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Nanopatterning of Perovskite Thin Films for Enhanced and Directional Light Emission

[Image: see text] Lead-halide perovskites offer excellent properties for lighting and display applications. Nanopatterning perovskite films could enable perovskite-based devices with designer properties, increasing their performance and adding novel functionalities. We demonstrate the potential of n...

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Autores principales: Muscarella, Loreta A., Cordaro, Andrea, Krause, Georg, Pal, Debapriya, Grimaldi, Gianluca, Antony, Leo Sahaya Daphne, Langhorst, David, Callies, Adrian, Bläsi, Benedikt, Höhn, Oliver, Koenderink, A. Femius, Polman, Albert, Ehrler, Bruno
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2022
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9412957/
https://www.ncbi.nlm.nih.gov/pubmed/35943781
http://dx.doi.org/10.1021/acsami.2c09643
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author Muscarella, Loreta A.
Cordaro, Andrea
Krause, Georg
Pal, Debapriya
Grimaldi, Gianluca
Antony, Leo Sahaya Daphne
Langhorst, David
Callies, Adrian
Bläsi, Benedikt
Höhn, Oliver
Koenderink, A. Femius
Polman, Albert
Ehrler, Bruno
author_facet Muscarella, Loreta A.
Cordaro, Andrea
Krause, Georg
Pal, Debapriya
Grimaldi, Gianluca
Antony, Leo Sahaya Daphne
Langhorst, David
Callies, Adrian
Bläsi, Benedikt
Höhn, Oliver
Koenderink, A. Femius
Polman, Albert
Ehrler, Bruno
author_sort Muscarella, Loreta A.
collection PubMed
description [Image: see text] Lead-halide perovskites offer excellent properties for lighting and display applications. Nanopatterning perovskite films could enable perovskite-based devices with designer properties, increasing their performance and adding novel functionalities. We demonstrate the potential of nanopatterning for achieving light emission of a perovskite film into a specific angular range by introducing periodic sol–gel structures between the injection and emissive layer by using substrate conformal imprint lithography (SCIL). Structural and optical characterization reveals that the emission is funnelled into a well-defined angular range by optical resonances, while the emission wavelength and the structural properties of the perovskite film are preserved. The results demonstrate a flexible and scalable approach to the patterning of perovskite layers, paving the way toward perovskite LEDs with designer angular emission patterns.
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spelling pubmed-94129572022-08-27 Nanopatterning of Perovskite Thin Films for Enhanced and Directional Light Emission Muscarella, Loreta A. Cordaro, Andrea Krause, Georg Pal, Debapriya Grimaldi, Gianluca Antony, Leo Sahaya Daphne Langhorst, David Callies, Adrian Bläsi, Benedikt Höhn, Oliver Koenderink, A. Femius Polman, Albert Ehrler, Bruno ACS Appl Mater Interfaces [Image: see text] Lead-halide perovskites offer excellent properties for lighting and display applications. Nanopatterning perovskite films could enable perovskite-based devices with designer properties, increasing their performance and adding novel functionalities. We demonstrate the potential of nanopatterning for achieving light emission of a perovskite film into a specific angular range by introducing periodic sol–gel structures between the injection and emissive layer by using substrate conformal imprint lithography (SCIL). Structural and optical characterization reveals that the emission is funnelled into a well-defined angular range by optical resonances, while the emission wavelength and the structural properties of the perovskite film are preserved. The results demonstrate a flexible and scalable approach to the patterning of perovskite layers, paving the way toward perovskite LEDs with designer angular emission patterns. American Chemical Society 2022-08-09 2022-08-24 /pmc/articles/PMC9412957/ /pubmed/35943781 http://dx.doi.org/10.1021/acsami.2c09643 Text en © 2022 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by/4.0/Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Muscarella, Loreta A.
Cordaro, Andrea
Krause, Georg
Pal, Debapriya
Grimaldi, Gianluca
Antony, Leo Sahaya Daphne
Langhorst, David
Callies, Adrian
Bläsi, Benedikt
Höhn, Oliver
Koenderink, A. Femius
Polman, Albert
Ehrler, Bruno
Nanopatterning of Perovskite Thin Films for Enhanced and Directional Light Emission
title Nanopatterning of Perovskite Thin Films for Enhanced and Directional Light Emission
title_full Nanopatterning of Perovskite Thin Films for Enhanced and Directional Light Emission
title_fullStr Nanopatterning of Perovskite Thin Films for Enhanced and Directional Light Emission
title_full_unstemmed Nanopatterning of Perovskite Thin Films for Enhanced and Directional Light Emission
title_short Nanopatterning of Perovskite Thin Films for Enhanced and Directional Light Emission
title_sort nanopatterning of perovskite thin films for enhanced and directional light emission
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9412957/
https://www.ncbi.nlm.nih.gov/pubmed/35943781
http://dx.doi.org/10.1021/acsami.2c09643
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