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Vertically aligned nanocomposite (BaTiO(3))(0.8) : (La(0.7)Sr(0.3)MnO(3))(0.2) thin films with anisotropic multifunctionalities

A new two-phase BaTiO(3) : La(0.7)Sr(0.3)MnO(3) nanocomposite system with a molar ratio of 8 : 2 has been grown on single crystal SrTiO(3) (001) substrates using a one-step pulsed laser deposition technique. Vertically aligned nanocomposite thin films with ultra-thin La(0.7)Sr(0.3)MnO(3) pillars emb...

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Detalles Bibliográficos
Autores principales: Gao, Xingyao, Zhang, Di, Wang, Xuejing, Jian, Jie, He, Zihao, Dou, Hongyi, Wang, Haiyan
Formato: Online Artículo Texto
Lenguaje:English
Publicado: RSC 2020
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9419260/
https://www.ncbi.nlm.nih.gov/pubmed/36134270
http://dx.doi.org/10.1039/d0na00232a
Descripción
Sumario:A new two-phase BaTiO(3) : La(0.7)Sr(0.3)MnO(3) nanocomposite system with a molar ratio of 8 : 2 has been grown on single crystal SrTiO(3) (001) substrates using a one-step pulsed laser deposition technique. Vertically aligned nanocomposite thin films with ultra-thin La(0.7)Sr(0.3)MnO(3) pillars embedded in the BaTiO(3) matrix have been obtained and the geometry of the pillars varies with deposition frequency. The room temperature multiferroic properties, including ferromagnetism and ferroelectricity, have been demonstrated. Anisotropic ferromagnetism and dielectric constants have been observed, which can be tuned by deposition frequencies. The tunable anisotropic optical properties originated from the conducting pillars in the dielectric matrix structure, which cause different electron transport paths. In addition, tunable band gaps have been discovered in the nanocomposites. This multiferroic and anisotropic system has shown its great potentials towards multiferroics and non-linear optics.