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Spin-polarized imaging of the antiferromagnetic structure and field-tunable bound states in kagome magnet FeSn

Kagome metals are an exciting playground for the explorations of novel phenomena at the intersection of topology, electron correlations and magnetism. The family of FeSn-based kagome magnets in particular attracted a lot of attention for simplicity of the layered crystal structure and tunable topolo...

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Autores principales: Li, Hong, Zhao, He, Yin, Qiangwei, Wang, Qi, Ren, Zheng, Sharma, Shrinkhala, Lei, Hechang, Wang, Ziqiang, Zeljkovic, Ilija
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9411549/
https://www.ncbi.nlm.nih.gov/pubmed/36008460
http://dx.doi.org/10.1038/s41598-022-18678-8
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author Li, Hong
Zhao, He
Yin, Qiangwei
Wang, Qi
Ren, Zheng
Sharma, Shrinkhala
Lei, Hechang
Wang, Ziqiang
Zeljkovic, Ilija
author_facet Li, Hong
Zhao, He
Yin, Qiangwei
Wang, Qi
Ren, Zheng
Sharma, Shrinkhala
Lei, Hechang
Wang, Ziqiang
Zeljkovic, Ilija
author_sort Li, Hong
collection PubMed
description Kagome metals are an exciting playground for the explorations of novel phenomena at the intersection of topology, electron correlations and magnetism. The family of FeSn-based kagome magnets in particular attracted a lot of attention for simplicity of the layered crystal structure and tunable topological electronic band structure. Despite a significant progress in understanding their bulk properties, surface electronic and magnetic structures are yet to be fully explored in many of these systems. In this work, we focus on a prototypical kagome metal FeSn. Using a combination of spin-averaged and spin-polarized scanning tunneling microscopy, we provide the first atomic-scale visualization of the layered antiferromagnetic structure at the surface of FeSn. In contrast to the field-tunable electronic structure of cousin material Fe(3)Sn(2) that is a ferromagnet, we find that electronic density-of-states of FeSn is robust to the application of external magnetic field. Interestingly, despite the field insensitive electronic band structure, FeSn exhibits bound states tied to specific impurities with large effective moments that strongly couple to the magnetic field. Our experiments provide microscopic insights necessary for theoretical modeling of FeSn and serve as a spring board for spin-polarized measurements of topological magnets in general.
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spelling pubmed-94115492022-08-27 Spin-polarized imaging of the antiferromagnetic structure and field-tunable bound states in kagome magnet FeSn Li, Hong Zhao, He Yin, Qiangwei Wang, Qi Ren, Zheng Sharma, Shrinkhala Lei, Hechang Wang, Ziqiang Zeljkovic, Ilija Sci Rep Article Kagome metals are an exciting playground for the explorations of novel phenomena at the intersection of topology, electron correlations and magnetism. The family of FeSn-based kagome magnets in particular attracted a lot of attention for simplicity of the layered crystal structure and tunable topological electronic band structure. Despite a significant progress in understanding their bulk properties, surface electronic and magnetic structures are yet to be fully explored in many of these systems. In this work, we focus on a prototypical kagome metal FeSn. Using a combination of spin-averaged and spin-polarized scanning tunneling microscopy, we provide the first atomic-scale visualization of the layered antiferromagnetic structure at the surface of FeSn. In contrast to the field-tunable electronic structure of cousin material Fe(3)Sn(2) that is a ferromagnet, we find that electronic density-of-states of FeSn is robust to the application of external magnetic field. Interestingly, despite the field insensitive electronic band structure, FeSn exhibits bound states tied to specific impurities with large effective moments that strongly couple to the magnetic field. Our experiments provide microscopic insights necessary for theoretical modeling of FeSn and serve as a spring board for spin-polarized measurements of topological magnets in general. Nature Publishing Group UK 2022-08-25 /pmc/articles/PMC9411549/ /pubmed/36008460 http://dx.doi.org/10.1038/s41598-022-18678-8 Text en © The Author(s) 2022 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Li, Hong
Zhao, He
Yin, Qiangwei
Wang, Qi
Ren, Zheng
Sharma, Shrinkhala
Lei, Hechang
Wang, Ziqiang
Zeljkovic, Ilija
Spin-polarized imaging of the antiferromagnetic structure and field-tunable bound states in kagome magnet FeSn
title Spin-polarized imaging of the antiferromagnetic structure and field-tunable bound states in kagome magnet FeSn
title_full Spin-polarized imaging of the antiferromagnetic structure and field-tunable bound states in kagome magnet FeSn
title_fullStr Spin-polarized imaging of the antiferromagnetic structure and field-tunable bound states in kagome magnet FeSn
title_full_unstemmed Spin-polarized imaging of the antiferromagnetic structure and field-tunable bound states in kagome magnet FeSn
title_short Spin-polarized imaging of the antiferromagnetic structure and field-tunable bound states in kagome magnet FeSn
title_sort spin-polarized imaging of the antiferromagnetic structure and field-tunable bound states in kagome magnet fesn
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9411549/
https://www.ncbi.nlm.nih.gov/pubmed/36008460
http://dx.doi.org/10.1038/s41598-022-18678-8
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