nitride Tandem Light‐Emitting Diodes with Improved Luminance and Color Tunability
title_short Perovskite‐Gallium Nitride Tandem Light‐Emitting Diodes with Improved Luminance and Color Tunability
title_sort perovskite‐gallium nitride tandem light‐emitting diodes with improved luminance and color tunability
topic Research Articles
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9353454/
https://www.ncbi.nlm.nih.gov/pubmed/35596610
http://dx.doi.org/10.1002/advs.202201844
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