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SUPER Scheme in Action: Experimental Demonstration of Red-Detuned Excitation of a Quantum Emitter

[Image: see text] The quest for the perfect single-photon source includes finding the optimal protocol for exciting the quantum emitter. Coherent optical excitation was, up until now, achieved by tuning the laser pulses to the transition frequency of the emitter, either directly or in average. Recen...

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Autores principales: Karli, Yusuf, Kappe, Florian, Remesh, Vikas, Bracht, Thomas K., Münzberg, Julian, Covre da Silva, Saimon, Seidelmann, Tim, Axt, Vollrath Martin, Rastelli, Armando, Reiter, Doris E., Weihs, Gregor
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2022
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9413213/
https://www.ncbi.nlm.nih.gov/pubmed/35792372
http://dx.doi.org/10.1021/acs.nanolett.2c01783
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author Karli, Yusuf
Kappe, Florian
Remesh, Vikas
Bracht, Thomas K.
Münzberg, Julian
Covre da Silva, Saimon
Seidelmann, Tim
Axt, Vollrath Martin
Rastelli, Armando
Reiter, Doris E.
Weihs, Gregor
author_facet Karli, Yusuf
Kappe, Florian
Remesh, Vikas
Bracht, Thomas K.
Münzberg, Julian
Covre da Silva, Saimon
Seidelmann, Tim
Axt, Vollrath Martin
Rastelli, Armando
Reiter, Doris E.
Weihs, Gregor
author_sort Karli, Yusuf
collection PubMed
description [Image: see text] The quest for the perfect single-photon source includes finding the optimal protocol for exciting the quantum emitter. Coherent optical excitation was, up until now, achieved by tuning the laser pulses to the transition frequency of the emitter, either directly or in average. Recently, it was theoretically discovered that an excitation with two red-detuned pulses is also possible where neither of which would yield a significant upper-level population individually. We show that the so-called swing-up of quantum emitter population (SUPER) scheme can be implemented experimentally with similar properties to existing schemes by precise amplitude shaping of a broadband pulse. Because of its truly off-resonant nature, this scheme has the prospect of powering high-purity photon sources with superior photon count rate.
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spelling pubmed-94132132022-08-27 SUPER Scheme in Action: Experimental Demonstration of Red-Detuned Excitation of a Quantum Emitter Karli, Yusuf Kappe, Florian Remesh, Vikas Bracht, Thomas K. Münzberg, Julian Covre da Silva, Saimon Seidelmann, Tim Axt, Vollrath Martin Rastelli, Armando Reiter, Doris E. Weihs, Gregor Nano Lett [Image: see text] The quest for the perfect single-photon source includes finding the optimal protocol for exciting the quantum emitter. Coherent optical excitation was, up until now, achieved by tuning the laser pulses to the transition frequency of the emitter, either directly or in average. Recently, it was theoretically discovered that an excitation with two red-detuned pulses is also possible where neither of which would yield a significant upper-level population individually. We show that the so-called swing-up of quantum emitter population (SUPER) scheme can be implemented experimentally with similar properties to existing schemes by precise amplitude shaping of a broadband pulse. Because of its truly off-resonant nature, this scheme has the prospect of powering high-purity photon sources with superior photon count rate. American Chemical Society 2022-07-06 2022-08-24 /pmc/articles/PMC9413213/ /pubmed/35792372 http://dx.doi.org/10.1021/acs.nanolett.2c01783 Text en © 2022 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by/4.0/Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Karli, Yusuf
Kappe, Florian
Remesh, Vikas
Bracht, Thomas K.
Münzberg, Julian
Covre da Silva, Saimon
Seidelmann, Tim
Axt, Vollrath Martin
Rastelli, Armando
Reiter, Doris E.
Weihs, Gregor
SUPER Scheme in Action: Experimental Demonstration of Red-Detuned Excitation of a Quantum Emitter
title SUPER Scheme in Action: Experimental Demonstration of Red-Detuned Excitation of a Quantum Emitter
title_full SUPER Scheme in Action: Experimental Demonstration of Red-Detuned Excitation of a Quantum Emitter
title_fullStr SUPER Scheme in Action: Experimental Demonstration of Red-Detuned Excitation of a Quantum Emitter
title_full_unstemmed SUPER Scheme in Action: Experimental Demonstration of Red-Detuned Excitation of a Quantum Emitter
title_short SUPER Scheme in Action: Experimental Demonstration of Red-Detuned Excitation of a Quantum Emitter
title_sort super scheme in action: experimental demonstration of red-detuned excitation of a quantum emitter
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9413213/
https://www.ncbi.nlm.nih.gov/pubmed/35792372
http://dx.doi.org/10.1021/acs.nanolett.2c01783
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