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Recent progress on covalent organic framework materials as CO(2) reduction electrocatalysts

CO(2) emission caused by fuel combustion and human activity has caused severe climate change and other subsequent pollutions around the world. Carbon neutralization via various novel technologies to alleviate the CO(2) level in the atmosphere has thus become one of the major topics in modern researc...

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Autores principales: Fan, Yang, Chen, Mengyin, Xu, Naizhang, Wang, Kaiqiang, Gao, Qiang, Liang, Jing, Liu, Yubing
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Frontiers Media S.A. 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9355711/
https://www.ncbi.nlm.nih.gov/pubmed/35936078
http://dx.doi.org/10.3389/fchem.2022.942492
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author Fan, Yang
Chen, Mengyin
Xu, Naizhang
Wang, Kaiqiang
Gao, Qiang
Liang, Jing
Liu, Yubing
author_facet Fan, Yang
Chen, Mengyin
Xu, Naizhang
Wang, Kaiqiang
Gao, Qiang
Liang, Jing
Liu, Yubing
author_sort Fan, Yang
collection PubMed
description CO(2) emission caused by fuel combustion and human activity has caused severe climate change and other subsequent pollutions around the world. Carbon neutralization via various novel technologies to alleviate the CO(2) level in the atmosphere has thus become one of the major topics in modern research field. These advanced technologies cover CO(2) capture, storage and conversion, etc., and electrocatalytic CO(2) reduction reaction (CO(2)RR) by heterogeneous catalysts is among the most promising methods since it could utilize renewable energy and generate valuable fuels and chemicals. Covalent organic frameworks (COFs) represent crystalline organic polymers with highly rigid, conjugated structures and tunable porosity, which exhibit significant potential as heterogeneous electrocatalysts for CO(2)RR. This review briefly introduces related pioneering works in COF-based materials for electrocatalytic CO(2)RR in recent years and provides a basis for future design and synthesis of highly active and selective COF-based electrocatalysts in this direction.
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spelling pubmed-93557112022-08-06 Recent progress on covalent organic framework materials as CO(2) reduction electrocatalysts Fan, Yang Chen, Mengyin Xu, Naizhang Wang, Kaiqiang Gao, Qiang Liang, Jing Liu, Yubing Front Chem Chemistry CO(2) emission caused by fuel combustion and human activity has caused severe climate change and other subsequent pollutions around the world. Carbon neutralization via various novel technologies to alleviate the CO(2) level in the atmosphere has thus become one of the major topics in modern research field. These advanced technologies cover CO(2) capture, storage and conversion, etc., and electrocatalytic CO(2) reduction reaction (CO(2)RR) by heterogeneous catalysts is among the most promising methods since it could utilize renewable energy and generate valuable fuels and chemicals. Covalent organic frameworks (COFs) represent crystalline organic polymers with highly rigid, conjugated structures and tunable porosity, which exhibit significant potential as heterogeneous electrocatalysts for CO(2)RR. This review briefly introduces related pioneering works in COF-based materials for electrocatalytic CO(2)RR in recent years and provides a basis for future design and synthesis of highly active and selective COF-based electrocatalysts in this direction. Frontiers Media S.A. 2022-07-22 /pmc/articles/PMC9355711/ /pubmed/35936078 http://dx.doi.org/10.3389/fchem.2022.942492 Text en Copyright © 2022 Fan, Chen, Xu, Wang, Gao, Liang and Liu. https://creativecommons.org/licenses/by/4.0/This is an open-access article distributed under the terms of the Creative Commons Attribution License (CC BY). The use, distribution or reproduction in other forums is permitted, provided the original author(s) and the copyright owner(s) are credited and that the original publication in this journal is cited, in accordance with accepted academic practice. No use, distribution or reproduction is permitted which does not comply with these terms.
spellingShingle Chemistry
Fan, Yang
Chen, Mengyin
Xu, Naizhang
Wang, Kaiqiang
Gao, Qiang
Liang, Jing
Liu, Yubing
Recent progress on covalent organic framework materials as CO(2) reduction electrocatalysts
title Recent progress on covalent organic framework materials as CO(2) reduction electrocatalysts
title_full Recent progress on covalent organic framework materials as CO(2) reduction electrocatalysts
title_fullStr Recent progress on covalent organic framework materials as CO(2) reduction electrocatalysts
title_full_unstemmed Recent progress on covalent organic framework materials as CO(2) reduction electrocatalysts
title_short Recent progress on covalent organic framework materials as CO(2) reduction electrocatalysts
title_sort recent progress on covalent organic framework materials as co(2) reduction electrocatalysts
topic Chemistry
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9355711/
https://www.ncbi.nlm.nih.gov/pubmed/35936078
http://dx.doi.org/10.3389/fchem.2022.942492
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