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Nanopatterning of Perovskite Thin Films for Enhanced and Directional Light Emission
[Image: see text] Lead-halide perovskites offer excellent properties for lighting and display applications. Nanopatterning perovskite films could enable perovskite-based devices with designer properties, increasing their performance and adding novel functionalities. We demonstrate the potential of n...
Autores principales: | , , , , , , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Chemical Society
2022
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Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9412957/ https://www.ncbi.nlm.nih.gov/pubmed/35943781 http://dx.doi.org/10.1021/acsami.2c09643 |
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author | Muscarella, Loreta A. Cordaro, Andrea Krause, Georg Pal, Debapriya Grimaldi, Gianluca Antony, Leo Sahaya Daphne Langhorst, David Callies, Adrian Bläsi, Benedikt Höhn, Oliver Koenderink, A. Femius Polman, Albert Ehrler, Bruno |
author_facet | Muscarella, Loreta A. Cordaro, Andrea Krause, Georg Pal, Debapriya Grimaldi, Gianluca Antony, Leo Sahaya Daphne Langhorst, David Callies, Adrian Bläsi, Benedikt Höhn, Oliver Koenderink, A. Femius Polman, Albert Ehrler, Bruno |
author_sort | Muscarella, Loreta A. |
collection | PubMed |
description | [Image: see text] Lead-halide perovskites offer excellent properties for lighting and display applications. Nanopatterning perovskite films could enable perovskite-based devices with designer properties, increasing their performance and adding novel functionalities. We demonstrate the potential of nanopatterning for achieving light emission of a perovskite film into a specific angular range by introducing periodic sol–gel structures between the injection and emissive layer by using substrate conformal imprint lithography (SCIL). Structural and optical characterization reveals that the emission is funnelled into a well-defined angular range by optical resonances, while the emission wavelength and the structural properties of the perovskite film are preserved. The results demonstrate a flexible and scalable approach to the patterning of perovskite layers, paving the way toward perovskite LEDs with designer angular emission patterns. |
format | Online Article Text |
id | pubmed-9412957 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2022 |
publisher | American Chemical Society |
record_format | MEDLINE/PubMed |
spelling | pubmed-94129572022-08-27 Nanopatterning of Perovskite Thin Films for Enhanced and Directional Light Emission Muscarella, Loreta A. Cordaro, Andrea Krause, Georg Pal, Debapriya Grimaldi, Gianluca Antony, Leo Sahaya Daphne Langhorst, David Callies, Adrian Bläsi, Benedikt Höhn, Oliver Koenderink, A. Femius Polman, Albert Ehrler, Bruno ACS Appl Mater Interfaces [Image: see text] Lead-halide perovskites offer excellent properties for lighting and display applications. Nanopatterning perovskite films could enable perovskite-based devices with designer properties, increasing their performance and adding novel functionalities. We demonstrate the potential of nanopatterning for achieving light emission of a perovskite film into a specific angular range by introducing periodic sol–gel structures between the injection and emissive layer by using substrate conformal imprint lithography (SCIL). Structural and optical characterization reveals that the emission is funnelled into a well-defined angular range by optical resonances, while the emission wavelength and the structural properties of the perovskite film are preserved. The results demonstrate a flexible and scalable approach to the patterning of perovskite layers, paving the way toward perovskite LEDs with designer angular emission patterns. American Chemical Society 2022-08-09 2022-08-24 /pmc/articles/PMC9412957/ /pubmed/35943781 http://dx.doi.org/10.1021/acsami.2c09643 Text en © 2022 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by/4.0/Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/). |
spellingShingle | Muscarella, Loreta A. Cordaro, Andrea Krause, Georg Pal, Debapriya Grimaldi, Gianluca Antony, Leo Sahaya Daphne Langhorst, David Callies, Adrian Bläsi, Benedikt Höhn, Oliver Koenderink, A. Femius Polman, Albert Ehrler, Bruno Nanopatterning of Perovskite Thin Films for Enhanced and Directional Light Emission |
title | Nanopatterning of
Perovskite Thin Films for Enhanced
and Directional Light Emission |
title_full | Nanopatterning of
Perovskite Thin Films for Enhanced
and Directional Light Emission |
title_fullStr | Nanopatterning of
Perovskite Thin Films for Enhanced
and Directional Light Emission |
title_full_unstemmed | Nanopatterning of
Perovskite Thin Films for Enhanced
and Directional Light Emission |
title_short | Nanopatterning of
Perovskite Thin Films for Enhanced
and Directional Light Emission |
title_sort | nanopatterning of
perovskite thin films for enhanced
and directional light emission |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9412957/ https://www.ncbi.nlm.nih.gov/pubmed/35943781 http://dx.doi.org/10.1021/acsami.2c09643 |
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