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SUPER Scheme in Action: Experimental Demonstration of Red-Detuned Excitation of a Quantum Emitter

[Image: see text] The quest for the perfect single-photon source includes finding the optimal protocol for exciting the quantum emitter. Coherent optical excitation was, up until now, achieved by tuning the laser pulses to the transition frequency of the emitter, either directly or in average. Recen...

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Detalles Bibliográficos
Autores principales: Karli, Yusuf, Kappe, Florian, Remesh, Vikas, Bracht, Thomas K., Münzberg, Julian, Covre da Silva, Saimon, Seidelmann, Tim, Axt, Vollrath Martin, Rastelli, Armando, Reiter, Doris E., Weihs, Gregor
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2022
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9413213/
https://www.ncbi.nlm.nih.gov/pubmed/35792372
http://dx.doi.org/10.1021/acs.nanolett.2c01783
Descripción
Sumario:[Image: see text] The quest for the perfect single-photon source includes finding the optimal protocol for exciting the quantum emitter. Coherent optical excitation was, up until now, achieved by tuning the laser pulses to the transition frequency of the emitter, either directly or in average. Recently, it was theoretically discovered that an excitation with two red-detuned pulses is also possible where neither of which would yield a significant upper-level population individually. We show that the so-called swing-up of quantum emitter population (SUPER) scheme can be implemented experimentally with similar properties to existing schemes by precise amplitude shaping of a broadband pulse. Because of its truly off-resonant nature, this scheme has the prospect of powering high-purity photon sources with superior photon count rate.